The invention discloses an intelligent remote control method of solar LED lamps, which comprises the following steps of: (1) setting the full electric quantity of a storage battery and the corresponding maximal illuminating brightness of a lamp in a remote control mode; (2) detecting the residual electric quantity of the storage battery in the solar LED lamp, and regulating the illuminating brightness of the lamp to the corresponding ratio according to the ratio of the residual electric quantity of the storage battery to the full electric quantity of the storage battery; (3) setting the electronic number of the lamp in a remote control mode; (4) setting the light control sensitivity of the lamp in a remote control mode; (5) lowering the illuminating brightness of the solar LED lamp at midnight in a remote control mode, and setting the brightness changing time; and (6) repeating the step (1) to the step (5) until all lamps are set. The method can effectively regulate the illuminating brightness of the LED lamps, can prolong the illuminating time of the LED lamps, can realize the purposes of long-distance remote control regulation, setting and detection, and is convenient in operation. The invention also discloses an intelligent remote control system of the solar LED lamps.