A method of forming a color filter substrate of a liquid crystal display device includes forming a black matrix on a substrate; attaching a color filter transfer film to the substrate, wherein the color filter transfer film includes red, green, and blue color filter patterns; irradiating a laser beam to an entirety of the color filter transfer film; removing the color filter transfer film from the substrate after the irradiating so, wherein red, green, and blue color filter patterns remain on the substrate; and curing the red, green, and blue color filter patterns remaining on the substrate.