A stainless steel-resin composite and method of preparing the same are provided. The method comprises providing a stainless steel substrate, spraying aluminum particles onto a first surface of the stainless steel substrate via thermal spraying to form an aluminum layer on the first surface of the stainless steel substrate, removing the aluminum layer by immersing the stainless steel substrate into an alkaline solution with a pH value greater than or equal to 10 so as to form a porous surface, and injecting a resin composition onto the porous surface of the stainless steel substrate so as to form a resin layer.