Computing systems and methods for processing collected data are disclosed. In one embodiment, a method for iteratively separating a simultaneous-source dataset is provided, wherein the simultaneous-source dataset is used as an input dataset for a first iteration of simultaneous-source separation. The input dataset includes a plurality of shots that include data corresponding to a plurality of source activations. The method of iteratively separating the input dataset includes generating simulated simultaneous shots based on shots separated in the input dataset; and forming an output dataset based on the separated simultaneous shots and the simultaneous-source dataset, wherein the output dataset is configured for use as the input dataset for the next iteration of separating the simultaneous-source dataset.