A non-Newtonian photo-curable ink composition that includes a metal oxide/alkoxysilane complex in an amount ranging from about 0.1 wt % to about 10 wt %, a salt in an amount ranging from about 0.05 wt % to about 20 wt %, a photo-initiator, an organic solvent, and water, wherein the ink composition has a first dynamic viscosity ranging from 25 cps to 10,000 cps at a first state and a second dynamic viscosity ranging from 1 cps to 50 cps at a second state. Also described herein is a method for making such non-Newtonian photo-curable ink composition and a method for producing printed images using such non-Newtonian photo-curable ink composition.