The invention provides a method for quickly removing residual organophosphorus pesticides on the epidermis of vegetables and fruits. The method comprises the following steps: (1) soaking vegetables and fruits in a salt solution; (2) treating the salt solution for soaking the vegetables and fruits by adopting normal-pressure plasma; (3) carrying out vibration treatment on the salt solution for soaking the vegetables and fruits and treated by the step (2); and (4) flushing the soaked vegetables and fruits with clear water. The method can quickly remove the residual organophosphorus pesticides onthe epidermis of the vegetables and the fruits, and no extra active component susceptible to environment such as a biological enzyme is needed, and no chemical cleaning agent is needed, so that the method has high reliability, causes no secondary pollution to the vegetables and the fruits, only needs electric energy and household salt, has low costs, is safe, and is easy to popularize and apply.During the process of cleaning the vegetables and the fruits, the normal-pressure plasma also plays a certain sterilization role, and further ensures the cleanness and safety of the treated vegetablesand fruits.