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    BIMENTAL-EXCHANGEDZEOLITE BETA FROM ORGANOTEMPLATE-FREE SYNTHESIS AND USETHEREOF IN THE SELECTIVE CATALYTIC REDUCTION OF NOx
    1.
    发明公开
    BIMENTAL-EXCHANGEDZEOLITE BETA FROM ORGANOTEMPLATE-FREE SYNTHESIS AND USETHEREOF IN THE SELECTIVE CATALYTIC REDUCTION OF NOx 审中-公开
    BIMETALL-AUSGETAUSCHTER ZEOLITH-BETA AUS ORGANOTEMPLATE-FREIER SYNTHESE UND VERWENDUNG DAVON IN DER SELKKTIVEN KATALYTISCHEN NOX-REDUKTION

    公开(公告)号：EP3097054A4

    公开(公告)日：2017-08-30

    申请号：EP14877063

    申请日：2014-12-30

    申请人： BASF SE ,  TOKYO INST TECH

    发明人： FEYEN MATHIAS ,  MAURER STEFAN ,  MÜLLER ULRICH ,  BAO XINHE ,  ZHANG WEIPING ,  DE VOS DIRK ,  GIES HERMANN ,  XIAO FENG-SHOU ,  YOKOI TOSHIYUKI ,  YILMAZ BILGE

    IPC分类号： B01J29/76 ,  B01D53/94 ,  B01J29/00 ,  C01B39/00

    CPC分类号： B01D53/9418 ,  B01D2255/20738 ,  B01D2255/20761 ,  B01D2255/502 ,  B01J29/7615 ,  B01J37/0203 ,  B01J37/04 ,  B01J37/30 ,  B01J2229/183 ,  B01J2229/186 ,  B01J2229/34 ,  C01B39/026 ,  C01B39/46

    摘要： The present invention relates to a process for the production of a zeolitic material having a BEA-type framework structure comprising YO2 and X2O3, wherein said process comprises the steps of (1) preparing a mixture comprising one or more sources for YO2 and one or more sources for X2O3; (2) crystallizing the mixture obtained in step (1); (3) subjecting the zeolitic material having a BEA-type framework structure obtained in step (2) to an ion-exchange procedure with Cu; and (4) subjecting the Cu ion-exchanged zeolitic material obtained in step (3) to an ion-exchange procedure with Fe; wherein Y is a tetravalent element, and X is a trivalent element, wherein the mixture provided in step (1) and crystallized in step (2) further comprises seed crystals comprising one or more zeolitic materials having a BEA-type framework structure, and wherein the mixture provided in step (1) and crystallized in step (2) does not contain an organotemplate as a structure-directing agent, as well as to the zeolitic material having a BEA frame work structure per se, and to its use, in particular in a method for the treatment of NOx by selective catalytic reduction (SCR).

    摘要翻译： 本发明涉及生产具有包含YO 2和X 2 O 3的BEA型骨架结构的沸石材料的方法，其中所述方法包括以下步骤：（1）制备包含一种或多种YO 2源和一种或多种 X2O3来源; （2）使步骤（1）中获得的混合物结晶; （3）使步骤（2）中获得的具有BEA型骨架结构的沸石材料与Cu进行离子交换程序; （4）将步骤（3）中获得的Cu离子交换沸石材料与Fe进行离子交换程序; 其中Y是四价元素，并且X是三价元素，其中步骤（1）中提供并在步骤（2）中结晶的混合物还包含含有一种或多种具有BEA型骨架结构的沸石材料的晶种，并且其中 在步骤（1）中提供并在步骤（2）中结晶的混合物不含有作为结构导向剂的有机模板以及具有BEA框架结构本身的沸石材料，特别是其用途 在通过选择性催化还原（SCR）处理NOx的方法中。