A method for manufacturing hybrid optical coatings and hybrid mirror assemblies, including: a) providing a first optical coating having layers of alternating high and low refractive indices of crystalline materials on a first host substrate via an epitaxial growth technique; b) providing a second optical coating having layers of alternating high and low refractive indices of dielectric materials on a second host substrate via a physical vapor deposition (PVD) technique; c) directly bonding the first optical coating to the second optical coating; and d) removing the first host substrate.