The invention provides a stripping debonding and packaging method used for preparing graphene via continuous adhesive tape method. A device of the stripping debonding and packaging method comprises an adhesive tape reel A, an adhesive tape reel B, a graphene reel, directional pair rollers, and an adhering and stripping hand roller; the stripping debonding and packaging method is used for transferring and adhering a graphene adhesive tape prepared via the continuous adhesive tape method onto the graphene reel via manual operation of the adhering and stripping hand roller and stripping graphene tape ends; synchronous equal tension uniform speed separation of graphene tape on a graphene adhesive tape is realized at an optimal angle controlled by the directional pair rollers via independent power reverse rotation of the adhesive tape reel B and the graphene reel, and the graphene reel is winded with the obtained graphene tape. Compared with the prior art, the stripping debonding and packaging method possesses following advantages: the mechanical structure and hand tools are simple; appliance principles are clear; operation is convenient and is easy to control; high-purity indefinitely-extended graphene tape sheet with the complete graphene physicochemical properties and performance can be prepared; and an optimal raw material is provided for down-stream products in the field of graphene applications.