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公开(公告)号：WO2022081654A1
公开(公告)日：2022-04-21
申请号：PCT/US2021/054703
申请日：2021-10-13
申请人： PHILLIPS 66 COMPANY
摘要： A process comprising a heterogeneous reaction between a solid oxyanion-modified metal organic framework and a hydrocarbon feed to form a modified hydrocarbon stream. The modified hydrocarbon stream comprises essentially of C6+ hydrocarbons.
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公开(公告)号：WO2022081639A1
公开(公告)日：2022-04-21
申请号：PCT/US2021/054684
申请日：2021-10-13
申请人： PHILLIPS 66 COMPANY
摘要： A process comprising a heterogenous reaction between a solid metal organic framework supported heteropolyacid catalyst and a hydrocarbon feed to form a modified hydrocarbon stream. The modified hydrocarbon stream comprises essentially of C6+ hydrocarbons.
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公开(公告)号：WO2022081660A1
公开(公告)日：2022-04-21
申请号：PCT/US2021/054712
申请日：2021-10-13
申请人： PHILLIPS 66 COMPANY
摘要： A solid metal organic framework composition comprising a solid oxyanion-modified metal organic framework wherein the oxyanion loading is at least 2 per node.
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公开(公告)号：WO2020076651A1
公开(公告)日：2020-04-16
申请号：PCT/US2019/054832
申请日：2019-10-04
申请人： PHILLIPS 66 COMPANY
发明人： BALDRIDGE, Anthony O. , McDANIEL, Neal D. , SUTTIL, James A. , WEINTROB, Edward C. , YAO, Jianhua , NEWMAN, Bruce B. , SARDASHTI, Maziar , WALSTON, Robert M. , LUSK, Steven E.
摘要： The present disclosure relates to processes and systems that catalytically convert a hydrocarbon feed stream that predominantly comprises both isopentane and n-pentane to yield upgraded hydrocarbon products that are suitable for use as a blend component of liquid transportation fuels or as an intermediate in the production of other value-added chemicals. The hydrocarbon feed stream is isomerized in a first reaction zone to convert at least a portion of the n-pentane to isopentane, followed by catalytic-activation of the isomerization effluent in a second reaction zone with an activation catalyst to produce an activation effluent. The process increases the conversion of the hydrocarbon feed stream to olefins and aromatics, while minimizing the production of C1-C4 light paraffins. Certain embodiments provide for further upgrading of at least a portion of the activation effluent by either oligomerization or alkylation.
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公开(公告)号：WO2022226063A1
公开(公告)日：2022-10-27
申请号：PCT/US2022/025541
申请日：2022-04-20
申请人： PHILLIPS 66 COMPANY
发明人： LIU, Ying , BAXTER, Samuel J. , YAO, Jianhua
IPC分类号： C25B3/26 , C10L3/10 , C25B3/20 , C25B11/075 , C25B11/081 , C25B13/07 , C25B3/03
摘要： A process for methanation comprising a first region for flowing a stream over a solid oxide electrolysis cell. In this first region the stream consists of CO2, H2, and H2O, the stream is converted into a first conversion stream, and the solid oxide electrolysis cell is enhanced with a methanation catalyst. The process also has a removal region connected to the first region wherein the removal region is able to flow the first conversion stream away from the solid oxide electrolysis cell.
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公开(公告)号：WO2022081651A1
公开(公告)日：2022-04-21
申请号：PCT/US2021/054700
申请日：2021-10-13
申请人： PHILLIPS 66 COMPANY
摘要： A solid metal organic framework composition comprising a solid metal organic framework supported sulfonic acid wherein the sulfur content is greater than 0.5 mmol/gram.
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公开(公告)号：WO2022081641A1
公开(公告)日：2022-04-21
申请号：PCT/US2021/054687
申请日：2021-10-13
申请人： PHILLIPS 66 COMPANY
摘要： A solid metal organic framework composition comprising a solid metal organic framework supported heteropolyacid wherein the heteropolyacid loading is greater than 25% by weight; and the pore volume is less than 2.0 mL/g; prepared by a method comprising: mixing a solution of metal organic framework precursors and a heteropolyacid to form a starting solution; and reacting the starting solution in a reactor to form a solid metal organic framework supported heteropolyacid.
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公开(公告)号：WO2013103515A1
公开(公告)日：2013-07-11
申请号：PCT/US2012/070315
申请日：2012-12-18
申请人： PHILLIPS 66 COMPANY , LIU, Shetian , YAO, Jianhua , XU, Xiaochun , BLOSSER, Patrick W. , ALLISON, Joe D. , SUGHRUE, Edward L. II
发明人： LIU, Shetian , YAO, Jianhua , XU, Xiaochun , BLOSSER, Patrick W. , ALLISON, Joe D. , SUGHRUE, Edward L. II
IPC分类号： C07C2/04
CPC分类号： C07C2/24 , C10G50/00 , C10G2300/1092 , C10G2400/02 , C10G2400/10
摘要： Methods and systems relate to upgrading light olefins, such as ethylene, propylene and butylenes, diluted in a gas mixture, such as refinery fuel gas. The upgrading yields products in a gasoline, distillate, lube oil or wax range without requiring purification or compression of the gas mixture prior to feeding the gas mixture to a reactor. In operation, the mixture contacts a solid oligimerization catalyst, such as silica supported chromium, within the reactor. This contact occurs at a first temperature suitable to produce oligomers that are formed of the olefins and adsorb on the catalyst in liquid or solid phases. Next, heating the catalyst to a second temperature higher the first temperature desorbs the oligomers that are recovered and separated into the products.
摘要翻译： 方法和系统涉及在诸如炼油厂燃料气体的气体混合物中稀释的轻质烯烃，例如乙烯，丙烯和丁烯。 升级产生汽油，馏出物，润滑油或蜡的产品，而不需要在将气体混合物送入反应器之前对气体混合物进行纯化或压缩。 在操作中，混合物在反应器内接触固体寡聚化催化剂，例如二氧化硅负载的铬。 该接触在适于产生由烯烃形成并以液相或固相吸附在催化剂上的低聚物的第一温度下进行。 接下来，将催化剂加热至高于第一温度的第二温度，第一温度将回收并分离成产物的低聚物解吸附。
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公开(公告)号：WO2022081647A1
公开(公告)日：2022-04-21
申请号：PCT/US2021/054694
申请日：2021-10-13
申请人： PHILLIPS 66 COMPANY
摘要： A process comprising a heterogeneous reaction between a solid metal organic framework supported sulfonic acid and a hydrocarbon feed to form a modified hydrocarbon stream. The modified hydrocarbon stream comprises essentially of C6+ hydrocarbons.
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公开(公告)号：WO2022076839A1
公开(公告)日：2022-04-14
申请号：PCT/US2021/054203
申请日：2021-10-08
申请人： PHILLIPS 66 COMPANY
发明人： YAO, Jianhua
摘要： Methods for modifying a ZSM-5 zeolite by contacting the zeolite with an alkaline solution prior to combining with a binder material to produce a modified ZSM-5 catalyst extrudate that has substantially longer catalyst life, relative to an untreated ZSM-5 catalyst, for converting light olefins to products that may be used as a liquid transportation fuel blend stock. The alkaline solution is optionally sodium hydroxide. The binder is optionally alumina, bentonite or silica.
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