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    Apparatus for the two-stage selective oxidation of carbon monoxide in a hydrogen-containing gas mixture
    2.
    发明授权
    Apparatus for the two-stage selective oxidation of carbon monoxide in a hydrogen-containing gas mixture 失效
    用于含氢气体混合物中一氧化碳的两级选择性氧化的装置

    公开(公告)号：US5750076A

    公开(公告)日：1998-05-12

    申请号：US580078

    申请日：1995-12-20

    申请人： Richard F. Buswell ,  Ronald Cohen ,  Leonard McNeilly ,  David S. Watkins

    发明人： Richard F. Buswell ,  Ronald Cohen ,  Leonard McNeilly ,  David S. Watkins

    IPC分类号： B01D53/86 ,  B01J8/04 ,  C01B3/58 ,  F16K17/00 ,  B01D50/00 ,  F01N3/10 ,  G01D7/00

    CPC分类号： B01D53/864 ,  B01J8/0446 ,  C01B3/583 ,  C01B2203/044 ,  C01B2203/047

    摘要： An apparatus for the two-stage selective oxidation of carbon monoxide to carbon dioxide in a fuel stream comprising hydrogen and carbon monoxide. The apparatus includes primary and secondary reaction chambers, which deliver a hydrogen-rich outlet gas stream having a carbon monoxide concentration of less than about 5 ppm. When an increase in the carbon monoxide concentration in the outlet stream of the primary reaction chamber is detected, then the flow through the primary reaction chamber is reversed. The selective oxidizer employs a temperature-based control strategy as an oxygen-containing gas stream flow rate adjustment around the flow rate initially set in direct proportion to the fuel gas stream flow rate. The control strategy regulates the amount of oxygen-containing gas mixed with the gaseous fuel stream as a function of the difference between the temperature at a location at or near the end of the primary reaction chamber and the temperature at the outlet of the primary reaction chamber.

    摘要翻译： 一种用于在包含氢气和一氧化碳的燃料流中二氧化碳二氧化碳选择性氧化的装置。 该设备包括一级和二级反应室，其输送一氧化碳浓度小于约5ppm的富氢出口气流。 当检测到初级反应室的出口流中一氧化碳浓度的增加时，反过来，通过初级反应室的流动反向。 选择性氧化剂采用基于温度的控制策略作为围绕最初与燃料气流流量成正比设定的流速的含氧气流流量调节。 控制策略调节与气体燃料流混合的含氧气体的量作为主反应室端部处或附近的温度与初级反应室出口处的温度之差的函数的函数 。

    Method and apparatus for the two-stage selective oxidation of carbon monoxide in a hydrogen-containing gas mixture
    3.
    发明授权
    Method and apparatus for the two-stage selective oxidation of carbon monoxide in a hydrogen-containing gas mixture 失效
    用于含氢气体混合物中一氧化碳的两级选择性氧化的方法和装置

    公开(公告)号：US5518705A

    公开(公告)日：1996-05-21

    申请号：US293653

    申请日：1994-08-22

    申请人： Richard F. Buswell ,  Ronald Cohen ,  Leonard McNeilly ,  David S. Watkins

    发明人： Richard F. Buswell ,  Ronald Cohen ,  Leonard McNeilly ,  David S. Watkins

    IPC分类号： B01D53/86 ,  B01J8/04 ,  C01B3/58 ,  C01B31/20 ,  B01J8/00

    CPC分类号： B01D53/864 ,  B01J8/0446 ,  C01B3/583 ,  C01B2203/044 ,  C01B2203/047

    摘要： An apparatus and method are provided for the two-stage selective oxidation of carbon monoxide to carbon dioxide in a fuel stream comprising hydrogen and carbon monoxide. The apparatus includes primary and secondary reaction chambers, which deliver a hydrogen-rich outlet gas stream having a carbon monoxide concentration of less than about 5 ppm. When an increase in the carbon monoxide concentration in the outlet stream of the primary reaction chamber is detected, then the flow through the primary reaction chamber is reversed. The selective oxidizer employs a temperature-based control strategy as an oxygen-containing gas stream flow rate adjustment around the flow rate initially set in direct proportion to the fuel gas stream flow rate. The control strategy regulates the amount of oxygen-containing gas mixed with the gaseous fuel stream as a function of the difference between the temperature at a location at or near the end of the primary reaction chamber and the temperature at the outlet of the primary reaction chamber.

    摘要翻译： 提供了一种装置和方法，用于在包含氢气和一氧化碳的燃料流中将一氧化碳二氧化碳选择性氧化成二氧化碳。 该设备包括一级和二级反应室，其输送一氧化碳浓度小于约5ppm的富氢出口气流。 当检测到初级反应室的出口流中一氧化碳浓度的增加时，反过来，通过初级反应室的流动反向。 选择性氧化剂采用基于温度的控制策略作为围绕最初与燃料气流流量成正比设定的流速的含氧气流流量调节。 控制策略调节与气体燃料流混合的含氧气体的量作为主反应室端部处或附近的温度与初级反应室出口处的温度之差的函数的函数 。