Organic metal compounds, and organic light-emitting devices employing the same are provided. The organic metal compound has a chemical structure represented by Formula (I) or Formula (II): wherein, R1 is hydrogen, C1-12 alkyl, C1-12 alkoxy, amine, C2-6 alkenyl, C2-6 alkynyl, C5-10 cycloalkyl, C3-12 heteroaryl, or C6-12 aryl; R2, R3, R4, and R5 can be hydrogen, halogen, C1-12 alkyl, C1-12 alkoxy, C1-12 fluoroalkyl; R6 and R7 are independent and can be C1-6 alkyl, or phenyl; R8, R9, R10, R11, R12, R13, R14, and R15 can be hydrogen, halogen, C1-12 alkyl, C1-12 fluoroalkyl, or two adjacent groups of R2, R3, R4, R5, R8, R9, R10, R11, R12, R13, R14 and R15 are optionally combined with the carbon atoms which they are attached to, to form a cycloalkyl group, or aryl; m is 1 or 2; and, n is 0 or 1.