Disclosed is a method of producing zeolite that includes obtaining a lithium residue including aluminosilicate from lithium ore including lithium oxide; washing the lithium residue to adjust the pH of the lithium residue; adjusting a molar ratio of silicon to aluminum (Si/Al) included in the lithium residue; preparing a hydrogel by adding an alkali material to the lithium residue; and preparing crystals by crystallizing the lithium residue in the form of a hydrogel.