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    β-amino-α-cyanoacrylates and their use as herbicides
    1.
    发明授权
    β-amino-α-cyanoacrylates and their use as herbicides 失效
    氨基-α-氰基丙烯酸酯及其作为除草剂的用途

    公开(公告)号：US07842832B2

    公开(公告)日：2010-11-30

    申请号：US10499568

    申请日：2002-12-17

    申请人： Albert C. Everson ,  Daniel J. Coughlin ,  Michael A. Guaciaro ,  Linda B. Fleming ,  Lester L. Maravetz ,  John L. Huppatz

    发明人： Albert C. Everson ,  Daniel J. Coughlin ,  Michael A. Guaciaro ,  Linda B. Fleming ,  Lester L. Maravetz ,  John L. Huppatz

    IPC分类号： C07C255/07 ,  A01N37/34

    CPC分类号： C07C255/23 ,  A01N37/42 ,  A01N37/44 ,  A01N43/08 ,  A01N43/16 ,  A01N43/18 ,  C07C255/30 ,  C07C255/31 ,  C07C323/60 ,  C07C2601/02 ,  C07C2601/08 ,  C07C2601/14 ,  C07D307/14 ,  C07D307/16 ,  C07D309/04 ,  C07D309/06

    摘要： β-Amino-α-Cyanoacrylates of formula I where the variables have the following meanings: R1 is n-alkyl, n-alkenyl or alkoxyalkyl; R2,R3 are alkyl, which may be partially or fully halogenated and/or may carry a substituent from the group consisting of cyano, alkoxy, haloalkoxy, alkylthio, haloalkylthio, C1-C6-alkylsulfinyl, haloalkylsulfinyl, alkylsulfonyl and haloalkylsulfonyl, are alkenyl or alkynyl; or R2 and R3 together with the carbon atom to which they are attached form a cycloalkyl ring in which one or two nonadjacent CH2 groups may be replaced by oxygen or sulfur, and where the cycloalkyl ring may be substituted by halogen or alkyl; R4 is hydrogen, halogen, cyano or alkyl, where the substituents R2, R3 and R4 or two of the radicals R2, R3 and R4 are not simultaneously methyl, and their agriculturally useful salts, processes and intermediates for their preparation; and the use of these compounds or of compositions comprising these compounds for controlling undesirable plants are described.

    摘要翻译： 式Ⅰ的氨基-α-氰基丙烯酸酯，其中变量具有以下含义：R 1是正烷基，正 - 链烯基或烷氧基烷基; R2，R3是烷基，其可以是部分或完全卤化的和/或可以从氰基，烷氧基，卤代烷氧基，烷硫基，卤代烷硫基，C 1 -C 6烷基亚磺酰基，卤代烷基亚磺酰基，烷基磺酰基和卤代烷基磺酰基中携带取代基，是烯基或 炔基; 或R 2和R 3与它们所连接的碳原子一起形成环烷基环，其中一个或两个不相邻的CH 2基团可被氧或硫取代，并且其中环烷基环可被卤素或烷基取代; R 4是氢，卤素，氰基或烷基，其中取代基R 2，R 3和R 4或基团R 2，R 3和R 4中的两个不同时为甲基，及其农业上有用的盐，其制备方法和中间体; 并描述了这些化合物或包含这些化合物的组合物用于防治不期望的植物的用途。

    Compounds and compositions
    2.
    发明授权
    Compounds and compositions 失效
    化合物和组合物

    公开(公告)号：US4134987A

    公开(公告)日：1979-01-16

    申请号：US756069

    申请日：1977-01-03

    申请人： John L. Huppatz

    发明人： John L. Huppatz

    IPC分类号： A01N43/56 ,  C07D231/14 ,  C07D231/16 ,  C07D231/20 ,  A01N9/22

    CPC分类号： C07D231/20 ,  A01N43/56 ,  C07D231/14 ,  C07D231/16

    摘要： Fungicidal compositions comprising as an active ingredient a compound of the general formula I ##STR1## wherein either R.sup.1 or R.sup.2 is the group ##STR2## in which X is an oxygen atom or a sulphur atom and R.sup.5 is straight chain alkyl group of 1 to 8 carbon atoms, branched chain alkyl group of 1 to 8 carbon atoms, cyclic alkyl group of 3 to 8 carbon atoms, alkenyl group, alkynyl group, hydroxyalkyl group phenyl group or a mono-, di- or tri- substituted phenyl group with substituents, which may be the same or different, chosen from the group consisting hydrogen alkyl, alkenyl, alkynyl, hydroxyalkyl, alkoxy, phenyl, halogen, trifluoromethyl, thiocyanate, nitro, cyano, amino, carboxy, alkoxycarbonyl, carbamoyl, N-alkylcarbamoyl and N,N-dialkylcarbamoyl; when R.sup.1 is the group ##STR3## then R.sup.3 is hydrogen, alkyl, alkenyl alkynyl, hydroxyalkyl, phenyl, CH.sub.2 CF.sub.3 or the group --CH.sub.2 COOR.sup.6 wherein R.sup.6 is alkyl, phenyl or substituted phenyl, and R.sup.2 and R.sup.4, which may be the same or different, are hydrogen, alkyl, alkenyl, alkynyl, hydroxalkyl, alkoxy, phenyl, halogen, trifluoromethyl, thiocyanate, nitro, cyano, amino, carboxy, alkoxycarbonyl, carbamoyl, N,alkylcarbamoyl, N,N-dialkylcarbamoyl, hydroxy or mercapto provided that R.sup.2 and R.sup.4 are not both hydrogen, hydroxy or mercapto; when R.sup.2 is the group ##STR4## then R.sup.3 is hydrogen, alkyl, alkenyl, alkynyl, hydroxyalkyl, phenyl or substituted phenyl, and R.sup.1 and R.sup.4, which may be the same or different, are hydrogen, alkyl, alkenyl, hydroxyalkyl, alkoxy, phenyl, substituted phenyl, halogen, trifluoromethyl, thiocyanate, nitro, cyano, amino, carboxy, alkoxycarbonyl, carbamoyl, N-alkylcarbamoyl, N,N-dialkylcarbamoyl, hydroxy or mercapto, provided that R.sup.1 and R.sup.3 are not both hydrogen and provided that R.sup.1 and R.sup.4 are not both hydroxy or mercapto; and an inert carrier material therefor.

    摘要翻译： 其中R 1和R 2中的一个是基团-CONHR 5，其中R 5是任选地被一个，两个或三个独立地选自烷基，烷氧基，卤素的取代基取代的苯基的基团的杀真菌的4-和5-吡唑酰甲酰胺 ，三氟甲基，硝基和氰基; R 3选自氢，烷基，羟基烷基，苯基和-CH 2 COOR 6，其中R 6是烷基; R 4和R 1或R 2，以不是-CONHR 5取代，独立地选自氢，卤素和烷基; 当R1为-CONHR5时，R2和R4不同时为氢; 当R 2为-CONHR 5时，R 1和R 3不同时为氢; 当R 1为-CONHR 5且R 5为苯基时，R 2，R 3和R 4各不为甲基。

    Fungicidal carboxamidopyrazoles
    4.
    发明授权
    Fungicidal carboxamidopyrazoles 失效
    杀菌甲酰胺吡唑

    公开(公告)号：US4214090A

    公开(公告)日：1980-07-22

    申请号：US951376

    申请日：1978-10-13

    申请人： John L. Huppatz

    发明人： John L. Huppatz

    IPC分类号： A01N43/56 ,  C07D231/14 ,  C07D231/16 ,  C07D231/20

    CPC分类号： A01N43/56 ,  C07D231/14 ,  C07D231/16 ,  C07D231/20

    摘要： Fungicidal 4- and 5-pyrazolecarboxamides of the formula ##STR1## wherein one of R.sup.1 and R.sup.2 is the group --CONHR.sup.5 in which R.sup.5 is phenyl optionally substituted with one, two or three substituents independently chosen from the group consisting of alkyl, alkoxy, halogen, trifluoromethyl, nitro and cyano; R.sup.3 is chosen from the group consisting of hydrogen, alkyl, hydroxyalkyl, phenyl and --CH.sub.2 COOR.sup.6 wherein R.sup.6 is alkyl; R.sup.4 and R.sup.1 or R.sup.2, whichever is not --CONHR.sup.5, are independently chosen from the group consisting of hydrogen, halogen, and alkyl; R.sup.2 and R.sup.4 are not both hydrogen when R.sup.1 is --CONHR.sup.5 ; R.sup.1 and R.sup.3 are not both hydrogen when R.sup.2 is --CONHR.sup.5 ; and R.sup.2, R.sup.3 and R.sup.4 are not each methyl when R.sup.1 is --CONHR.sup.5 and R.sup.5 is phenyl.

    摘要翻译： 其中R 1和R 2中的一个是基团-CONHR 5，其中R 5是任选地被一个，两个或三个独立地选自烷基，烷氧基，卤素的取代基取代的苯基的基团的杀真菌的4-和5-吡唑酰甲酰胺 ，三氟甲基，硝基和氰基; R 3选自氢，烷基，羟基烷基，苯基和-CH 2 COOR 6，其中R 6是烷基; R 4和R 1或R 2，以不是-CONHR 5取代，独立地选自氢，卤素和烷基; 当R1为-CONHR5时，R2和R4不同时为氢; 当R 2为-CONHR 5时，R 1和R 3不同时为氢; 当R 1为-CONHR 5且R 5为苯基时，R 2，R 3和R 4各不为甲基。

    Substituted anthranilates
    5.
    发明授权
    Substituted anthranilates 失效
    取代的邻氨基苯甲酸酯

    公开(公告)号：US4182877A

    公开(公告)日：1980-01-08

    申请号：US795595

    申请日：1977-05-10

    申请人： Roger L. N. Harris ,  John L. Huppatz ,  John N. Phillips ,  Barbara Witrzens

    发明人： Roger L. N. Harris ,  John L. Huppatz ,  John N. Phillips ,  Barbara Witrzens

    IPC分类号： A01N33/02 ,  A01N33/06 ,  A01N33/08 ,  A01N33/18 ,  A01N33/20 ,  A01N35/04 ,  A01N37/44 ,  A01N47/48 ,  C07C67/00 ,  C07C209/00 ,  C07C211/44 ,  C07C213/00 ,  C07C215/68 ,  C07C215/76 ,  C07C223/06 ,  C07C227/00 ,  C07C227/16 ,  C07C229/56 ,  C07C325/00 ,  C07C331/12 ,  C07D295/06 ,  A61K31/245

    CPC分类号： A01N47/48 ,  A01N33/06 ,  A01N33/08 ,  A01N33/18 ,  A01N35/04 ,  A01N37/44

    摘要： Anthranilic acid derivatives exhibiting fungicidal properties and useful as synthesis intermediates have the formula: ##STR1## wherein R is selected from the group consisting of a hydrogen atom; a --COOR.sup.3 group and a --CH.sub.2 OH group; R.sup.1 and R.sup.2 are the same or different and selected from the group consisting of a hydrogen atom and alkyl and cycloalkyl groups (provided that R.sup.1 and R.sup.2 are not both hydrogen atoms), or R.sup.1 and R.sup.2, together with the nitrogen atom to which they are attached, form a non-aromatic heterocyclic ring structure;R.sup.3 is selected from the group consisting of a hydrogen atom and an alkyl group;R.sup.4 is selected from the group consisting of a hydrogen atom, a halogen atom and a hydroxyl group;R.sup.6 is selected from the group consisting of a hydrogen atom and a halogen atom; andR.sup.5 is selected from the group consisting of a hydrogen atom, a halogen atom, and nitro, thiocyano and formyl groups.A process for production of these compounds by self-condensation of a substituted aminocrotonate by phosphorous oxychloride is also disclosed.

    摘要翻译： 显示杀真菌性的邻氨基苯甲酸衍生物可用作合成中间体具有下式：其中R选自氢原子; -COOR 3基团和-CH 2 OH基团; R1和R2相同或不同，选自氢原子和烷基和环烷基（条件是R1和R2不同时为氢原子），或R1和R2与它们所在的氮原子一起 附着，形成非芳族杂环结构; R3选自氢原子和烷基; R4选自氢原子，卤素原子和羟基; R 6选自氢原子和卤素原子; 并且R 5选自氢原子，卤素原子和硝基，硫氰基和甲酰基。 还公开了通过取代的氨基巴豆酸盐通过三氯氧化磷自缩合来生产这些化合物的方法。