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    Use of metal complex compounds as catalysts for oxidation using molecular oxygen or air
    17.
    发明申请
    Use of metal complex compounds as catalysts for oxidation using molecular oxygen or air 审中-公开

    公开(公告)号：US20060019853A1

    公开(公告)日：2006-01-26

    申请号：US10531907

    申请日：2003-10-21

    申请人： Torsten Wieprecht ,  Gunther Schlingloff ,  Juntao Xia ,  Uwe Heinz ,  Abert Schneider ,  Marie-Josee Dubs ,  Frank Bachmann ,  Menno Hazekamp ,  Josef Dannacher

    发明人： Torsten Wieprecht ,  Gunther Schlingloff ,  Juntao Xia ,  Uwe Heinz ,  Abert Schneider ,  Marie-Josee Dubs ,  Frank Bachmann ,  Menno Hazekamp ,  Josef Dannacher

    IPC分类号： C07F15/00 ,  C11D3/28

    CPC分类号： C11D3/3932 ,  C11D3/168

    摘要： Use, as a catalyst for oxidation reactions using molecular oxygen and/or air, of at least one metal complex compound of formula (1) wherein Me is manganese, titanium, iron, cobalt, nickel or copper, X is a coordinating or bridging radical, n and m are each independently of the other an integer having a value of from 1 to 8, p is an integer having a value of from 0 to 32, z is the charge of the metal complex, Y is a counter-ion, q=z/(charge of Y), and L is a ligand of formula (2) wherein R1, R2, R3, R4, R5, R6, R7, R8, R9, R10 and R11 are each independently of the others hydrogen; unsubstituted or substituted C1-C18alkyl or aryl; cyano; halogen; nitro; —COOR12 or —SO3R12 wherein R12 is in each case hydrogen, a cation or unsubstituted or substituted C1-C18alkyl or aryl; —SR13, —SO2R13 or —OR13 wherein R13 is in each case hydrogen or unsubstituted or substituted C1-C18alkyl or aryl; —NR14R15; —(C1-C6alkylene)-NR14R15; —N(+)R14R15R16; —(C1-C6alkylene)-N(+)R14R15R16; —N(R13)—(C1-C6alkylene)-NR14R15; —N[(C1-C6alkylene)-NR14R15]2; —N(R13)—(C1-C6alkylene)-N(+)R14R15R16; —N[(C1-C6alkylene)-N(+)R14R15R16]2; —N(R13)—N—R14R15 or —N(R13)N″R14R15R16, wherein R13 is as defined above and R14, R15 and R16 are each independently of the other(s) hydrogen or unsubstituted or substituted C1-C18alkyl or aryl, or R14 and R15, together with the nitrogen atom linking them, form an unsubstituted or substituted 5-, 6- or 7-membered ring which may contain further hetero atoms. [LnMemXp]zYq  (1)