A well-logging tool may be positioned within a borehole of a subterranean formation. The well-logging tool may include a housing having an interior defining a dual-detector receiving chamber extending longitudinally, and having first and second portions, and a first azimuthal radiation detector carried by the first portion of the dual-detector receiving chamber. The first azimuthal radiation detector may include a first gamma-ray detector and a first photodetector associated with the first gamma-ray detector. The well-logging tool may include a second spectral radiation detector carried by the second portion of the dual-detector receiving chamber. The second spectral radiation detector may include a second gamma-ray detector and a second photodetector associated with the second gamma-ray detector.