Embodiments of methods for depositing silicon germanium (SiGe) layers on a substrate are disclosed herein. In some embodiments, the method includes depositing a silicon germanium seed layer atop the substrate using a first precursor comprising silicon and chlorine; and depositing a silicon germanium bulk layer atop the silicon germanium seed layer using a second precursor comprising silicon and hydrogen. In some embodiments, the first silicon precursor gas may comprise at least one of dichlorosilane (H2SiCl2), trichlorosilane (HSiCl3), or silicon tetrachloride (SiCl4). In some embodiments, the second silicon precursor gas may comprise at least one of silane (SiH4), or disilane (Si2H6).