The invention discloses a simple method for performing coating modification on microsphere surfaces by using a two-dimensional material thin film, a simple method for stripping the two-dimensional material, and products formed by coating and stripping. In the coating process, no solvent is used, a physical friction transfer method is adopted to transfer a lamellar compound thin film from the surface of a lamellar compound sphere to the surface of the microsphere, and screening is performed to obtain the coated product by utilizing the size difference between the product (coated microsphere) and the lamellar compound sphere. The whole process has the advantages of simple technique, low cost, high efficiency and high product purity, and is suitable for industrial production. In addition, the lamellar compound can be transferred from the microsphere surface into the solution by simple ultrasonic treatment in the solution; and thus, the invention provides a simple non-chemical method for stripping the lamellar compound, which is suitable for industrial production.