A method includes determining whether selective catalytic reduction (SCR) test conditions are present, and in response to the SCR test conditions being present, operating an SCR aftertreatment system at a number of reduced ammonia to NOx ratio (ANR) operating points. The method further includes determining a deNOx efficiency value corresponding to each of the ANR operating points. The method further includes determining a reductant correction value in response to the deNOx efficiency values corresponding to each of the ANR operating points, and providing a reductant injection command in response to the reductant correction value.