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1.发明申请ELECTROCHEMICAL REDUCTION DEVICE AND METHOD FOR MANUFACTURING HYDRIDE OF AROMATIC COMPOUND 审中-公开电化学还原装置及其制备芳族化合物的方法公开(公告)号：US20160010224A1
公开(公告)日：2016-01-14
申请号：US14864225
申请日：2015-09-24
发明人： Yasushi SATO , Kota MIYOSHI , Kojiro NAKAGAWA , Yoshihiro KOBORI
CPC分类号： C25B3/04 , C25B1/10 , C25B9/08 , C25B15/08 , Y02E60/366
摘要： An electrochemical reduction device comprising: an electrode unit configured to include an electrolyte membrane, a reduction electrode that contains a reduction catalyst for hydrogenating at least one benzene ring of an aromatic compound, and an oxygen evolving electrode; a power control unit that applies a voltage Va between the reduction electrode and the oxygen evolving electrode; a concentration measurement unit that measures a concentration of an aromatic compound to be supplied to the reduction electrode; and a raw material supply amount adjustment unit that adjusts the amount of an organic liquid including an aromatic compound to be supplied to the reduction electrode per unit time based on the concentration measured by the concentration measurement unit.
摘要翻译： 一种电化学还原装置，包括：电极单元，被配置为包括电解质膜，还原电极，其包含用于氢化至少一个芳香族化合物的苯环的还原催化剂和放出氧的电极; 功率控制单元，其在所述还原电极和所述放氧电极之间施加电压Va; 浓度测定单元，测定供给到还原电极的芳香族化合物的浓度; 以及原料供给量调整单元，其基于由浓度测定单元测定的浓度，调整每单位时间内供给到还原电极的芳香族化合物的有机液的量。
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2.发明申请公开(公告)号：US20180002823A1
公开(公告)日：2018-01-04
申请号：US15704801
申请日：2017-09-14
发明人： Yasushi SATO , Kota MIYOSHI , Kojiro NAKAGAWA , Yoshihiro KOBORI
CPC分类号： C25B3/04 , C25B1/10 , C25B9/08 , C25B15/08 , Y02E60/366
摘要： An electrochemical reduction device comprising: an electrode unit configured to include an electrolyte membrane, a reduction electrode that contains a reduction catalyst for hydrogenating at least one benzene ring of an aromatic compound, and an oxygen evolving electrode; a power control unit that applies a voltage Va between the reduction electrode and the oxygen evolving electrode; a concentration measurement unit that measures a concentration of an aromatic compound to be supplied to the reduction electrode; and a raw material supply amount adjustment unit that adjusts the amount of an organic liquid including an aromatic compound to be supplied to the reduction electrode per unit time based on the concentration measured by the concentration measurement unit.
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3.发明申请公开(公告)号：US20150008138A1
公开(公告)日：2015-01-08
申请号：US14493396
申请日：2014-09-23
发明人： Yasushi SATO , Kota MIYOSHI , Kojiro NAKAGAWA , Yoshihiro KOBORI
摘要： An electrochemical reduction device is provided with an electrode unit, a power control unit, an organic material storage tank, a water storage tank, a gas-liquid separator, and a control unit. The electrode unit has an electrolyte membrane, a reduction electrode, and an oxygen evolving electrode. The electrolyte membrane is formed of an ionomer. A reduction catalyst used for the reduction electrode contains at least one of Pt and Pd. The oxygen evolving electrode contains catalysts of noble metal oxides such as RuO2, IrO2, and the like. The control unit controls the power control unit such that a relationship, VHER−20 mV≦VCA≦VTRR, can be satisfied when the potential at a reversible hydrogen electrode, the standard redox potential of an aromatic hydrocarbon compound or an N-containing heterocyclic aromatic compound, and the potential of the reduction electrode are expressed as VHER, VTRR, and VCA, respectively.
摘要翻译： 电化学还原装置设置有电极单元，功率控制单元，有机材料储罐，储水箱，气液分离器和控制单元。 电极单元具有电解质膜，还原电极和放氧电极。 电解质膜由离聚物形成。 用于还原电极的还原催化剂含有Pt和Pd中的至少一种。 放氧电极含有RuO 2，IrO 2等贵金属氧化物的催化剂。 控制单元控制功率控制单元，使得当可逆氢电极处的电位，芳香族烃化合物的标准氧化还原电位或含N杂环芳族化合物时，可以满足VHER-20mV和nLE; VCA＆NlE; VTRR的关系 化合物，还原电极的电位分别表示为VHER，VTRR和VCA。
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4.发明申请ELECTROCHEMICAL REDUCTION DEVICE AND METHOD FOR MANUFACTURING HYDRIDE OF AROMATIC COMPOUND 审中-公开电化学还原装置及其制备芳族化合物的方法公开(公告)号：US20160145751A1
公开(公告)日：2016-05-26
申请号：US15008870
申请日：2016-01-28
发明人： Yasushi SATO , Kota MIYOSHI , Kojiro NAKAGAWA , Yoshihiro KOBORI , Shinji OSHIMA
摘要： An electrochemical reduction device includes an electrode unit, a power control unit, a concentration measurement unit, and a control unit. The electrode unit includes an electrolyte membrane, a reduction electrode, and an oxygen evolving electrode. The control unit controls the power control unit such that a current value I flowing through the reduction electrode and the oxygen evolving electrode satisfies Equation, I≦Imax (C). In Equation, a maximum current value Imax (C) is defined according to a concentration C of an aromatic compound obtained by the concentration measurement unit such that Faraday efficiency is to be a predetermined value or more.
摘要翻译： 电化学还原装置包括电极单元，功率控制单元，浓度测量单元和控制单元。 电极单元包括电解质膜，还原电极和放氧电极。 控制单元控制功率控制单元，使得流过还原电极和放氧电极的电流值I满足公式I＆nlE; Imax（C）。 在等式中，最大电流值Imax（C）根据由浓度测量单元获得的芳族化合物的浓度C来定义，使得法拉第效率为预定值或更大。
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5.发明申请ELECTROCHEMICAL REDUCTION DEVICE AND METHOD OF MANUFACTURING HYDRIDE OF AROMATIC HYDROCARBON COMPOUND OR NITROGEN-CONTAINING HETEROCYCLIC AROMATIC COMPOUND 审中-公开电化学还原装置及制备芳香烃化合物或含氮杂环芳族化合物的液体的方法公开(公告)号：US20150114842A1
公开(公告)日：2015-04-30
申请号：US14588645
申请日：2015-01-02
发明人： Yasushi SATO , Kota MIYOSHI , Kojiro NAKAGAWA , Yoshihiro KOBORI
CPC分类号： C25B3/04 , C25B1/04 , C25B9/08 , Y02E60/366
摘要： An electrochemical reduction device is provided with an electrolyte membrane, an electrode unit, a power control unit, hydrogen gas generation amount measuring unit, and a control unit. The electrolyte membrane has ion conductivity. The electrode unit includes both a reduction electrode that is provided on one side of the electrolyte membrane and contains a reduction catalyst for hydrogenating at least one benzene ring of an aromatic hydrocarbon compound or a nitrogen-containing heterocyclic aromatic compound, and an oxygen evolving electrode. The control unit releases, when the hydrogen gas generation amount F1 is larger than an acceptable upper limit F0 of a hydrogen gas generation amount in the electrode unit, the application of a voltage by the power control unit.
摘要翻译： 电化学还原装置设置有电解质膜，电极单元，功率控制单元，氢气产生量测量单元和控制单元。 电解质膜具有离子传导性。 电极单元包括还原电极，其设置在电解质膜的一侧，并且含有用于氢化至少一个芳香族烃化合物或含氮杂环芳香族化合物的苯环的还原催化剂和放出氧的电极。 当氢气产生量F1大于电极单元中的氢气产生量的可接受上限F0时，控制单元释放电力控制单元施加的电压。
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公开(公告)号：US20150056526A1
公开(公告)日：2015-02-26
申请号：US14493428
申请日：2014-09-23
发明人： Yasushi SATO , Kota MIYOSHI , Kojiro NAKAGAWA , Yoshihiro KOBORI
CPC分类号： H01M8/0618 , C01B3/22 , C01B3/26 , C01B2203/0277 , C01B2203/04 , C01B2203/0405 , C01B2203/066 , C01B2203/1252 , H01M8/04014 , H01M8/04022 , H01M8/0625 , H01M8/0631 , H01M8/243 , H01M2008/1293
摘要： A fuel cell module of an aspect of the present invention includes: a fuel cell; a dehydrogenation reaction part that performs a dehydrogenation reaction of a hydride of an aromatic compound; a hydrogen separator that separates the hydrogen produced in the dehydrogenation reaction part from a dehydrogenated product of the hydride; a hydrogen supplier that supplies the hydrogen separated in the hydrogen separator to the fuel cell; and a single housing that houses the fuel cell, the dehydrogenation reaction part, the hydrogen separator, and the hydrogen supplier. The dehydrogenation reaction part is heated by at least one of the heat generated in the fuel cell and that generated by combustion of offgas from the fuel cell.
摘要翻译： 本发明的燃料电池组件包括：燃料电池; 脱氢反应部，其进行芳香族化合物的氢化物的脱氢反应; 氢分离器，其将在脱氢反应部分中产生的氢气与氢化物的脱氢产物分离; 氢供应器，其将在氢气分离器中分离的氢气供应到燃料电池; 和容纳燃料电池，脱氢反应部分，氢分离器和氢供应器的单个壳体。 脱氢反应部分被燃料电池中产生的热量中的至少一种和从燃料电池燃烧废气产生的热量加热。
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