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1.发明申请公开(公告)号：US20100326528A1
公开(公告)日：2010-12-30
申请号：US12872435
申请日：2010-08-31
申请人： Ashraful Islam , Liyuan Han , Atsushi Fukui
发明人： Ashraful Islam , Liyuan Han , Atsushi Fukui
CPC分类号： H01L51/0086 , C07F15/0053 , H01G9/2031 , H01G9/2059 , H01L51/0083 , H01L51/0088 , Y02E10/542 , Y02E10/549
摘要： A photosensitizing transition metal complex of the formula (Ia) MLY1, (Ib) MLX3 (Ic) MLY2X, (Id) MLY3X or (Ie) MLY4X in which M is a transition metal selected from ruthenium, osmium, iron, rhenium and technetium, preferably ruthenium or osmium. X is a co-ligand independently selected from NCS—, Cl—, Br—, I—, CN—, H2O; pyridine unsubstituted or substituted by at least one group selected from vinyl, primary, secondary or tertiary amine, OH and C1-30 alkyl, preferably NSC and CN—; L is a tridentate polypyridine ligand, carrying at least one carboxylic, phosphoric acid or a chelating group and one substituted or unsubstituted alkyl group having 1 to 50 carbon atoms, substituted or unsubstituted alkylamide group having 2 to 30 carbon atoms or substituted or unsubstituted aralkyl group having 7 to 50 carbon atoms. A dye-sensitized electrode includes a substrate having an electrically conductive surface, an oxide semiconductor film formed on the conductive surface, and the above sensitizer of formula (Ia), (Ib), (Ic), (Id) or (Ie) as specified above; supported on the film. A solar cell includes the above electrode, a counter electrode, and an electrolyte deposited there between.
摘要翻译： 式（Ia）MLY1，（Ib）MLX3（Ic）MLY2X，（Id）MLY3X或（Ie）MLY4X的光敏过渡金属络合物，其中M是选自钌，锇，铁，铼和锝的过渡金属， 优选钌或锇。 X是独立地选自NCS-，Cl-，Br-，I-，CN-，H 2 O的共配体; 未取代的或被至少一个选自乙烯基，伯，仲或叔胺，OH和C 1-3烷基，优选NSC和CN-的基团取代的吡啶; L是携带至少一种羧酸，磷酸或螯合基团的三齿多吡啶配体，和一个取代或未取代的碳原子数为1〜50的烷基，取代或未取代的碳原子数为2〜30的烷基酰胺基或取代或未取代的芳烷基 具有7至50个碳原子。 染料敏化电极包括具有导电表面的基底，在导电表面上形成的氧化物半导体膜，以及上述式（Ia），（Ib），（Ic），（Id）或（Ie）的敏化剂作为 以上指定; 支持电影。 太阳能电池包括上述电极，对电极和沉积在其间的电解质。
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2.发明申请Photosensitizing transition metal complex containing quaterpyridine and photovoltaic cell with the metal complex 审中-公开含有金属络合物的四联吡啶和光伏电池的光敏化过渡金属络合物公开(公告)号：US20050139257A1
公开(公告)日：2005-06-30
申请号：US11017649
申请日：2004-12-22
申请人： Ashraful Islam , Liyuan Han , Atsushi Fukui
发明人： Ashraful Islam , Liyuan Han , Atsushi Fukui
IPC分类号： C07D213/79 , C07F13/00 , C07F15/00 , C07F15/02 , H01G9/20 , H01L31/00 , H01L31/04 , H01M14/00
CPC分类号： C07F15/0053 , C09B57/10 , H01G9/2031 , H01G9/2059 , H01L51/0086 , Y02E10/542 , Y02E10/549
摘要： A photosensitizer complex of formula (I) MLX2 in which M is a transition metal selected from ruthenium, osmium, iron, rhenium and technetium; each X is a co-ligand independently selected from NCS−, Cl−, Br−, I−, CN−, H2O; pyridine unsubstituted or substituted by at least one group selected from vinyl, primary, secondary or tertiary amine, OH and C1-30 alky, preferably NSC− and CN−. L is a tetradentate polypyridine ligand, carrying at least one carboxylic, phosphoric acid or a chelating group and one substituted or unsubstituted alkyl group having 1 to 50 carbon atoms, substituted or unsubstituted alkylamide group having 2 to 30 carbon atoms or substituted or unsubstituted aralkyl group having 7 to 50 carbon atoms. A dye-sensitized electrode includes a substrate having an electrically conductive surface, an oxide semiconductor film formed thereon, and the above sensitizer of formula (I) as specified above, supported on the film.
摘要翻译： 式（I）MLX 2的光敏剂配合物，其中M是选自钌，锇，铁，铼和锝的过渡金属; 每个X是独立地选自N，C，C，O，C，O， H 2 O 2; H 2 O; 未被取代或被至少一个选自乙烯基，伯，仲或叔胺的基团取代的吡啶，OH和C 1-3 - 烷基，优选NSC - 和 - - 。 L是四齿多聚吡啶配体，其携带至少一个羧酸，磷酸或螯合基团和一个取代或未取代的碳原子数为1〜50的烷基，取代或未取代的碳原子数为2〜30的烷基酰胺基或取代或未取代的芳烷基 具有7至50个碳原子。 染料敏化电极包括具有导电表面的基底，形成在其上的氧化物半导体膜，以及上述的上述式（I）的敏化剂，负载在膜上。
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公开(公告)号：US20100326529A1
公开(公告)日：2010-12-30
申请号：US12872499
申请日：2010-08-31
申请人： Ashraful Islam , Liyuan Han , Atsushi Fukui
发明人： Ashraful Islam , Liyuan Han , Atsushi Fukui
CPC分类号： H01L51/0086 , C07F15/0053 , H01G9/2031 , H01G9/2059 , H01L51/0083 , H01L51/0088 , Y02E10/542 , Y02E10/549
摘要： A photosensitizing transition metal complex of the formula (Ia) MLY1, (Ib) MLX3 (Ic) MLY2X, (Id) MLY3X or (Ie) MLY4X in which M is a transition metal selected from ruthenium, osmium, iron, rhenium and technetium, preferably ruthenium or osmium. X is a co-ligand independently selected from NCS—, Cl—, Br—, I—, CN—, H2O; pyridine unsubstituted or substituted by at least one group selected from vinyl, primary, secondary or tertiary amine, OH and C1-30 alkyl, preferably NSC and CN—; L is a tridentate polypyridine ligand, carrying at least one carboxylic, phosphoric acid or a chelating group and one substituted or unsubstituted alkyl group having 1 to 50 carbon atoms, substituted or unsubstituted alkylamide group having 2 to 30 carbon atoms or substituted or unsubstituted aralkyl group having 7 to 50 carbon atoms. A dye-sensitized electrode includes a substrate having an electrically conductive surface, an oxide semiconductor film formed on the conductive surface, and the above sensitizer of formula (Ia), (Ib), (Ic), (Id) or (Ie) as specified above; supported on the film. A solar cell includes the above electrode, a counter electrode, and an electrolyte deposited there between.
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公开(公告)号：US20110011456A1
公开(公告)日：2011-01-20
申请号：US12933221
申请日：2009-03-17
申请人： Liyuan Han , Nobuhiro Fuke , Naoki Koide , Ashraful Islam , Atsushi Fukui
发明人： Liyuan Han , Nobuhiro Fuke , Naoki Koide , Ashraful Islam , Atsushi Fukui
CPC分类号： H01G9/2031 , H01G9/2054 , H01L2251/306 , Y02E10/542
摘要： A photosensitizer attaining high incident photon-to-current conversion efficiency and having long durability life and a solar cell using the photosensitizer are provided. A solar cell 1 includes: a semiconductor electrode 10 including a substrate 18 having a conductive film 16 formed on its surface and a porous semiconductor layer 20 formed on the substrate 18; a counter electrode 12 including a substrate 30 having a conductive film 28 formed on its surface; and a carrier transport layer 14 including conductive material, posed between the semiconductor electrode 10 and the counter electrode 12. The surface of porous semiconductor layer 20 is caused to carry a light absorber 22 including inorganic material 24 carrying organic molecules 26 each having an aromatic ring.
摘要翻译： 提供了获得高入射光子到电流转换效率并且具有长的耐久寿命的光敏剂和使用光敏剂的太阳能电池。 太阳能电池1包括：半导体电极10，其包括在其表面上形成有导电膜16的基板18和形成在基板18上的多孔半导体层20; 对电极12，其包括在其表面上形成有导电膜28的基板30; 以及包括导电材料的载流子传输层14，其设置在半导体电极10和对电极12之间。使多孔半导体层20的表面携带包含无机材料24的光吸收体22，该无机材料24具有各自具有芳环的有机分子26 。
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5.发明授权Photosensitizing transition metal complex and its use for photovoltaic cell 有权光敏化过渡金属络合物及其在光伏电池中的应用公开(公告)号：US07812251B2
公开(公告)日：2010-10-12
申请号：US10964745
申请日：2004-10-15
申请人： Ashraful Islam , Liyuan Han , Atsushi Fukui
发明人： Ashraful Islam , Liyuan Han , Atsushi Fukui
CPC分类号： H01L51/0086 , C07F15/0053 , H01G9/2031 , H01G9/2059 , H01L51/0083 , H01L51/0088 , Y02E10/542 , Y02E10/549
摘要： A photosensitizing transition metal complex of the formula (Ia) MLY1, (Ib) MLX3 (Ic) MLY2X, (Id) MLY3X or (Ie) MLY4X in which M is a transition metal selected from ruthenium, osmium, iron, rhenium and technetium, preferably ruthenium or osmium. X is a co-ligand independently selected from NCS—, Cl—, Br—, I—, CN—, H2O; pyridine unsubstituted or substituted by at least one group selected from vinyl, primary, secondary or tertiary amine, OH and C1-30 alkyl, preferably NSC and CN—; L is a tridentate polypyridine ligand, carrying at least one carboxylic, phosphoric acid or a chelating group and one substituted or unsubstituted alkyl group having 1 to 50 carbon atoms, substituted or unsubstituted alkylamide group having 2 to 30 carbon atoms or substituted or unsubstituted aralkyl group having 7 to 50 carbon atoms. A dye-sensitized electrode includes a substrate having an electrically conductive surface, an oxide semiconductor film formed on the conductive surface, and the above sensitizer of formula (Ia), (Ib), (Ic), (Id) or (Ie) as specified above, supported on the film. A solar cell includes the above electrode, a counter electrode, and an electrolyte deposited there between.
摘要翻译： 式（Ia）MLY1，（Ib）MLX3（Ic）MLY2X，（Id）MLY3X或（Ie）MLY4X的光敏过渡金属络合物，其中M是选自钌，锇，铁，铼和锝的过渡金属， 优选钌或锇。 X是独立地选自NCS-，Cl-，Br-，I-，CN-，H 2 O的共配体; 未取代的或被至少一个选自乙烯基，伯，仲或叔胺，OH和C 1-3烷基，优选NSC和CN-的基团取代的吡啶; L是携带至少一种羧酸，磷酸或螯合基团的三齿多吡啶配体，和一个取代或未取代的碳原子数为1〜50的烷基，取代或未取代的碳原子数为2〜30的烷基酰胺基或取代或未取代的芳烷基 具有7至50个碳原子。 染料敏化电极包括具有导电表面的基底，在导电表面上形成的氧化物半导体膜，以及上述式（Ia），（Ib），（Ic），（Id）或（Ie）的敏化剂作为 以上指定，支持电影。 太阳能电池包括上述电极，对电极和沉积在其间的电解质。
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6.发明申请Photosensitizing transition metal complex and its use for photovoltaic cell 有权光敏化过渡金属络合物及其在光伏电池中的应用公开(公告)号：US20050081911A1
公开(公告)日：2005-04-21
申请号：US10964745
申请日：2004-10-15
申请人： Ashraful Islam , Liyuan Han , Atsushi Fukui
发明人： Ashraful Islam , Liyuan Han , Atsushi Fukui
IPC分类号： H01L31/00
CPC分类号： H01L51/0086 , C07F15/0053 , H01G9/2031 , H01G9/2059 , H01L51/0083 , H01L51/0088 , Y02E10/542 , Y02E10/549
摘要： A photosensitizing transition metal complex of the formula (Ia) MLY1, (Ib) MLX3 (Ic) MLY2X, (Id) MLY3X or (Ie) MLY4X in which M is a transition metal selected from ruthenium, osmium, iron, rhenium and technetium, preferably ruthenium or osmium. X is a co-ligand independently selected from NCS—, Cl—, Br—, I—, CN—, H2O; pyridine unsubstituted or substituted by at least one group selected from vinyl, primary, secondary or tertiary amine, OH and C1-30 alkyl, preferably NSC and CN—; L is a tridentate polypyridine ligand, carrying at least one carboxylic, phosphoric acid or a chelating group and one substituted or unsubstituted alkyl group having 1 to 50 carbon atoms, substituted or unsubstituted alkylamide group having 2 to 30 carbon atoms or substituted or unsubstituted aralkyl group having 7 to 50 carbon atoms. A dye-sensitized electrode includes a substrate having an electrically conductive surface, an oxide semiconductor film formed on the conductive surface, and the above sensitizer of formula (Ia), (Ib), (Ic), (Id) or (Ie) as specified above, supported on the film. A solar cell includes the above electrode, a counter electrode, and an electrolyte deposited there between.
摘要翻译： 式（Ia）MLY 1，（Ib）MLX 3（Ic）MLY 2 X的光敏过渡金属络合物，（Id） MLY 3 X或（Ie）MLY 4 X其中M是选自钌，锇，铁，铼和锝的过渡金属，优选钌或锇。 X是独立地选自NCS-，Cl-，Br-，I-，CN-，H 2 O 2的共配体; 未取代的或被至少一个选自乙烯基，伯，仲或叔胺，OH和C 1-3烷基，优选NSC和CN-的基团取代的吡啶。 L是携带至少一种羧酸，磷酸或螯合基团的三齿多吡啶配体，和一个取代或未取代的碳原子数为1〜50的烷基，取代或未取代的碳原子数为2〜30的烷基酰胺基或取代或未取代的芳烷基 具有7至50个碳原子。 染料敏化电极包括具有导电表面的基底，在导电表面上形成的氧化物半导体膜，以及上述式（Ia），（Ib），（Ic），（Id）或（Ie）的敏化剂作为 以上指定，支持电影。 太阳能电池包括上述电极，对电极和沉积在其间的电解质。
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7.发明申请Photoelectrode, and Dye-Sensitized Solar Cell and Dye-Sensitized Solar Cell Module Using the Same 有权光电极和染料敏化太阳能电池和使用其的染料敏化太阳能电池模块公开(公告)号：US20080308155A1
公开(公告)日：2008-12-18
申请号：US11659080
申请日：2005-08-01
申请人： Atsushi Fukui , Ryohsuke Yamanaka , Liyuan Han
发明人： Atsushi Fukui , Ryohsuke Yamanaka , Liyuan Han
IPC分类号： H01L31/00
CPC分类号： H01G9/2031 , H01G9/2059 , Y02E10/542
摘要： A photoelectrode has a conductive substrate and a semiconductor layer formed on the conductive substrate, the semiconductor layer being formed of semiconductor particles, the semiconductor layer having a plurality of layers, the plurality of layers being different in an average particle diameter of semiconductor particles from one another, a distal layer of the plurality of layers, placed at a location farther from the substrate, covering at least a part of side faces of a proximal layer of the plurality of layers, placed at a location closer to the substrate.
摘要翻译： 光电极具有形成在导电性基板上的导电性基板和半导体层，该半导体层由半导体粒子形成，该半导体层具有多层，该多个层与半导体粒子的平均粒径不同 另一个是多个层的远侧层，放置在离衬底更远的位置处，覆盖多个层的近侧层的至少一部分侧面，放置在更靠近衬底的位置。
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8.发明授权Dye-sensitized solar cell, method of producing the same, and dye-sensitized solar cell module 有权染料敏化太阳能电池，其制造方法和染料敏化太阳能电池组件公开(公告)号：US09406446B2
公开(公告)日：2016-08-02
申请号：US13002070
申请日：2009-06-30
申请人： Atsushi Fukui , Ryoichi Komiya , Nobuhiro Fuke , Shinsuke Kobayashi , Liyuan Han
发明人： Atsushi Fukui , Ryoichi Komiya , Nobuhiro Fuke , Shinsuke Kobayashi , Liyuan Han
CPC分类号： H01G9/2059 , C09B57/10 , H01G9/0029 , H01G9/0036 , H01G9/2018 , H01G9/2022 , H01G9/2027 , H01G9/2031 , H01G9/2077 , H01G9/2081 , H01L51/0086 , H01L2251/306 , Y02E10/542 , Y02P70/521
摘要： Provided are a dye-sensitized solar cell wherein a counter electrode composed of a stable counter electrode conductive layer and a catalyst layer is formed on a porous insulation layer, and a dye-sensitized solar cell module wherein the dye-sensitized solar cell is utilized. A dye-sensitized solar cell includes a supporting body made of a light-transmissive material, and a laminate wherein a conductive layer, a photoelectric conversion layer having a porous semiconductor layer with a dye adsorbed therein, a porous insulation layer, a counter electrode conductive layer, and a catalyst layer are laminated in the order presented. The photoelectric conversion layer and the porous insulation lay are filled with a carrier transport material.
摘要翻译： 提供了一种染料敏化太阳能电池，其中在多孔绝缘层上形成由稳定的对电极导电层和催化剂层组成的对电极以及其中使用染料敏化太阳能电池的染料敏化太阳能电池模块。 染料敏化太阳能电池包括由透光材料制成的支撑体和层压体，其中导电层，具有吸附有染料的多孔半导体层的光电转换层，多孔绝缘层，对电极导电 层和催化剂层按照呈现的顺序层压。 光电转换层和多孔绝缘层填充载体输送材料。
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9.发明授权Paste for dye-sensitized solar cell, transparent insulation film for dye-sensitized solar cell, dye-sensitized solar cell, and dye-sensitized solar cell fabrication method 有权用于染料敏化太阳能电池的浆料，用于染料敏化太阳能电池的透明绝缘膜，染料敏化太阳能电池和染料敏化太阳能电池制造方法公开(公告)号：US09076598B2
公开(公告)日：2015-07-07
申请号：US12936309
申请日：2009-03-27
申请人： Liyuan Han , Ryohsuke Yamanaka , Nobuhiro Fuke , Atsushi Fukui , Shingo Takano , Gaku Fujihashi
发明人： Liyuan Han , Ryohsuke Yamanaka , Nobuhiro Fuke , Atsushi Fukui , Shingo Takano , Gaku Fujihashi
CPC分类号： H01G9/2031 , H01B1/122 , H01G9/2059 , H01G9/2081 , H01L51/0086 , H01L51/4226 , Y02E10/542 , Y02P70/521
摘要： A paste containing a silica polymer, made by substituting at least some of the surface functional groups thereof with alkyl groups, and solvent-removable inorganic particles is prepared, and the paste is applied and fired to form a transparent insulating film in a dye-sensitized solar cell.
摘要翻译： 制备含有通过用烷基取代至少一些其表面官能团而制成的二氧化硅聚合物和溶剂可除去的无机颗粒的糊料，并且将该糊剂施加并烧制以在染料敏化剂中形成透明绝缘膜 太阳能电池。
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10.发明授权Photoelectrode, and dye-sensitized solar cell and dye-sensitized solar cell module using the same 有权光电极和染料敏化太阳能电池和使用其的染料敏化太阳能电池模块公开(公告)号：US08581095B2
公开(公告)日：2013-11-12
申请号：US11659080
申请日：2005-08-01
申请人： Atsushi Fukui , Ryohsuke Yamanaka , Liyuan Han
发明人： Atsushi Fukui , Ryohsuke Yamanaka , Liyuan Han
IPC分类号： H01L31/00
CPC分类号： H01G9/2031 , H01G9/2059 , Y02E10/542
摘要： A photoelectrode has a conductive substrate and a semiconductor layer formed on the conductive substrate, the semiconductor layer being formed of semiconductor particles, the semiconductor layer having a plurality of layers, the plurality of layers being different in an average particle diameter of semiconductor particles from one another, a distal layer of the plurality of layers, placed at a location farther from the substrate, covering at least a part of side faces of a proximal layer of the plurality of layers, placed at a location closer to the substrate.
摘要翻译： 光电极具有形成在导电性基板上的导电性基板和半导体层，该半导体层由半导体粒子形成，该半导体层具有多层，该多个层与半导体粒子的平均粒径不同 另一个是多个层的远侧层，放置在离衬底更远的位置处，覆盖多个层的近侧层的至少一部分侧面，放置在更靠近衬底的位置。
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