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公开(公告)号：EP4082659A1
公开(公告)日：2022-11-02
申请号：EP20957237.9
申请日：2020-10-16
发明人： ZHANG, Tao , YE, Mao , ZHANG, Jinling , XU, Shuliang , TANG, Hailong , WANG, Xiangao , ZHANG, Cheng , JIA, Jinming , WANG, Jing , LI, Hua , LI, Chenggong , LIU, Zhongmin
摘要： The present application discloses a regeneration device, a device for preparing low-carbon olefins, and a use thereof. The regeneration device includes a first regenerator and a second regenerator; a first activation zone of the first regenerator is connected to the second regenerator through a pipeline, such that a catalyst in the first activation zone is able to be delivered to the second regenerator; and the second regenerator is connected to a gas-solid separation zone of the first regenerator through a pipeline, such that a catalyst in the second regenerator is able to be delivered to the gas-solid separation zone. The regeneration device can adjust the coke content, coke content distribution, and coke species in a dimethyl ether/methanol to olefins (DMTO) catalyst to control an operation window of the DMTO catalyst, which improves the selectivity for low-carbon olefins and the atomic economy of a methanol-to-olefins (MTO) technology.
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公开(公告)号：EP4023333A1
公开(公告)日：2022-07-06
申请号：EP20912191.2
申请日：2020-11-26
申请人： Dalian Institute Of Chemical Physics Chinese Academy of Sciences , Formosa Plastics Corporation
发明人： FAN, Sisi , XU, Jinming , HUANG, Yanqiang , DUAN, Hongmin , ZHANG, Tao , HUNG, Wan-tun , CHEN, Yu-Cheng , WU, Chien-Hui , CHENG, Ya-Wen , WEN, Ming-Hsien , CHANG, Chao-Chin , HUANG, Tsao-Cheng , YEH, Lu-Chen , CHENG, Ming-Hung
摘要： The present disclosure provides a regeneration method of a nitrogen-containing carbon catalyst, including the following steps: roasting the nitrogen-containing carbon catalyst in a nitrogen-containing atmosphere to obtain a regenerated nitrogen-containing carbon catalyst. The method is a universal method, which is suitable for nitrogen-doped carbon catalysts and can be used to regenerate a nitrogen-containing carbon catalyst for producing vinyl chloride (VC) through 1,2-dichloroethane cracking. The method can greatly reduce the production cost of the catalyst and increase the service life of the catalyst, and a regeneration process thereof is fast, simple, and controllable, and does not require high temperatures.
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3.发明公开
公开(公告)号：EP3918035A1
公开(公告)日：2021-12-08
申请号：EP19710128.0
申请日：2019-01-28
申请人： SABIC Global Technologies B.V. , Dalian Institute Of Chemical Physics, Chinese Academy Of Sciences
发明人： ZHAO, Yinfeng , YE, Mao , LIU, Zhongmin , TANG, Hailong , WANG, Jing , ZHANG, Jinling , ZHANG, Tao , AL-SHAMMARI, Talal Khaled
IPC分类号： C10G11/18
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公开(公告)号：EP3078651B1
公开(公告)日：2019-01-02
申请号：EP13898489.3
申请日：2013-12-03
发明人： LIU, Zhongmin , YE, Mao , ZHANG, Tao , HE, Changqing , WANG, Xiangao , ZHAO, Yinfeng
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5.发明授权A method for preparing ethylene glycol from polyhydroxy compound 有权一种用于从Polyhydroxidverbindung制备乙二醇的方法
公开(公告)号：EP2351725B1
公开(公告)日：2014-07-23
申请号：EP09828605.7
申请日：2009-11-05
发明人： ZHANG, Tao , ZHENG, Mingyuan , WANG, Aiqin , JI, Na , PANG, Jifeng , TAI, Zhijun , ZHOU, Likun , CHEN, Jingguang , WANG, Xiaodong
IPC分类号： C07C29/00 , C07C31/20 , B01J23/652 , B01J23/85 , B01J23/882 , B01J23/883 , B01J23/888 , B01J37/02 , B01J37/18 , B01J21/04 , B01J21/06 , B01J21/08 , B01J21/18 , B01J27/19 , B01J27/22 , B01J27/24
CPC分类号： B01J23/6525 , B01J21/04 , B01J21/06 , B01J21/063 , B01J21/08 , B01J21/18 , B01J23/652 , B01J23/6527 , B01J23/85 , B01J23/882 , B01J23/883 , B01J23/888 , B01J27/19 , B01J27/22 , B01J27/24 , B01J37/0205 , B01J37/18 , C07C29/00 , C07C29/132 , Y02P20/52 , C07C31/202 , C07C31/26
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6.发明公开A PROCESS FOR PREPARING ETHYLENE GLYCOL USING CELLULOSE 有权VERFAHREN ZUR HERSTELLUNG VON ETHYLINGLYKOL UNTER VERWENDUNG VON CELLULOSE
公开(公告)号：EP2338867A1
公开(公告)日：2011-06-29
申请号：EP08877495.5
申请日：2008-10-31
发明人： ZHANG, Tao , ZHENG, Mingyuan , JI, Na , WANG, Aiqin , SHU, Yuying , WANG, Hui , WANG, Xiaodong , CHEN, Jingguang
CPC分类号： C07C29/00 , B01J21/063 , B01J21/18 , B01J23/652 , B01J23/6527 , B01J23/85 , B01J23/888 , B01J27/19 , B01J27/22 , B01J27/25 , Y02P20/52 , C07C31/202
摘要： A method for preparing ethylene glycol from cellulose uses the cellulose as the feed for the reaction. The cellulose conversion is performed over catalysts which are composed of the metallic state, carbides, nitrides, or phosiphides of molybdenum or tungsten, and metallic cobalt, nickel, ruthenium, rhodium, palladium, iridium, and platinum of the group 8, 9, or 10 transition metals. The catalytic conversion of cellulose is conducted at 120 to 300°C and hydrogen pressure 1 to 12MPa under the hydrothermal conditions to achieve the high efficiency, high selectivity, and high yield of ethylene glycol. Compared to the existing method of preparing ethylene glycol from ethylene, the method, using the renewable raw material for the reaction, is friendly to the environment, and has high atom economy.
摘要翻译： 从纤维素制备乙二醇的方法使用纤维素作为反应的进料。 纤维素转化在由金属状态，碳化物，氮化物或钼或钨的高温以及金属钴，镍，钌，铑，钯，铱和铂组成的催化剂上进行，第8,9或9族 10个过渡金属。 在水热条件下，纤维素的催化转化率为120〜300℃，氢压为1〜12MPa，实现了乙二醇的高效，高选择性和高产率。 与从乙烯制备乙二醇的现有方法相比，使用可再生原料进行反应的方法对环境友好，原子经济性高。
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公开(公告)号：EP3967400A1
公开(公告)日：2022-03-16
申请号：EP19928705.3
申请日：2019-05-10
发明人： ZHANG, Jinling , YE, Mao , LIU, Zhongmin , ZHOU, Jibin , ZHANG, Tao , WANG, Xiangao , TANG, Hailong , WANG, Jing
摘要： Disclosed is a method for partially regenerating a catalyst for methanol and/or dimethyl ether-to-olefin. The method comprises: introducing a mixed gas into a regenerated region containing a catalyst to be regenerated, and subjecting same to a partial regeneration reaction to obtain a regenerated catalyst, wherein the mixed gas contains water vapor and air; and in the regenerated catalyst, the coke content of at least part of the regenerated catalyst is greater than 1%. The method utilizes the coupling of a mixed gas of water vapor and air to activate a deactivated catalyst, selectively eliminate part of a coke deposit in the catalyst to be regenerated, and obtain a partially regenerated catalyst for methanol-to-olefin. Another aspect of the present invention is that further provided is a method for methanol and/or dimethyl ether-to-olefin by using the partially regenerated catalyst for methanol-to-olefin regenerated by means of the method.
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公开(公告)号：EP2548858B2
公开(公告)日：2020-01-08
申请号：EP10847750.6
申请日：2010-11-04
发明人： ZHANG, Tao , TAI, Zhijun , WANG, Aiqin , ZHENG, Mingyuan
IPC分类号： C07C29/00 , C07C29/132 , C07C29/136 , C07C31/20 , B01J23/30 , B01J23/64
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公开(公告)号：EP3530641A1
公开(公告)日：2019-08-28
申请号：EP16919298.6
申请日：2016-10-19
发明人： ZHANG, Tao , YE, Mao , HE, Changqing , ZHANG, Jinling , WANG, Xiangao , TANG, Hailong , JIA, Jinming , ZHAO, Yinfeng , LIU, Zhongmin
摘要： The present invention refers to a method and device for preparing propylene and C4 hydrocarbons from oxygen-containing compounds. The main characteristics of the method lie in that: returning 70 wt.% or more of the light fractions in the generated product to a dense phase zone of a fast fluidized-bed reactor from a reactor feed distributor at the bottom-most of the fast fluidized-bed reactor to react ethylene and the oxygen-containing compounds to perform an alkylation reaction in presence of a catalyst to produce products of propylene and the like, and circulating 80 wt.% or more of the hydrocarbons with 5 or more carbons into a catalytic cracking lift pipe to perform a cracking reaction to generate a product containing propylene and C4 hydrocarbons, which is subsequently fed into a dilute phase zone of the fast fluidized-bed reactor. The method and device of the present invention improve the reaction rate of ethylene alkylation, and the unit volume production capacity of reactor is high.
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公开(公告)号：EP3078414B1
公开(公告)日：2018-09-19
申请号：EP13898849.8
申请日：2013-12-03
发明人： ZHANG, Tao , YE, Mao , LIU, Zhongmin
CPC分类号： B01J8/26 , B01J8/1827 , B01J8/1836 , B01J8/1872 , B01J8/34 , B01J2208/0015 , B01J2208/00902 , B01J2208/00938 , C07C1/20 , Y02P20/52 , Y02P30/42 , C07C11/04 , C07C11/06
摘要： This present invention relates to a reaction device for preparing light olefins from methanol and/or dimethyl ether, and more specifically relates to a reaction device for preparing light olefins from methanol and/or dimethyl ether, which mainly comprises a dense phase fluidized bed reactor (2), a cyclone separator (3), a stripper (5), a lift pipe (7), a dense phase fluidized bed regenerator (10), a cyclone separator (11), a stripper (13), and a lift pipe (15), wherein the dense phase fluidized bed reactor (2) is separated into n (n‰¥2) secondary reaction zones by a material flow controller (17), and the dense phase fluidized bed regenerator (10) is separated into m (m‰¥2) secondary regeneration zones by the material flow controller (17). The use of the reaction device of this present invention solves the problems in the prior art that the distribution of carbon deposition on a catalyst is non-uniform and the selectivity for the light olefins is relatively low.
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