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    Catalyst for preparation of synthesis gas and process for preparing carbon monoxide
    1.
    发明授权
    Catalyst for preparation of synthesis gas and process for preparing carbon monoxide 失效
    用于制备合成气的催化剂和一氧化碳的制备方法

    公开(公告)号：US06376423B2

    公开(公告)日：2002-04-23

    申请号：US09254634

    申请日：1999-03-11

    申请人： Fuyuki Yagi ,  Atsuro Nagumo ,  Yukitaka Wada ,  Mitsunori Shimura ,  Sachio Asaoka ,  Shuhei Wakamatsu

    发明人： Fuyuki Yagi ,  Atsuro Nagumo ,  Yukitaka Wada ,  Mitsunori Shimura ,  Sachio Asaoka ,  Shuhei Wakamatsu

    IPC分类号： B01J2340

    CPC分类号： C01B3/40 ,  B01J23/40 ,  C01B32/40 ,  C01B2203/1064 ,  C01B2203/107 ,  C01B2203/1082 ,  Y02P20/52

    摘要： Disclosed are a catalyst for producing a synthesis gas using a carbon-containing organic compound as a raw material and a process for producing carbon monoxide. The catalyst for producing a synthesis gas is composed of a carrier formed of a metal oxide and at least one catalytic metal selected from rhodium, ruthenium, iridium, palladium and platinum and supported on the carrier and is characterized in that the catalyst has a specific surface area of 25 m2/g or less, in that the electronegativity of the metal ion of the carrier metal oxide is 13.0 or less and in that the amount of the supported catalytic metal is 0.0005-0.1 mole %, in terms of a metal, based on the carrier metal oxide. The process for producing carbon monoxide includes a step of reacting a carbon-containing organic compound with carbon dioxide in a pressurized condition to produce a synthesis gas, and a step of concentrating carbon monoxide in the thus obtained synthesis gas and is characterized in that the above-described catalyst is used as a catalyst in the synthesis gas producing step.

    摘要翻译： 公开了使用含碳有机化合物作为原料的合成气的制造催化剂和一氧化碳的制造方法。 用于生产合成气的催化剂由金属氧化物和选自铑，钌，铱，钯和铂的至少一种催化金属形成的载体组成，并载持在载体上，其特征在于催化剂具有比表面积 面积为25m 2 / g以下，其中，载体金属氧化物的金属离子的电负性为13.0以下，以金属为基准的负载催化金属的量为0.0005〜0.1摩尔％ 在载体金属氧化物上。 生产一氧化碳的方法包括在加压状态下使含碳有机化合物与二氧化碳反应以产生合成气的步骤，以及将一氧化碳浓缩在所得合成气中的步骤，其特征在于上述 在合成气生产步骤中使用描述的催化剂作为催化剂。

    Reactor employing high-temperature air combustion technology
    2.
    发明授权
    Reactor employing high-temperature air combustion technology 有权
    采用高温空气燃烧技术的反应堆

    公开(公告)号：US08403662B2

    公开(公告)日：2013-03-26

    申请号：US12665163

    申请日：2008-06-19

    申请人： Tomoyuki Mikuriya ,  Toshiaki Yoshioka ,  Ryoichi Kawabata ,  Eiji Watanabe ,  Nobuhiro Onda ,  Takeo Nikkuni ,  Shuhei Wakamatsu ,  Susumu Mochida ,  Tadahiro Araake ,  Hiroyuki Nakamura

    发明人： Tomoyuki Mikuriya ,  Toshiaki Yoshioka ,  Ryoichi Kawabata ,  Eiji Watanabe ,  Nobuhiro Onda ,  Takeo Nikkuni ,  Shuhei Wakamatsu ,  Susumu Mochida ,  Tadahiro Araake ,  Hiroyuki Nakamura

    IPC分类号： F23D14/66

    CPC分类号： F23C6/047 ,  F23C2201/301 ,  F23D14/66 ,  F23L15/02 ,  F23N2037/02 ,  F23N2037/08 ,  Y02E20/348

    摘要： A combustion air supply apparatus 9 of alternating heat exchange type supplies combustion air and discharges combustion exhaust gas at a flow velocity of 80 to 200 m/sec. A burner assembly 4 is configured in such a manner that low-caloric fuel gas is pre-heated with heat of pre-combusting high-caloric fuel gas before the low-caloric fuel gas reaches a mixing starting space CA in the combustion chamber where the pre-combusting high-caloric fuel gas and the low-caloric fuel gas come to burn together in a full scale in the mixing starting space CA. When an air amount of the combustion air supplied through the high-temperature air supply ports of the plurality of fuel gas combustion apparatuses is defined as Q1 and an air amount of the pre-combustion air to be mixed with the high-caloric fuel gas, supplied from the fuel gas combustion apparatuses, is defined as Q2, a total air amount (Q1+Q2) is 1.02 to 1.10 times more than a theoretical air amount QS required for combustion, and a ratio of Q2/(Q1+Q2) is 0.011 to 0.047.

    摘要翻译： 交替热交换型的燃烧用空气供给装置9以80〜200m /秒的流速供给燃烧空气并排出燃烧废气。 燃烧器组件4被构造成使得低热量燃料气体在预热燃烧高热量燃料气体的热量之前被预热，在低热量燃料气体到达燃烧室中的混合起始空间CA之前， 预燃烧高热量燃料气体和低热量燃料气体在混合起动空间CA中以一定范围一起燃烧。 当通过多个燃料气体燃烧装置的高温空气供给口供给的燃烧空气的空气量被定义为Q1和与高热量燃料气体混合的预燃空气的空气量时， 从燃料气体燃烧装置供给的燃料气体燃烧装置被定义为Q2，总空气量（Q1 + Q2）是燃烧所需的理论空气量QS的1.02〜1.10倍，Q2 /（Q1 + Q2）的比率 0.011〜0.047。

    REACTOR EMPLOYING HIGH-TEMPERATURE AIR COMBUSTION TECHNOLOGY
    6.
    发明申请
    REACTOR EMPLOYING HIGH-TEMPERATURE AIR COMBUSTION TECHNOLOGY 有权
    采用高温空气燃烧技术的反应器

    公开(公告)号：US20100143854A1

    公开(公告)日：2010-06-10

    申请号：US12665163

    申请日：2008-06-19

    申请人： Tomoyuki Mikuriya ,  Toshiaki Yoshioka ,  Ryoichi Kawarata ,  Eiji Watanabe ,  Nobuhiro Onda ,  Takeo Nikkuni ,  Shuhei Wakamatsu ,  Susumu Mochida ,  Tadahiro Araake ,  Hiroyuki Nakamura

    发明人： Tomoyuki Mikuriya ,  Toshiaki Yoshioka ,  Ryoichi Kawarata ,  Eiji Watanabe ,  Nobuhiro Onda ,  Takeo Nikkuni ,  Shuhei Wakamatsu ,  Susumu Mochida ,  Tadahiro Araake ,  Hiroyuki Nakamura

    IPC分类号： F23D14/66

    CPC分类号： F23C6/047 ,  F23C2201/301 ,  F23D14/66 ,  F23L15/02 ,  F23N2037/02 ,  F23N2037/08 ,  Y02E20/348

    摘要： In a burning air feeding device (9) of alternating heat-exchanging type, the feed of burning air and the discharge of a burned exhaust gas are performed at the speeds of 80 to 200 m/sec. A burner structure (4) is constituted such that a low-calorie fuel gas is preheated with the heat of a precombustion high-calorie fuel gas till the low-calorie fuel gas reaches a mixing starting zone (CA), and such that the precombustion high-calorie fuel gas and the low-calorie fuel gas are burned together in the mixing starting zone (CA). The sum (Q1+Q2) of an air quantity (Q1) fed from the hot air feeding ports of a plurality of fuel gas burning devices and an air quantity (Q2) of a precombustion air to be mixed with the high-calorie fuel gas in the plural fuel gas burning devices is set to 1.02 to 1.10 times as high as the stoichiometric air quantity (Qs) necessary for the combustion, and the ratio (Q2/(Q1+Q2)) is set within the range of 0.011 to 0.047.

    摘要翻译： 在交替热交换型的燃烧空气供给装置（9）中，以80〜200m /秒的速度进行燃烧空气的供给和燃烧废气的排出。 燃烧器结构（4）构成为使得低热量燃料气体用预燃高热量燃料气体的热量预热，直到低热量燃料气体到达混合起始区域（CA），并且使得预燃 高热量燃料气体和低热量燃料气体在混合起始区域（CA）中一起燃烧。 从多个燃料气体燃烧装置的热空气供给口供给的空气量（Q1）和与高热量燃料气体混合的预燃空气的空气量（Q2）的总和（Q1 + Q2） 在多个燃料气体燃烧装置中，设定为燃烧所需的理论空燃比（Qs）的1.02〜1.10倍，比率（Q2 /（Q1 + Q2））设定在0.011〜0.047的范围内 。

    Process for preparing synthesis gas by autothermal reforming
    10.
    发明授权
    Process for preparing synthesis gas by autothermal reforming 有权
    通过自热重整制备合成气的方法

    公开(公告)号：US06340437B1

    公开(公告)日：2002-01-22

    申请号：US09254636

    申请日：1999-03-11

    申请人： Fuyuki Yagi ,  Atsuro Nagumo ,  Yukitaka Wada ,  Mitsunori Shimura ,  Sachio Asaoka ,  Shuhei Wakamatsu

    发明人： Fuyuki Yagi ,  Atsuro Nagumo ,  Yukitaka Wada ,  Mitsunori Shimura ,  Sachio Asaoka ,  Shuhei Wakamatsu

    IPC分类号： C07C102

    CPC分类号： B01J23/40 ,  C01B3/40 ,  C01B32/40 ,  C01B2203/1064 ,  C01B2203/107 ,  C01B2203/1082 ,  Y02P20/52

    摘要： Disclosed is a process for producing a synthesis gas by an autothermal reforming method including a step of partially oxidizing a carbon-containing organic compound to produce a high temperature mixed gas, and a synthesis producing step of reacting the unreacted carbon-containing organic compound contained in the high temperature mixed gas with carbon dioxide and/or steam, wherein a catalyst having a considerably suppressed carbon deposition activity is used as a catalyst for the synthesis gas producing step. The catalyst is characterized in that the catalyst comprises a carrier formed of a metal oxide, and at least one catalytic metal selected from rhodium, ruthenium, iridium, palladium and platinum and supported on the carrier, in that the catalyst has a specific surface area of 25 m2/g or less, in that metal ion of the carrier metal oxide has electronegativity of 13.0 or less, and in that the amount of the catalytic metal supported is 0.0005-0.1 mole %, in terms of a metal, based on the carrier metal oxide.

    摘要翻译： 公开了一种通过自热重整法制备合成气的方法，该方法包括将含碳有机化合物部分氧化以产生高温混合气体的步骤，以及合成制备步骤，使含有 具有二氧化碳和/或蒸汽的高温混合气体，其中具有显着抑制的碳沉积活性的催化剂用作合成气生产步骤的催化剂。 催化剂的特征在于催化剂包含由金属氧化物形成的载体和至少一种选自铑，钌，铱，钯和铂的催化金属并负载在载体上，因为催化剂具有比表面积 25m 2 / g以下，载体金属氧化物的金属离子的电负性为13.0以下，并且，以金属为基准，载体的载体量为0.0005〜0.1摩尔％ 金属氧化物。