The present invention relates to a method for attaching nanomaterials by using a Langmuir- Blodgett method, wherein a Langmuir-Blodgett (LB) film, which is comprised of nanomaterials, is formed from a dispersed solution where the nanomaterials are stably dispersed in a volatile organic solvent, and then the nanomaterials of the LB film are transferred to a substrate or a holder. The method according to the present invention may be desirably applied to fabrication of a nanopattern structure, or manufacture of a probe, as a mechanical and electric device, for detecting signals such as surface or chemical signals.