Polyethylene-based compositions are provided that can be used, for example, in the formation of film layers. In one aspect, a composition comprises (a) a first linear low density polyethylene having a density of 0.900 to 0.915 g/cm3 and a melt index (I2) of 5.0 to 25 g/10 min, wherein the linear low density polyethylene is a blend of at least two components: (i) 20-40% by weight of a second linear low density polyethylene, wherein the second linear low density polyethylene is a homogeneously branched ethylene/α-olefin interpolymer having a density of 0.870-0.895 g/cm3 and a melt index (I2) of 2.0-6.0 g/10 min; and (ii) 60-80% by weight of a third linear low density polyethylene, wherein the density of the third linear low density polyethylene is at least 0.02 g/cm3 greater than the density of the second linear low density polyethylene and wherein the melt index (I2) of the third linear low density polyethylene is at least twice the melt index (I2) of the second linear low density polyethylene.