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公开(公告)号：US07605295B1
公开(公告)日：2009-10-20
申请号：US12146865
申请日：2008-06-26
IPC分类号： C07C6/12
CPC分类号： C07C6/126 , C07C2521/04 , C07C2521/08 , C07C2521/12 , C07C2523/28 , C07C2523/30 , C07C2523/46 , C07C2523/75 , C07C2523/755 , C07C2529/18 , C07C2529/83 , Y02P20/125 , Y02P20/52 , C07C15/08
摘要： The subject invention comprises an aromatics complex to improve yields from a mixed aromatics feed. Through the use of a novel catalyst having higher activity and stability in a transalkylation unit in the complex, a higher xylene yield is obtained.
摘要翻译： 本发明包括芳族化合物以提高混合芳烃进料的产率。 通过使用在络合物中的烷基转移单元中具有较高活性和稳定性的新型催化剂，可获得更高的二甲苯产率。
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2.发明授权Shaped catalysts for transalkylation of aromatics for enhanced xylenes production 有权用于芳族化合物烷基转移用于增强二甲苯生产的成型催化剂公开(公告)号：US07393989B2
公开(公告)日：2008-07-01
申请号：US11678857
申请日：2007-02-26
IPC分类号： C07C6/10
CPC分类号： C07C6/126 , B01J29/18 , B01J29/40 , B01J29/80 , B01J35/026 , B01J37/0009 , B01J2229/37 , B01J2229/42 , C07C2521/04 , C07C2521/12 , C07C2529/18 , C07C2529/22 , C07C2529/24 , C07C2529/26 , C07C2529/70 , C07C2529/74 , C07C2529/76 , C07C2529/78 , C07C2529/80 , Y02P20/52 , C07C15/08 , C07C15/067
摘要： A catalyst, a process for using the catalyst whereby the catalyst effectively transalkylates C7, C9, and C10 aromatics to C8 aromatics are disclosed. The catalyst comprises a support such as mordenite plus a metal component. The catalyst provides an enhanced life and activity for carrying out the transalkylation reactions at relatively low temperatures. This is achieved by reducing the maximum particle diameter of cylindrical pellets to 1/32 inch (0.08 cm) or a trilobe to 1/16 inch (0.16 cm).
摘要翻译： 催化剂，使用催化剂的方法，其中催化剂有效地使C 7，C 9和C 10芳烷烃基烷基化至C 1 -C 10烷基， 公开了8种芳族化合物。 催化剂包括支链如丝光沸石加金属组分。 催化剂提供了在较低温度下进行烷基转移反应的寿命和活性。 这是通过将圆柱形丸粒的最大粒径减小到1/32英寸（0.08cm）或三叶至1/16英寸（0.16cm）来实现的。
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公开(公告)号：US07220885B2
公开(公告)日：2007-05-22
申请号：US10855463
申请日：2004-05-27
CPC分类号： B01J37/18 , B01J21/12 , B01J23/36 , B01J29/061 , B01J29/076 , B01J29/26 , B01J29/48 , B01J29/7815 , B01J37/0009 , B01J37/0201 , B01J37/12 , B01J37/20 , B01J2229/42 , C07C5/2737 , C07C5/2775 , C10G45/64 , Y02P20/52 , C07C15/08
摘要： A process for preparing a transalkylation catalyst, the catalyst itself, and a transalkylation process for using the catalyst are herein disclosed. The catalyst comprises rhenium metal on a solid-acid support such as mordenite, which has been treated with a sulfur-based agent. Such treatment reduces the amount of methane produced by metal hydrogenolysis in a transalkylation process wherein heavy aromatics like A9+ are reacted with toluene to produce xylenes. Reduced methane production relative to total light ends gas production results in lower hydrogen consumption and lower reactor exotherms.
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4.发明授权Shaped catalysts for transalkylation of aromatics for enhanced xylenes production 失效用于芳族化合物烷基转移用于增强二甲苯生产的成型催化剂公开(公告)号：US06815570B1
公开(公告)日：2004-11-09
申请号：US10141294
申请日：2002-05-07
IPC分类号： C07C500
CPC分类号： C07C6/126 , B01J29/18 , B01J29/40 , B01J29/80 , B01J35/026 , B01J37/0009 , B01J2229/37 , B01J2229/42 , C07C2521/04 , C07C2521/12 , C07C2529/18 , C07C2529/22 , C07C2529/24 , C07C2529/26 , C07C2529/70 , C07C2529/74 , C07C2529/76 , C07C2529/78 , C07C2529/80 , Y02P20/52 , C07C15/08 , C07C15/067
摘要： A catalyst, a process for using the catalyst whereby the catalyst effectively transalkylates C7, C9, and C10 aromatics to C8 aromatics are disclosed. The catalyst comprises a support such as mordenite plus a metal component. The catalyst provides an enhanced life and activity for carrying out the transalkylation reactions at relatively low temperatures. This is achieved by reducing the maximum particle diameter of cylindrical pellets to {fraction (1/32)} inch (0.08 cm) or a trilobe to {fraction (1/16)} inch (0.16 cm).
摘要翻译： 一种催化剂，一种使用该催化剂的方法，其中该催化剂有效地将C7，C9和C10芳族化合物烷基化为C8芳族化合物。 催化剂包括支链如丝光沸石加金属组分。 催化剂提供了在较低温度下进行烷基转移反应的寿命和活性。 这通过将圆柱形丸粒的最大粒径减小到{部分（1/32英寸（0.08cm））或三叶形至{部分（1/16英寸（0.16cm））而实现。
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公开(公告)号：US20120083635A1
公开(公告)日：2012-04-05
申请号：US12894204
申请日：2010-09-30
申请人： Edwin P. Boldingh , Antoine Negiz
发明人： Edwin P. Boldingh , Antoine Negiz
IPC分类号： C07C2/02
CPC分类号： C07C6/126 , B01J29/26 , B01J29/48 , B01J29/78 , B01J29/80 , B01J35/1019 , B01J35/1038 , B01J35/108 , B01J37/20 , B01J2229/20 , B01J2229/42 , C07C2529/78 , C07C2529/80 , Y02P20/52 , C07C15/08 , C07C15/04
摘要： A process for transalkylating aromatic hydrocarbon compounds, the process comprising introducing an aromatic hydrocarbon feed stream and a water source to a transalkylation zone. The feed stream contacts a catalyst in the transalkylation zone in the presence of water, and produces a reaction product stream comprising benzene and xylene. The invention includes methods to control the transalkylation process.
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6.发明授权公开(公告)号：US07456124B2
公开(公告)日：2008-11-25
申请号：US11843719
申请日：2007-08-23
申请人： Edwin P. Boldingh , Antoine Negiz , James E. Rekoske , Eric J. Baker , Robert B. Larson , Terrence E. Deak , Sergey V. Gurevich
发明人： Edwin P. Boldingh , Antoine Negiz , James E. Rekoske , Eric J. Baker , Robert B. Larson , Terrence E. Deak , Sergey V. Gurevich
IPC分类号： B01J29/06
CPC分类号： B01J29/80 , B01J29/26 , B01J29/48 , B01J37/0009 , B01J37/08 , B01J37/14 , B01J37/18 , B01J37/20 , B01J2229/20 , B01J2229/42 , C07C6/123 , C07C6/126 , C07C2529/18 , C07C2529/26 , C07C2529/80 , Y02P20/52 , C07C15/08
摘要： Transalkylation catalysts containing rhenium and a molecular sieve component comprising an acidic MFI molecular sieve having a Si/Al2 molar ratio of less than about 80 and mordenite provide a transalkylation product with a low content of benzene co-boilers. The invention encompasses sulfided catalyst embodiments and methods of making the catalysts.
摘要翻译： 含有铼的分子筛催化剂和包含Si / Al 2摩尔比小于约80的酸性MFI分子筛和丝光沸石的分子筛组分提供了具有低含量苯共锅炉的烷基转移产物 。 本发明包括硫化催化剂实施方案和制备催化剂的方法。
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公开(公告)号：US07273828B1
公开(公告)日：2007-09-25
申请号：US10855139
申请日：2004-05-27
申请人： Edwin P. Boldingh , Antoine Negiz
发明人： Edwin P. Boldingh , Antoine Negiz
IPC分类号： B01J27/02 , B01J21/00 , C07C2/64 , C07C15/067
CPC分类号： C07C6/126 , B01J29/005 , B01J29/26 , B01J29/48 , B01J29/7823 , B01J29/7846 , B01J29/7869 , B01J29/7884 , B01J29/7892 , B01J29/80 , B01J29/84 , B01J29/85 , B01J37/18 , B01J2229/20 , B01J2229/42 , C07C2529/26 , C07C2529/48 , C07C2529/78 , C07C2529/80 , C07C2529/85 , Y02P20/52 , C07C15/067
摘要： A process for preparing a transalkylation catalyst, the catalyst itself, and a transalkylation process for using the catalyst are herein disclosed. The catalyst comprises rhenium metal on a solid-acid support such as mordenite, which has been treated with a sulfur-based agent. Such treatment reduces the amount of methane produced by metal hydrogenolysis in a transalkylation process wherein heavy aromatics like A9+ are reacted with toluene to produce xylenes. Reduced methane production relative to total light ends gas production results in lower hydrogen consumption and lower reactor exotherms.
摘要翻译： 本文公开了制备烷基转移催化剂的方法，催化剂本身以及使用该催化剂的烷基转移方法。 该催化剂包括在固体酸性载体上的铼金属，例如已经用硫基试剂处理的丝光沸石。 这样的处理减少了在烷基转移过程中金属氢解产生的甲烷的量，其中重芳烃如A 9+与甲苯反应以产生二甲苯。 降低甲烷生产相对于总轻馏分气体生产导致较低的氢消耗和较低的反应器放热。
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公开(公告)号：US06972348B2
公开(公告)日：2005-12-06
申请号：US10807626
申请日：2004-03-24
CPC分类号： C07C6/126 , C07C2529/26 , C07C15/08
摘要： A catalyst, and a process for using the catalyst, that effectively converts and transalkylates indane and C10 and heavier polycyclic aromatics into C8 aromatics is herein disclosed. The catalyst comprises a solid-acid support such as mordenite plus a metal component such as rhenium. The catalyst provides excellent conversion of such heavy aromatic species as naphthalene, which is also observed by a decrease in the ending-boiling-point of a hydrocarbon stream passed over the catalyst. The same catalyst is also effective for transalkylation of lighter aromatics, thus yielding a valuable xylenes product stream out of the process.
摘要翻译： 本文公开了一种催化剂和使用该催化剂的方法，其有效地将茚满和C 10 N和更重的多环芳烃转化和烷基化到C 8芳烷烃中。 催化剂包括固体酸载体如丝光沸石和金属组分如铼。 该催化剂提供了诸如萘之类的重芳族物质的极好的转化率，这也是通过在催化剂上通过的烃流的终沸点降低而观察到的。 相同的催化剂对于较轻的芳族化合物的烷基转移也是有效的，因此在工艺中产生有价值的二甲苯产物流。
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公开(公告)号：US20110046427A1
公开(公告)日：2011-02-24
申请号：US12917045
申请日：2010-11-01
IPC分类号： C07C15/08
摘要： A process for aromatic transalkylation and olefin reduction of a feed stream is disclosed. Transalkylation conditions provide a product having increased xylene concentration and reduced olefin concentration relative to the feed. The process may be used in a xylene production facility to minimize or avoid the necessity of feedstock pretreatment such as hydrotreating, hydrogenation, or treating with clay and/or molecular sieves.
摘要翻译： 公开了一种进料流的芳族烷基转移和烯烃还原方法。 烷基转移条件提供了相对于进料的二甲苯浓度增加和烯烃浓度降低的产物。 该方法可用于二甲苯生产设备中以最小化或避免原料预处理（如加氢处理，氢化或用粘土和/或分子筛处理）的必要性。
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公开(公告)号：US07847137B2
公开(公告)日：2010-12-07
申请号：US11830424
申请日：2007-07-30
摘要： A process for aromatic transalkylation and olefin reduction of a feed stream is disclosed. Transalkylation conditions provide a product having increased xylene concentration and reduced olefin concentration relative to the feed. The process may be used in a xylene production facility to minimize or avoid the necessity of feedstock pretreatment such as hydrotreating, hydrogenation, or treating with clay and/or molecular sieves.
摘要翻译： 公开了一种进料流的芳族烷基转移和烯烃还原方法。 烷基转移条件提供了相对于进料的二甲苯浓度增加和烯烃浓度降低的产物。 该方法可用于二甲苯生产设备中以最小化或避免原料预处理（如加氢处理，氢化或用粘土和/或分子筛处理）的必要性。
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