A radioactive structure dismantling method of a heavy water reactor facility that includes a calandria including a main shell and a sub shell, a calandria vault that receives the calandria therein, and a cover assembly that covers the calandria according to an embodiment, includes: preparing dismantling of the calandria; dismantling a reactor pipe installed in the calandria; dismantling the cover assembly that covers the calandria; dismantling the calandria; and dismantling the calandria vault.