Provided is a method for preparing a graphene-copper calcium titanate CCTO based ceramic composite dielectric material, which includes: dissolving metal ion sources in respective solvents to obtain respective solutions, and mixing the solutions evenly to obtain a precursor collosol of the CCTO based ceramic; allowing the precursor collosol of the CCTO based ceramic to stand for aging, followed by adding a graphene oxide dispersion to mix with the precursor collosol evenly, drying the resulting mixture to obtain dry precursor powders of the graphene-CCTO based ceramic, which are then grinded into fine powders, followed by irradiating by a low-power laser to obtain graphene-CCTO based ceramic composite powders; and compacting and molding the graphene-CCTO based ceramic composite powders, followed by catalytic synthesis with a high-power laser to obtain the graphene-CCTO based ceramic composite dielectric material.