Methods of evaluating a parameter of interest of a formation intersected by a borehole, including exposing a radiation sensor in the borehole to a calibration radiation source while a measurement operation using the radiation sensor is suspended. Methods may include exposing the radiation sensor to the calibration radiation source when the radiation sensor is stationary relative to the formation or during interruption of drilling operations or at predetermined intervals; processing response information, including performing a mitigation process on a portion of the response information relating to exposure of the radiation sensor to a calibration radiation source during measurement operations; or using the calibrated measurement information to estimate parameters of interest. Devices may include a radiation sensor, a calibrator including a calibration radiation source, and an actuator configured to intermittently expose the radiation sensor to the calibration radiation source. The radiation sensor may be a spectral gamma ray detector.