Compositions are disclosed that comprise a piezoelectric material according to Chemical Formula 1: (1−y)(NaaK1-a)(Nb1-x,Sbx)-ySrZrO3+n mol % CuO, wherein 0.01≤y≤0.10, 0.4≤a≤0.6, 0≤x≤0.06, and 0.5≤n≤1.5. The compositions can further comprise a first material, and a second material surrounded by the first material. A piezoelectric device is also described, which includes a piezoelectric device layer including a composition of Chemical Formula 1, and having a first material layer and a second material layer surrounded by the first material layer; a first electrode part disposed on a first surface of the piezoelectric device layer; and a second electrode part disposed on a second surface facing the first surface.