A light-adjusting structure, a method for manufacturing the light-adjusting structure, and a light-adjusting module are provided, which belong to the field of display technology, the light-adjusting structure includes: a first flexible substrate and a second flexible substrate oppositely arranged; a first transparent electrode and a second transparent electrode which are located between the first flexible substrate and the second flexible substrate; a first alignment layer located on a side of the first flexible substrate facing towards the second flexible substrate; a second alignment layer located on a side of the second flexible substrate facing towards the first flexible substrate; and a spacer and a dye liquid crystal layer which are located between the first alignment layer and the second alignment layer. The solutions of the present disclosure can meet light-adjusting requirements of vehicle windows.