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    High-temperature adhesive of polyimide
    1.
    发明公开
    High-temperature adhesive of polyimide 失效
    聚酰亚胺的高温胶粘剂

    公开(公告)号：EP0234882A3

    公开(公告)日：1989-03-15

    申请号：EP87301478.1

    申请日：1987-02-20

    申请人： MITSUI TOATSU CHEMICALS, Inc.

    发明人： Tamai, Shoji ,  Ohta, Masahiro ,  Kawashima, Saburo ,  Oikawa, Hideaki ,  Ohkoshi, Kouji ,  Yamaguchi, Akihiro

    IPC分类号： C09J179/08 ,  C08G73/10 ,  B32B27/04

    CPC分类号： C08G73/105

    摘要： This invention discloses high-temperature adhesives having a good light-transmittance and excellent high-temperature flowability which comprises polyimide having recurring units represented by the following formula (I)
    (where R is a tetra-valent radical selected from the group consisting of aliphatic radical having not less than two carbons, cyclo-aliphatic radical, monoaromatic radical, condensed polyaromatic radical, and non condensed polyaromatic radical wherein aromatic radicals are mutally connected with a bond or a crosslinking function). The ployimide is obtained by preparing polyamic acid through the reaction of 2,2-bis[4-(3-aminophenoxy)phenyl]-1,1,1,3,3,3,-­hexafluoropropane as a diamine component with tetracarboxylic dianhydride such as pyromellitic dianhydride, 3,3ʹ,4,4ʹ-­biphenyltetracarboxylic dianhydride, bis(3,4-dicarboxyphenyl) ether dianhydride and 3,3ʹ4,4ʹ-benzophenonetetracarboxylic dianhydride, and further conducting the ring-closing reaction of resultant polyamic acid by dehydration.

    High-temperature adhesive of polyimide
    4.
    发明公开
    High-temperature adhesive of polyimide 失效
    高温聚酰亚胺粘合剂。

    公开(公告)号：EP0234882A2

    公开(公告)日：1987-09-02

    申请号：EP87301478.1

    申请日：1987-02-20

    申请人： MITSUI TOATSU CHEMICALS, Inc.

    发明人： Tamai, Shoji ,  Ohta, Masahiro ,  Kawashima, Saburo ,  Oikawa, Hideaki ,  Ohkoshi, Kouji ,  Yamaguchi, Akihiro

    IPC分类号： C09J179/08 ,  C08G73/10 ,  B32B27/04

    CPC分类号： C08G73/105

    摘要： This invention discloses high-temperature adhesives having a good light-transmittance and excellent high-temperature flowability which comprises polyimide having recurring units represented by the following formula (I)
    (where R is a tetra-valent radical selected from the group consisting of aliphatic radical having not less than two carbons, cyclo-aliphatic radical, monoaromatic radical, condensed polyaromatic radical, and non condensed polyaromatic radical wherein aromatic radicals are mutally connected with a bond or a crosslinking function).
    The ployimide is obtained by preparing polyamic acid through the reaction of 2,2-bis[4-(3-aminophenoxy)phenyl]-1,1,1,3,3,3,-­hexafluoropropane as a diamine component with tetracarboxylic dianhydride such as pyromellitic dianhydride, 3,3ʹ,4,4ʹ-­biphenyltetracarboxylic dianhydride, bis(3,4-dicarboxyphenyl) ether dianhydride and 3,3ʹ4,4ʹ-benzophenonetetracarboxylic dianhydride, and further conducting the ring-closing reaction of resultant polyamic acid by dehydration.

    Polyimide and high-temperature adhesive of polyimide
    5.
    发明公开
    Polyimide and high-temperature adhesive of polyimide 失效
    聚酰亚胺和。e e e。。nd nd nd。。。。。。

    公开(公告)号：EP0729995A1

    公开(公告)日：1996-09-04

    申请号：EP96101394.3

    申请日：1986-06-30

    申请人： MITSUI TOATSU CHEMICALS, Inc.

    发明人： Ohta, Masahiro ,  Sanobe, Yoshiho ,  Kawashima, Saburo ,  Tamai, Shoji ,  Oikawa, Hideaki ,  Yamaguchi, Akihiro ,  Ohkoshi, Kouji

    IPC分类号： C08G73/10 ,  C09J179/08

    CPC分类号： C08G73/1039 ,  C08G73/105 ,  C08G73/1064 ,  C08G73/1071 ,  C09J179/08

    摘要： Polyimide having repeating units of the following formula (I) and its polyamic acid precursor having repeating units of the following formula (II) are disclosed;
    (where Y is a radical selected from the group consisting of a bond, divalent hydrocarbon having 1 to 10 carbons, hexafluorinated isopropylidene, carbonyl, thio, sulfinyl, sulfonyl and oxide, and R is a tetra-valent radical selected from the group consisting of aliphatic radical having 2 and more carbons, cyclo-aliphatic radical, monoaromatic radical, condensed polyaromatic radical, and non-condensed polyaromatic radical wherein aromatic radicals are mutually connected with a bond or a crosslinking function).
    Typical examples of polyimide and polyamic acid include where
    Y is thio radical and R is
    Y is a bond and R is III or IV, and Y is isopropylidene radical and R is IV.
    The polymers can be prepared from corresponding diamine and tetracarboxylic acid dianhydride.
    Polyimide or polyamic acid of this invention is excellent for high-temperature adhesive.

    摘要翻译： 公开了具有下式（I）的重复单元的聚酰亚胺及其具有下式（II）的重复单元的聚酰胺酸前体; （其中Y是选自由键，碳数1〜10的二价烃，六氟化异亚丙基，羰基，硫代，亚磺酰基，磺酰基和氧化物组成的组，R是选自 由具有2个或更多个碳的脂族基团，环脂族基团，单芳族基团，缩合多芳族基团和非稠合多芳族基团组成的组，其中芳族基团与键或交联官能团相互连接）。 聚酰亚胺和聚酰胺酸的典型实例包括其中Y是硫基，R是 Y是一个键，R是III或IV，Y是异丙叉基，R是IV。 聚合物可以由相应的二胺和四羧酸二酐制备。 本发明的聚酰亚胺或聚酰胺酸对于高温粘合剂是优异的。