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    Use of a Copper (I) Complexes For Organic Luminescent Diodes
    1.
    发明申请
    Use of a Copper (I) Complexes For Organic Luminescent Diodes 有权
    用于有机发光二极管的铜（I）配合物

    公开(公告)号：US20080199731A1

    公开(公告)日：2008-08-21

    申请号：US11575554

    申请日：2005-09-20

    申请人： Arnd Vogler ,  Valeri Pawlowski ,  Hans-Werner Schmidt ,  Mukundan Thelakkat ,  Markus Bate

    发明人： Arnd Vogler ,  Valeri Pawlowski ,  Hans-Werner Schmidt ,  Mukundan Thelakkat ,  Markus Bate

    IPC分类号： H01J1/63 ,  C07F9/28

    CPC分类号： C07F1/005 ,  C08G73/00 ,  C09K11/06 ,  C09K2211/188 ,  H01L51/0059 ,  H01L51/0062 ,  H01L51/0077 ,  H01L51/5012 ,  H01L51/5096 ,  H05B33/14

    摘要： The present invention relates to the use of copper(I) complexes of the formula I where X is nitrogen or a C—R group, R is alkyl or aryl, Ar is phenyl or naphthyl, each of which is optionally substituted by from one to three radicals selected from the group consisting of alkoxy, alkylthio, alkylamino, dialkylamino, alkoxycarbonyl, alkoxysulfonyl, halogen, cyano, carboxyl, hydroxysulfonyl and nitro, and the two optionally substituted phenyl or naphthyl radicals may be joined to one another by a chemical single bond via the carbon atoms in the α- and α′-position relative to the phosphorus atom, n is 1, 2 or 3, and Y is halogen, cyano, thiocyanato, alkoxy, aryloxy, alkylthio, arylthio, alkylamino, dialkylamino, arylamino or diarylamino, in organic light-emitting diodes (OLEDs), The present invention further relates to light-emitting layers which comprise at least one copper(I) complex of the formula I, to OLEDs which comprise at least one copper(I) complex of the formula I or an inventive light-emitting layer, and to stationary visual display units which comprise inventive OLEDs.Furthermore, the present invention relates to novel copper(I) complexes of the formula Ia and Ib where R, Ar and n are each as defined in formula I, Y in formula Ia is defined as cyano, thiocyanato, alkoxy, aryloxy, alkylthio, arylthio, alkylamino, dialkylamino, arylamino or diarylamino, and Y in formula Ib is defined as halogen, cyano, thiocyanato, alkoxy, aryloxy, alkylthio, arylthio, alkylamino, dialkylamino, arylamino or diarylamino.

    摘要翻译： 本发明涉及式I的铜（I）络合物，其中X是氮或CR基团，R是烷基或芳基，Ar是苯基或萘基，其各自任选被1-3个基团取代 选自烷氧基，烷硫基，烷基氨基，二烷基氨基，烷氧基羰基，烷氧基磺酰基，卤素，氰基，羧基，羟基磺酰基和硝基，并且两个任选取代的苯基或萘基可以通过化学单键经由 氰基，氰硫基，烷氧基，芳氧基，烷硫基，芳硫基，烷基氨基，二烷基氨基，芳基氨基或二芳基氨基，其中R 1，R 2， 在有机发光二极管（OLED）中，本发明还涉及包含至少一种式I的铜（I）络合物的发光层与包含至少一种式（I）的络合物 我还是一个 透气发光层，以及包括本发明的OLED的静止视觉显示单元。 此外，本发明涉及式Ia和Ib的新型铜（I）络合物，其中R，Ar和n各自如式I中所定义，式Ia中的Y定义为氰基，氰硫基，烷氧基，芳氧基，烷硫基， 氰基，氰硫基，烷氧基，芳氧基，烷硫基，芳硫基，烷氨基，二烷基氨基，芳基氨基或二芳基氨基。

    Use of a copper (I) complexes for organic luminescent diodes
    2.
    发明授权
    Use of a copper (I) complexes for organic luminescent diodes 有权
    铜（I）配合物用于有机发光二极管

    公开(公告)号：US07858208B2

    公开(公告)日：2010-12-28

    申请号：US11575554

    申请日：2005-09-20

    申请人： Arnd Vogler ,  Valeri Pawlowski ,  Hans-Werner Schmidt ,  Mukundan Thelakkat ,  Markus Baete

    发明人： Arnd Vogler ,  Valeri Pawlowski ,  Hans-Werner Schmidt ,  Mukundan Thelakkat ,  Markus Baete

    IPC分类号： H01J1/63 ,  C07F9/28

    CPC分类号： C07F1/005 ,  C08G73/00 ,  C09K11/06 ,  C09K2211/188 ,  H01L51/0059 ,  H01L51/0062 ,  H01L51/0077 ,  H01L51/5012 ,  H01L51/5096 ,  H05B33/14

    摘要： The present invention relates to the use of copper(I) complexes of the formula I where X is nitrogen or a C—R group, R is alkyl or aryl, Ar is phenyl or naphthyl, each of which is optionally substituted by from one to three radicals selected from the group consisting of alkoxy, alkylthio, alkylamino, dialkylamino, alkoxycarbonyl, alkoxysulfonyl, halogen, cyano, carboxyl, hydroxysulfonyl and nitro, and the two optionally substituted phenyl or naphthyl radicals may be joined to one another by a chemical single bond via the carbon atoms in the α- and α′-position relative to the phosphorus atom, n is 1, 2 or 3, and Y is halogen, cyano, thiocyanato, alkoxy, aryloxy, alkylthio, arylthio, alkylamino, dialkylamino, arylamino or diarylamino, in organic light-emitting diodes (OLEDs), The present invention further relates to light-emitting layers which comprise at least one copper(I) complex of the formula I, to OLEDs which comprise at least one copper(I) complex of the formula I or an inventive light-emitting layer, and to stationary visual display units which comprise inventive OLEDs.Furthermore, the present invention relates to novel copper(I) complexes of the formula Ia and Ib where R, Ar and n are each as defined in formula I, Y in formula Ia is defined as cyano, thiocyanato, alkoxy, aryloxy, alkylthio, arylthio, alkylamino, dialkylamino, arylamino or diarylamino, and Y in formula Ib is defined as halogen, cyano, thiocyanato, alkoxy, aryloxy, alkylthio, arylthio, alkylamino, dialkylamino, arylamino or diarylamino.

    摘要翻译： 本发明涉及式I的铜（I）络合物，其中X是氮或C-R基，R是烷基或芳基，Ar是苯基或萘基，其各自任选被一个 选自烷氧基，烷硫基，烷基氨基，二烷基氨基，烷氧基羰基，烷氧基磺酰基，卤素，氰基，羧基，羟基磺酰基和硝基的三个基团和两个任选取代的苯基或萘基可以通过化学单键彼此连接 通过相对于磷原子的α-和α'-位的碳原子，n是1,2或3，Y是卤素，氰基，氰硫基，烷氧基，芳氧基，烷硫基，芳硫基，烷基氨基，二烷基氨基，芳基氨基或 在有机发光二极管（OLED）中的二芳基氨基，本发明还涉及包含至少一种式I的铜（I）配合物的发光层与包含至少一种铜（I）络合物 公式I或者inve 发光层，以及包括本发明的OLED的固定的视觉显示单元。 此外，本发明涉及式Ia和Ib的新型铜（I）络合物，其中R，Ar和n各自如式I中所定义，式Ia中的Y定义为氰基，氰硫基，烷氧基，芳氧基，烷硫基， 氰基，氰硫基，烷氧基，芳氧基，烷硫基，芳硫基，烷氨基，二烷基氨基，芳基氨基或二芳基氨基。

    Phenothiazines, S-oxides, and S,S-dioxides as well as phenoxazines as emitters for OLEDs
    6.
    发明授权
    Phenothiazines, S-oxides, and S,S-dioxides as well as phenoxazines as emitters for OLEDs 有权
    吩噻嗪，S-氧化物和S，S-二氧化物以及吩恶嗪作为OLED的发射体

    公开(公告)号：US08029919B2

    公开(公告)日：2011-10-04

    申请号：US11720274

    申请日：2005-11-25

    申请人： Thomas Gessner ,  Hans-Werner Schmidt ,  Mukundan Thelakkat ,  Markus Baete

    发明人： Thomas Gessner ,  Hans-Werner Schmidt ,  Mukundan Thelakkat ,  Markus Baete

    IPC分类号： H01L51/00

    CPC分类号： C09K11/06 ,  C07D279/26 ,  C07D279/28 ,  C07D279/34 ,  C07D417/04 ,  C07D417/10 ,  C09B19/00 ,  C09B21/00 ,  C09B23/141 ,  C09B23/145 ,  C09K2211/1033 ,  C09K2211/1037 ,  C09K2211/1044 ,  C09K2211/185 ,  H01L51/005 ,  H01L51/0052 ,  H01L51/0059 ,  H01L51/0072 ,  H01L51/0085 ,  H01L51/5012 ,  H01L51/5096 ,  H01L2251/308 ,  H05B33/14 ,  Y10S428/917

    摘要： The use of phenoxazine, phenothiazine, phenothiazine S-oxide or phenothiazine S,S-dioxide derivatives as emitter substances in organic light-emitting diodes, an organic light-emitting diode comprising a light-emitting layer, the light-emitting layer comprising at least one phenoxazine, phenothiazine, phenothiazine S-oxide or phenothiazine S,S-dioxide derivative as an emitter substance, and a light-emitting layer comprising or consisting of the aforementioned phenoxazine, phenothiazine-phenothiazine, phenothiazine S-oxide or phenothiazine S,S-dioxide derivative as an emitter substance, a hole- and exciton-blocking layer comprising or consisting of the aforementioned phenoxazine derivative, phenothiazine derivative, phenothiazine S-oxide derivative or phenothiazine S,S-dioxide derivative, and a device which comprises an inventive organic light-emitting diode. The present invention further relates to specific phenothiazine S,S-dioxide derivatives, phenothiazine S-oxide derivatives and phenothiazine derivatives and production processes thereof, and to their use in organic light-emitting diodes.

    摘要翻译： 在有机发光二极管中使用吩恶嗪，吩噻嗪，吩噻嗪S-氧化物或吩噻嗪S，S-二氧化物衍生物作为发射物质，包含发光层的有机发光二极管，至少包含发光层 一种吩恶嗪，吩噻嗪，吩噻嗪S-氧化物或吩噻嗪S，S-二氧化物衍生物作为发射体物质，以及由上述吩恶嗪，吩噻嗪 - 吩噻嗪，吩噻嗪S-氧化物或吩噻嗪S组成或组成的发光层，S- 作为发射体物质的二氧化物衍生物，包含前述吩恶嗪衍生物，吩噻嗪衍生物，吩噻嗪S-氧化物衍生物或吩噻嗪S，S-二氧化物衍生物或包含本发明有机光的器件的空穴 - 和激子阻断层 发光二极管。 本发明还涉及特定的吩噻嗪S，S-二氧化物衍生物，吩噻嗪S-氧化物衍生物和吩噻嗪衍生物及其制备方法，以及它们在有机发光二极管中的应用。

    Phenothiazines, S-Oxides, And S,S-Dioxides As Well As Phenoxazines As Emitters For Oleds
    10.
    发明申请
    Phenothiazines, S-Oxides, And S,S-Dioxides As Well As Phenoxazines As Emitters For Oleds 有权
    吩噻嗪，S-氧化物和S，S-二氧化物以及苯并恶嗪作为Oleds的发射体

    公开(公告)号：US20100308714A1

    公开(公告)日：2010-12-09

    申请号：US11720274

    申请日：2005-11-25

    申请人： Thomas Gessner ,  Hans-Werner Schmidt ,  Mukundan Thelakkat ,  Markus Baete

    发明人： Thomas Gessner ,  Hans-Werner Schmidt ,  Mukundan Thelakkat ,  Markus Baete

    IPC分类号： H01L51/00 ,  C07D279/18 ,  H01J1/62 ,  C07D417/02

    CPC分类号： C09K11/06 ,  C07D279/26 ,  C07D279/28 ,  C07D279/34 ,  C07D417/04 ,  C07D417/10 ,  C09B19/00 ,  C09B21/00 ,  C09B23/141 ,  C09B23/145 ,  C09K2211/1033 ,  C09K2211/1037 ,  C09K2211/1044 ,  C09K2211/185 ,  H01L51/005 ,  H01L51/0052 ,  H01L51/0059 ,  H01L51/0072 ,  H01L51/0085 ,  H01L51/5012 ,  H01L51/5096 ,  H01L2251/308 ,  H05B33/14 ,  Y10S428/917

    摘要： The use of phenoxazine, phenothiazine, phenothiazine S-oxide or phenothiazine S,S-dioxide derivatives as emitter substances in organic light-emitting diodes, an organic light-emitting diode comprising a light-emitting layer, the light-emitting layer comprising at least one phenoxazine, phenothiazine, phenothiazine S-oxide or phenothiazine S,S-dioxide derivative as an emitter substance, and a light-emitting layer comprising or consisting of the aforementioned phenoxazine, phenothiazine-phenothiazine, phenothiazine S-oxide or phenothiazine S,S-dioxide derivative as an emitter substance, a hole- and exciton-blocking layer comprising or consisting of the aforementioned phenoxazine derivative, phenothiazine derivative, phenothiazine S-oxide derivative or phenothiazine S,S-dioxide derivative, and a device which comprises an inventive organic light-emitting diode. The present invention further relates to specific phenothiazine S,S-dioxide derivatives, phenothiazine S-oxide derivatives and phenothiazine derivatives and production processes thereof, and to their use in organic light-emitting diodes.

    摘要翻译： 在有机发光二极管中使用吩恶嗪，吩噻嗪，吩噻嗪S-氧化物或吩噻嗪S，S-二氧化物衍生物作为发射物质，包含发光层的有机发光二极管，至少包含发光层 一种吩恶嗪，吩噻嗪，吩噻嗪S-氧化物或吩噻嗪S，S-二氧化物衍生物作为发射体物质，以及由上述吩恶嗪，吩噻嗪 - 吩噻嗪，吩噻嗪S-氧化物或吩噻嗪S组成或组成的发光层，S- 作为发射体物质的二氧化物衍生物，包含前述吩恶嗪衍生物，吩噻嗪衍生物，吩噻嗪S-氧化物衍生物或吩噻嗪S，S-二氧化物衍生物或包含本发明有机光的器件的空穴 - 和激子阻断层 发光二极管。 本发明还涉及特定的吩噻嗪S，S-二氧化物衍生物，吩噻嗪S-氧化物衍生物和吩噻嗪衍生物及其制备方法，以及它们在有机发光二极管中的应用。