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公开(公告)号：US07700518B2
公开(公告)日：2010-04-20
申请号：US11231708
申请日：2005-09-20
IPC分类号： B01J23/00 , B01J21/04 , B01J20/00 , B01J27/24 , B01J21/18 , B01J8/02 , B01J8/04 , B01J19/00 , B01J35/02 , B01D50/00 , B01D53/34
CPC分类号： B01J23/8913 , B01J8/0285 , B01J12/007 , B01J19/248 , B01J23/462 , B01J23/75 , B01J35/0006 , B01J35/002 , B01J35/04 , B01J35/10 , B01J35/1009 , B01J37/0221 , B01J37/0238 , B01J37/0244 , B01J2219/32293 , B01J2219/32296 , B01J2219/32408 , B01J2219/32466 , B01J2219/32475 , C07C1/041 , C07C1/0425 , C07C1/0455 , C07C2523/46 , C07C2523/745 , C07C2523/75 , C10G2/33 , C10G2/332
摘要： The present invention includes Fischer-Tropsch catalysts, reactions using Fischer-Tropsch catalysts, methods of making Fischer-Tropsch catalysts, processes of hydrogenating carbon monoxide, and fuels made using these processes. The invention provides the ability to hydrogenate carbon monoxide with low contact times, good conversion rates and low methane selectivities. In a preferred method, the catalyst is made using a metal foam support.
摘要翻译： 本发明包括费 - 托催化剂，使用费 - 托催化剂的反应，制备费 - 托催化剂的方法，氢化一氧化碳的方法和使用这些方法制备的燃料。 本发明提供了以低接触时间，良好的转化率和低的甲烷选择性氢化一氧化碳的能力。 在优选的方法中，催化剂是使用金属泡沫载体制成的。
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公开(公告)号：US07045486B2
公开(公告)日：2006-05-16
申请号：US10666430
申请日：2003-09-19
CPC分类号： C10G2/332 , B01J8/0285 , B01J12/007 , B01J19/0093 , B01J19/248 , B01J19/249 , B01J19/2495 , B01J23/8913 , B01J35/0006 , B01J35/04 , B01J35/10 , B01J35/1076 , B01J37/0217 , B01J37/0225 , B01J37/0238 , B01J37/0244 , B01J37/0248 , B01J2219/00783 , B01J2219/00822 , B01J2219/00835 , B01J2219/00844 , B01J2219/0086 , B01J2219/00873 , B01J2219/00984 , B01J2219/2453 , B01J2219/2458 , B01J2219/2462 , B01J2219/32244 , B01J2219/32293 , B01J2219/32296 , B01J2219/32408 , B01J2219/32466 , B01J2219/32475 , C07C1/041 , C07C1/0425 , C07C1/0455 , C07C2523/46 , C07C2523/745 , C07C2523/75 , C10G2/32 , C10G2/33 , C10G2/34 , C10G2/341
摘要： The present invention includes a catalyst structure and method of making the catalyst structure for Fischer-Tropsch synthesis that both rely upon the catalyst structure having a first porous structure with a first pore surface area and a first pore size of at least about 0.1 μm, preferably from about 10 μm to about 300 μm. A porous interfacial layer with a second pore surface area and a second pore size less than the first pore size is placed upon the first pore surface area. Finally, a Fischer-Tropsch catalyst selected from the group consisting of cobalt, ruthenium, iron and combinations thereof is placed upon the second pore surface area. Further improvement is achieved by using a microchannel reactor wherein the reaction chamber walls define a microchannel with the catalyst structure is placed therein through which pass reactants. The walls may separate the reaction chamber from at least one cooling chamber. The present invention also includes a method of Fischer-Tropsch synthesis.
摘要翻译： 本发明包括一种制备费 - 托合成催化剂结构的催化剂结构和方法，它们都依赖于具有第一孔表面积和至少约0.1μm的第一孔径的第一多孔结构的催化剂结构，优选 从约10毫米到约300毫米。 具有第二孔表面积和小于第一孔径的第二孔径的多孔界面层被放置在第一孔表面积上。 最后，将选自钴，钌，铁及其组合的费 - 托催化剂置于第二孔表面积上。 通过使用微通道反应器来实现进一步的改进，其中反应室壁限定了具有催化剂结构的微通道，通过反应物通过该通道。 壁可以将反应室与至少一个冷却室分开。 本发明还包括费 - 托合成方法。
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公开(公告)号：US06982287B2
公开(公告)日：2006-01-03
申请号：US10392479
申请日：2003-03-18
IPC分类号： C07C27/00
CPC分类号： B01J23/8913 , B01J8/0285 , B01J12/007 , B01J19/248 , B01J23/462 , B01J23/75 , B01J35/0006 , B01J35/002 , B01J35/04 , B01J35/10 , B01J35/1009 , B01J37/0221 , B01J37/0238 , B01J37/0244 , B01J2219/32293 , B01J2219/32296 , B01J2219/32408 , B01J2219/32466 , B01J2219/32475 , C07C1/041 , C07C1/0425 , C07C1/0455 , C07C2523/46 , C07C2523/745 , C07C2523/75 , C10G2/33 , C10G2/332
摘要： The present invention includes Fischer-Tropsch catalysts, reactions using Fischer-Tropsch catalysts, methods of making Fischer-Tropsch catalysts, processes of hydrogenating carbon monoxide, and fuels made using these processes. The invention provides the ability to hydrogenate carbon monoxide with low contact times, good conversion rates and low methane selectivities. In a preferred method, the catalyst is made using a metal foam support.
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公开(公告)号：US06750258B2
公开(公告)日：2004-06-15
申请号：US10282554
申请日：2002-10-28
IPC分类号： C07C2700
CPC分类号： C10G2/332 , B01J8/0285 , B01J12/007 , B01J19/248 , B01J23/8913 , B01J35/0006 , B01J35/10 , B01J37/0244 , B01J2219/32293 , B01J2219/32296 , B01J2219/32408 , B01J2219/32466 , B01J2219/32475 , C07C1/041 , C07C1/0425 , C07C1/0455 , C07C2523/46 , C07C2523/745 , C07C2523/75
摘要： The present invention includes Fischer-Tropsch catalysts, reactions using Fischer-Tropsch catalysts, methods of making Fischer-Tropsch catalysts, processes of hydrogenating carbon monoxide, and fuels made using these processes. The invention provides the ability to hydrogenate carbon monoxide with low contact times, good conversion rates and low methane selectivities. In a preferred method, the catalyst is made using a metal foam support.
摘要翻译： 本发明包括费 - 托催化剂，使用费 - 托催化剂的反应，制备费 - 托催化剂的方法，氢化一氧化碳的方法和使用这些方法制备的燃料。 本发明提供了以低接触时间，良好的转化率和低的甲烷选择性氢化一氧化碳的能力。 在优选的方法中，催化剂是使用金属泡沫载体制成的。
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公开(公告)号：US06660237B2
公开(公告)日：2003-12-09
申请号：US10038228
申请日：2002-01-03
IPC分类号： B01J3504
CPC分类号： C10G2/332 , B01J8/0285 , B01J12/007 , B01J19/0093 , B01J19/248 , B01J19/249 , B01J19/2495 , B01J23/8913 , B01J35/0006 , B01J35/04 , B01J35/10 , B01J35/1076 , B01J37/0217 , B01J37/0225 , B01J37/0238 , B01J37/0244 , B01J37/0248 , B01J2219/00783 , B01J2219/00822 , B01J2219/00835 , B01J2219/00844 , B01J2219/0086 , B01J2219/00873 , B01J2219/00984 , B01J2219/2453 , B01J2219/2458 , B01J2219/2462 , B01J2219/32244 , B01J2219/32293 , B01J2219/32296 , B01J2219/32408 , B01J2219/32466 , B01J2219/32475 , C07C1/041 , C07C1/0425 , C07C1/0455 , C07C2523/46 , C07C2523/745 , C07C2523/75 , C10G2/32 , C10G2/33 , C10G2/34 , C10G2/341
摘要： The present invention includes a catalyst structure and method of making the catalyst structure for Fischer-Tropsch synthesis that both rely upon the catalyst structure having a first porous structure with a first pore surface area and a first pore size of at least about 0.1 &mgr;m, preferably from about 10 &mgr;m to about 300 &mgr;m. A porous interfacial layer with a second pore surface area and a second pore size less than the first pore size is placed upon the first pore surface area. Finally, a Fischer-Tropsch catalyst selected from the group consisting of cobalt, ruthenium, iron and combinations thereof is placed upon the second pore surface area. Further improvement is achieved by using a microchannel reactor wherein the reaction chamber walls define a microchannel with the catalyst structure placed therein through which pass reactants. The walls may separate the reaction chamber from at least one cooling chamber. The present invention also includes a method of Fischer-Tropsch synthesis.
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公开(公告)号：US06558634B1
公开(公告)日：2003-05-06
申请号：US09492254
申请日：2000-01-27
IPC分类号： B01J3504
CPC分类号： C10G2/332 , B01J8/0285 , B01J12/007 , B01J19/0093 , B01J19/248 , B01J19/249 , B01J19/2495 , B01J23/8913 , B01J35/0006 , B01J35/04 , B01J35/10 , B01J35/1076 , B01J37/0217 , B01J37/0225 , B01J37/0238 , B01J37/0244 , B01J37/0248 , B01J2219/00783 , B01J2219/00822 , B01J2219/00835 , B01J2219/00844 , B01J2219/0086 , B01J2219/00873 , B01J2219/00984 , B01J2219/2453 , B01J2219/2458 , B01J2219/2462 , B01J2219/32244 , B01J2219/32293 , B01J2219/32296 , B01J2219/32408 , B01J2219/32466 , B01J2219/32475 , C07C1/041 , C07C1/0425 , C07C1/0455 , C07C2523/46 , C07C2523/745 , C07C2523/75 , C10G2/32 , C10G2/33 , C10G2/34 , C10G2/341
摘要： The present invention includes Fischer-Tropsch catalysts, reactions using Fischer-Tropsch catalysts, methods of making Fischer-Tropsch catalysts, processes of hydrogenating carbon monoxide, and fuels made using these processes. The invention provides the ability to hydrogenate carbon monoxide with low contact times, good conversion rates and low methane selectivities. In a preferred method, the catalyst is made using a metal foam support.
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公开(公告)号：US06451864B1
公开(公告)日：2002-09-17
申请号：US09375610
申请日：1999-08-17
IPC分类号： C07C2700
CPC分类号： C10G2/332 , B01J8/0285 , B01J12/007 , B01J19/0093 , B01J19/248 , B01J19/249 , B01J19/2495 , B01J23/8913 , B01J35/0006 , B01J35/04 , B01J35/10 , B01J35/1076 , B01J37/0217 , B01J37/0225 , B01J37/0238 , B01J37/0244 , B01J37/0248 , B01J2219/00783 , B01J2219/00822 , B01J2219/00835 , B01J2219/00844 , B01J2219/0086 , B01J2219/00873 , B01J2219/00984 , B01J2219/2453 , B01J2219/2458 , B01J2219/2462 , B01J2219/32244 , B01J2219/32293 , B01J2219/32296 , B01J2219/32408 , B01J2219/32466 , B01J2219/32475 , C07C1/041 , C07C1/0425 , C07C1/0455 , C07C2523/46 , C07C2523/745 , C07C2523/75 , C10G2/32 , C10G2/33 , C10G2/34 , C10G2/341
摘要： The present invention includes a catalyst structure and method of making the catalyst structure for Fischer-Tropsch synthesis that both rely upon the catalyst structure having a first porous structure with a first pore surface area and a first pore size of at least about 0.1 &mgr;m, preferably from about 10 &mgr;m to about 300 &mgr;m. A porous interfacial layer with a second pore surface area and a second pore size less than the first pore size is placed upon the first pore surface area. Finally, a Fischer-Tropsch catalyst selected from the group consisting of cobalt, ruthenium, iron and combinations thereof is placed upon the second pore surface area. Further improvement is achieved by using a microchannel reactor wherein the reaction chamber walls define a microchannel with the catalyst structure placed therein through which pass reactants. The walls may separate the reaction chamber from at least one cooling chamber. The present invention also includes a method of Fischer-Tropsch synthesis.
摘要翻译： 本发明包括一种制备费 - 托合成催化剂结构的催化剂结构和方法，它们均依赖于具有第一孔表面积和至少约0.1μm的第一孔径的第一多孔结构的催化剂结构，优选 从约10毫米到约300毫米。 具有第二孔表面积和小于第一孔径的第二孔径的多孔界面层被放置在第一孔表面积上。 最后，将选自钴，钌，铁及其组合的费 - 托催化剂置于第二孔表面积上。 通过使用微通道反应器来实现进一步的改进，其中反应室壁限定了具有催化剂结构置于其中的微通道，通过反应物。 壁可以将反应室与至少一个冷却室分开。 本发明还包括费 - 托合成方法。
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公开(公告)号：US20100292074A1
公开(公告)日：2010-11-18
申请号：US12758795
申请日：2010-04-12
CPC分类号： B01J23/8913 , B01J8/0285 , B01J12/007 , B01J19/248 , B01J23/462 , B01J23/75 , B01J35/0006 , B01J35/002 , B01J35/04 , B01J35/10 , B01J35/1009 , B01J37/0221 , B01J37/0238 , B01J37/0244 , B01J2219/32293 , B01J2219/32296 , B01J2219/32408 , B01J2219/32466 , B01J2219/32475 , C07C1/041 , C07C1/0425 , C07C1/0455 , C07C2523/46 , C07C2523/745 , C07C2523/75 , C10G2/33 , C10G2/332
摘要： The present invention includes Fischer-Tropsch catalysts, reactions using Fischer-Tropsch catalysts, methods of making Fischer-Tropsch catalysts, processes of hydrogenating carbon monoxide, and fuels made using these processes. The invention provides the ability to hydrogenate carbon monoxide with low contact times, good conversion rates and low methane selectivities. In a preferred method, the catalyst is made using a metal foam support.
摘要翻译： 本发明包括费 - 托催化剂，使用费 - 托催化剂的反应，制备费 - 托催化剂的方法，氢化一氧化碳的方法和使用这些方法制备的燃料。 本发明提供了以低接触时间，良好的转化率和低的甲烷选择性氢化一氧化碳的能力。 在优选的方法中，催化剂是使用金属泡沫载体制成的。
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公开(公告)号：US07585899B2
公开(公告)日：2009-09-08
申请号：US11364595
申请日：2006-02-27
IPC分类号： C07C27/00
CPC分类号： C10G2/332 , B01J8/0285 , B01J12/007 , B01J19/0093 , B01J19/248 , B01J19/249 , B01J19/2495 , B01J23/8913 , B01J35/0006 , B01J35/04 , B01J35/10 , B01J35/1076 , B01J37/0217 , B01J37/0225 , B01J37/0238 , B01J37/0244 , B01J37/0248 , B01J2219/00783 , B01J2219/00822 , B01J2219/00835 , B01J2219/00844 , B01J2219/0086 , B01J2219/00873 , B01J2219/00984 , B01J2219/2453 , B01J2219/2458 , B01J2219/2462 , B01J2219/32244 , B01J2219/32293 , B01J2219/32296 , B01J2219/32408 , B01J2219/32466 , B01J2219/32475 , C07C1/041 , C07C1/0425 , C07C1/0455 , C07C2523/46 , C07C2523/745 , C07C2523/75 , C10G2/32 , C10G2/33 , C10G2/34 , C10G2/341
摘要： The present invention includes a catalyst structure and method of making the catalyst structure for Fischer-Tropsch synthesis that both rely upon the catalyst structure having a first porous structure with a first pore surface area and a first pore size of at least about 0.1 μm, preferably from about 10 μm to about 300 μm. A porous interfacial layer with a second pore surface area and a second pore size less than the first pore size is placed upon the first pore surface area. Finally, a Fischer-Tropsch catalyst selected from the group consisting of cobalt, ruthenium, iron and combinations thereof is placed upon the second pore surface area. Further improvement is achieved by using a microchannel reactor wherein the reaction chamber walls define a microchannel with the catalyst structure placed therein through which pass reactants. The walls may separate the reaction chamber from at least one cooling chamber. The present invention also includes a method of Fischer-Tropsch synthesis.
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公开(公告)号：US06491880B1
公开(公告)日：2002-12-10
申请号：US09492245
申请日：2000-01-27
IPC分类号： B01J800
CPC分类号： C10G2/332 , B01J8/0285 , B01J12/007 , B01J19/0093 , B01J19/248 , B01J19/249 , B01J19/2495 , B01J23/8913 , B01J35/0006 , B01J35/04 , B01J35/10 , B01J35/1076 , B01J37/0217 , B01J37/0225 , B01J37/0238 , B01J37/0244 , B01J37/0248 , B01J2219/00783 , B01J2219/00822 , B01J2219/00835 , B01J2219/00844 , B01J2219/0086 , B01J2219/00873 , B01J2219/00984 , B01J2219/2453 , B01J2219/2458 , B01J2219/2462 , B01J2219/32244 , B01J2219/32293 , B01J2219/32296 , B01J2219/32408 , B01J2219/32466 , B01J2219/32475 , C07C1/041 , C07C1/0425 , C07C1/0455 , C07C2523/46 , C07C2523/745 , C07C2523/75 , C10G2/32 , C10G2/33 , C10G2/34 , C10G2/341
摘要： The present invention includes Fischer-Tropsch catalysts, reactions using Fischer-Tropsch catalysts, methods of making Fischer-Tropsch catalysts, processes of hydrogenating carbon monoxide, and fuels made using these processes. The invention provides the ability to hydrogenate carbon monoxide with low contact times, good conversion rates and low methane selectivities. In a preferred method, the catalyst is made using a metal foam support.
摘要翻译： 本发明包括费 - 托催化剂，使用费 - 托催化剂的反应，制备费 - 托催化剂的方法，氢化一氧化碳的方法和使用这些方法制备的燃料。 本发明提供了以低接触时间，良好的转化率和低的甲烷选择性氢化一氧化碳的能力。 在优选的方法中，催化剂是使用金属泡沫载体制成的。
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