A virtual reality display device, a display device, and a calculation method of a line-of-sight angle are provided. The virtual reality display device includes: a display screen configured to display a picture to a user, at least one infrared light source, and an infrared camera; and the infrared camera is on a side of the display screen away from an eye of the user, and is configured to acquire an eye image of the eye of the user that is illuminated by the at least one infrared light source.