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1.发明授权EISEN- UND MANGANHALTIGER HETEROGENKATALYSATOR UND VERFAHREN ZUR HERSTELLUNG VON OLEFINEN DURCH UMSETZUNG VON KOHLENMONOXID MIT WASSERSTOFF 有权铁和生产烯烃THROUGH一氧化碳和氢反应用锰非均相催化剂及工艺
公开(公告)号：EP2496348B1
公开(公告)日：2016-01-06
申请号：EP10771128.5
申请日：2010-10-28
Applicant: BASF SE
Inventor： STEINER, Jochen , BAY, Kerem , WERNER, Vera , AMANN, Jürgen , BUNZEL, Stefan , MOßBACHER, Claudia , MÜLLER, Joachim , SCHWAB, Ekkehard , WEBER, Markus
IPC: B01J23/889 , B01J23/00 , B01J37/08 , C07C1/04
CPC classification number: B01J23/8892 , B01J23/002 , B01J23/005 , B01J35/023 , B01J37/0201 , B01J37/086 , B01J37/14 , B01J37/18 , B01J2523/00 , C10G2/332 , C10G2400/20 , B01J2523/72 , B01J2523/842
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2.发明公开EISEN- UND MANGANHALTIGER HETEROGENKATALYSATOR UND VERFAHREN ZUR HERSTELLUNG VON OLEFINEN DURCH UMSETZUNG VON KOHLENMONOXID MIT WASSERSTOFF 有权铁和生产烯烃THROUGH一氧化碳和氢反应用锰非均相催化剂及工艺
公开(公告)号：EP2496348A1
公开(公告)日：2012-09-12
申请号：EP10771128.5
申请日：2010-10-28
Applicant: BASF SE
Inventor： STEINER, Jochen , BAY, Kerem , WERNER, Vera , AMANN, Jürgen , BUNZEL, Stefan , MOßBACHER, Claudia , MÜLLER, Joachim , SCHWAB, Ekkehard , WEBER, Markus
IPC: B01J23/889 , B01J23/00 , B01J37/08 , C07C1/04
CPC classification number: B01J23/8892 , B01J23/002 , B01J23/005 , B01J35/023 , B01J37/0201 , B01J37/086 , B01J37/14 , B01J37/18 , B01J2523/00 , C10G2/332 , C10G2400/20 , B01J2523/72 , B01J2523/842
Abstract: The invention relates to a heterogeneous catalyst containing iron and manganese and to a method for the production thereof comprising the following steps: I. Pyrolyzing gaseous iron pentacarbonyl to yield carbonyl iron powder having spherical primary particles, II. Treating the carbonyl iron powder yielded in step I with hydrogen, wherein the metal spherical primary particles at least partially agglomerate, III. Surface oxidation of the iron particles from step II (agglomerates = secondary particles, and optionally remaining primary particles), forming iron oxide, IV. Bringing the particles from step III in contact with an aqueous solution of a manganese compound, V. Drying in the presence of oxygen and subsequent calcination in the absence of oxygen, wherein manganese compounds containing oxygen initially result on the particles, said compounds then reacting with the iron oxide, forming a mixed oxide of the formula Mn
x Fe
3-x O
4 , where 0-
3.发明公开EISEN- UND KUPFERHALTIGER HETEROGENKATALYSATOR UND VERFAHREN ZUR HERSTELLUNG VON OLEFINEN DURCH UMSETZUNG VON KOHLENMONOXID MIT WASSERSTOFF 审中-公开铁和生产烯烃THROUGH一氧化碳和氢反应用铜多相催化剂及工艺
公开(公告)号：EP2496346A1
公开(公告)日：2012-09-12
申请号：EP10771739.9
申请日：2010-10-28
Applicant: BASF SE
Inventor： STEINER, Jochen , BAY, Kerem , WERNER, Vera , AMANN, Jürgen , BUNZEL, Stefan , MOßBACHER, Claudia , MÜLLER, Joachim , SCHWAB, Ekkehard , WEBER, Markus
IPC: B01J23/745 , B01J23/72 , B01J23/00 , B01J37/08 , C07C1/04
CPC classification number: B01J23/745 , B01J23/002 , B01J23/005 , B01J23/72 , B01J23/78 , B01J35/023 , B01J37/0201 , B01J37/086 , B01J37/14 , B01J37/18 , B01J2523/00 , C07C1/044 , C07C2523/04 , C07C2523/72 , C07C2523/745 , C07C2523/885 , C10G2/332 , C10G2400/20 , C07C11/02 , B01J2523/17 , B01J2523/842
Abstract: The invention relates to a heterogeneous catalyst containing iron and copper and to a method for the production thereof comprising the following steps: I. Pyrolyzing gaseous iron pentacarbonyl to yield carbonyl iron powder having spherical primary particles, II. Treating the carbonyl iron powder yielded in step I with hydrogen, wherein the metal spherical primary particles at least partially agglomerate, III. Surface oxidation of the iron particles from step II (agglomerates = secondary particles, and optionally remaining primary particles), forming iron oxide, IV. Bringing the particles from step III in contact with an aqueous solution of a copper compound, V. Drying in the presence of oxygen and subsequent calcination in the absence of oxygen, wherein copper compounds containing oxygen initially result on the particles, which compounds then react with the iron oxide forming a mixed oxide of the formula Cu
x Fe
3-x O
4 , where 0
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