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1.发明公开公开(公告)号：US20240336713A1
公开(公告)日：2024-10-10
申请号：US18296564
申请日：2023-04-06
发明人： Karthikeyan Kallupalayam Ramasamy , Mond F. Guo , Udishnu Sanyal , Robert Dagle , Johnny Saavedra Lopez , Vanessa Dagle
摘要： Disclosed herein are embodiments of a method for making jet-range olefins using co-oligomerization of a mixed olefin composition as a feedstock. In some embodiments, C2 and C3+ olefins can be reacted in the presence of a hybrid catalyst system to produce a jet-range olefin product suitable for use in making jet fuel. In some additional embodiments, C2 and C4 olefins can be reacted in the presence of a single catalyst component to produce a jet-range and/or diesel-range olefin product suitable for use in making jet fuel. Combinations comprising catalysts and feedstocks disclosed herein also are described, along with system embodiments for conducting the co-oligomerization method embodiments.
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公开(公告)号：US10647625B2
公开(公告)日：2020-05-12
申请号：US15837382
申请日：2017-12-11
发明人： Vanessa Dagle , Robert A. Dagle
摘要： A process for producing 1,3-butadiene (BD) from ethanol in a single step by s7passing a mixture containing ethanol in a gas phase over a multifunctional catalyst having a transition metal dispersion of at least 30% on a silica metal oxide support. In some examples the multifunctional catalyst comprises a silica metal oxide having a surface area of at least 200 m{circumflex over ( )}2/g. The multifunctional catalyst can include a transition metal oxide, a silica metal oxide made from a high purity silica gel, mesoporous silica and fumed silica, such as high purity SBA16, SBA15, or Davisil grade 646.
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公开(公告)号：US10538464B1
公开(公告)日：2020-01-21
申请号：US16165198
申请日：2018-10-19
发明人： Vanessa Dagle , Karl O. Albrecht , Robert A. Dagle
摘要： A system and process for processing biologically-derived compounds or a complex bio-oil by converting cyclic compounds in a complex bio-oil or biologically-derived compounds to desired materials such as high molecular weight paraffins with minimal carbon loss by using a ring-contraction catalyst to selectively produce C5 ring containing compounds; and then reacting the C5 ring containing compounds with a C5 ring opening catalyst in a second reactor to minimize carbon loss via cracking reactions.
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公开(公告)号：US11840491B2
公开(公告)日：2023-12-12
申请号：US17846476
申请日：2022-06-22
发明人： Vanessa Dagle , Robert A. Dagle
CPC分类号： C07C1/22 , B01J8/1881 , B01J8/24 , B01J21/066 , B01J21/08 , B01J23/72 , C07C2521/06 , C07C2521/08 , C07C2523/72
摘要： Systems for preparing butenes are provided. The systems can include a reactor inlet coupled to both a reactor and at least one reactant reservoir; at least one of the reactant reservoirs containing one or both of an aldehyde and/or ethanol; a catalyst within the reactor, the catalyst comprising a metal component and an acidic support material; and a reactor outlet operationally configured to convey a butene-rich reaction product to a product reservoir. Methods for preparing butenes are also provided. The methods can include exposing one or both of ethanol and/or an aldehyde to a catalyst comprising a metal component and an acidic support to form a butene-rich product that comprises one or both of 1-butene and/or 2-butene.
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公开(公告)号：US20230202946A1
公开(公告)日：2023-06-29
申请号：US18116181
申请日：2023-03-01
发明人： Vanessa Dagle , Robert A. Dagle
CPC分类号： C07C1/22 , B01J8/24 , B01J8/1881 , B01J23/72 , B01J21/08 , B01J21/066 , C07C2521/08 , C07C2523/72 , C07C2521/06
摘要： Systems for preparing butenes are provided. The systems can include a reactor inlet coupled to both a reactor and at least one reactant reservoir; at least one of the reactant reservoirs containing one or both of an aldehyde and/or ethanol; a catalyst within the reactor, the catalyst comprising a metal component and an acidic support material; and a reactor outlet operationally configured to convey a butene-rich reaction product to a product reservoir. Methods for preparing butenes are also provided. The methods can include exposing one or both of ethanol and/or an aldehyde to a catalyst comprising a metal component and an acidic support to form a butene-rich product that comprises one or both of 1-butene and/or 2-butene.
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公开(公告)号：US20220411348A1
公开(公告)日：2022-12-29
申请号：US17846476
申请日：2022-06-22
发明人： Vanessa Dagle , Robert A. Dagle
摘要： Systems for preparing butenes are provided. The systems can include a reactor inlet coupled to both a reactor and at least one reactant reservoir; at least one of the reactant reservoirs containing one or both of an aldehyde and/or ethanol; a catalyst within the reactor, the catalyst comprising a metal component and an acidic support material; and a reactor outlet operationally configured to convey a butene-rich reaction product to a product reservoir. Methods for preparing butenes are also provided. The methods can include exposing one or both of ethanol and/or an aldehyde to a catalyst comprising a metal component and an acidic support to form a butene-rich product that comprises one or both of 1-butene and/or 2-butene.
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公开(公告)号：US20180222813A1
公开(公告)日：2018-08-09
申请号：US15837382
申请日：2017-12-11
发明人： Vanessa Dagle , Robert A. Dagle
IPC分类号： C07C1/24
CPC分类号： C07C1/24 , C07C1/20 , C07C2521/06 , C07C2521/08 , C07C2523/42 , C07C2523/46 , C07C2523/50 , C07C11/167
摘要： A process for producing 1,3-butadiene (BD) from ethanol in a single step by s7 passing a mixture containing ethanol in a gas phase over a multifunctional catalyst having a transition metal dispersion of at least 30% on a silica metal oxide support. In some examples the multifunctional catalyst comprises a silica metal oxide having a surface area of at least 200 m̂2/g. The multifunctional catalyst can include a transition metal oxide, a silica metal oxide made from a high purity silica gel, mesoporous silica and fumed silica, such as high purity SBA16, SBA15, or Davisil grade 646.
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