Methods of providing dehumidification control in unoccupied spaces are disclosed. An illustrative method can include the steps of providing a controller having an away mode of operation adapted to provide dehumidification within the interior space of a building or room, providing one or more system components adapted to control the humidity and/or temperature within the interior space, initiating the away mode of operation within the controller, and operating the one or more system components for at least one cycle to reduce the humidity within the interior space.