A phase-locked loop with dual-mode phase/frequency detection is provided. The phase-locked loop circuit includes a dual-mode phase/frequency detector, a loop filter, a voltage-controlled oscillator, and a frequency converter. In addition, the dual-mode phase/frequency detector includes a digital phase/frequency detector, an analog phase/frequency detector, a charge pump, and a control unit. When the phase-locked loop circuit starts, the control unit causes a detection output signal from the dual-mode phase/frequency detector to correspond to a digital signal from the digital phase/frequency detector. When the phase-locked loop circuit approaches a lock state, the control unit causes the detection output signal to correspond to an analog signal from the analog phase/frequency detector. The phase-locked loop with dual-mode phase/frequency detection has the advantages of providing linear characteristics, fast switching speed, and high sensitivity.