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公开(公告)号：US6160154A
公开(公告)日：2000-12-12
申请号：US301698
申请日：1999-04-29
申请人： James Lawrence Spivack , Donald Wayne Whisenhunt, Jr. , James Norman Cawse , Bruce Fletcher Johnson , Marsha Mottel Grade , Grigorii Lev Soloveichik , John Yaw Ofori , Eric James Pressman
发明人： James Lawrence Spivack , Donald Wayne Whisenhunt, Jr. , James Norman Cawse , Bruce Fletcher Johnson , Marsha Mottel Grade , Grigorii Lev Soloveichik , John Yaw Ofori , Eric James Pressman
CPC分类号： B01J31/2234 , B01J23/89 , B01J31/0231 , B01J31/0235 , B01J2231/321 , B01J2531/16 , B01J2531/38 , B01J2531/46 , B01J2531/54 , B01J2531/62 , B01J2531/72 , B01J2531/824 , B01J2531/842 , B01J2531/847 , C07C68/005 , C07C69/96
摘要： A method and catalyst system for economically producing aromatic carbonates from aromatic hydroxy compounds. In one embodiment, the present invention provides a method of carbonylating aromatic hydroxy compounds by contacting at least one aromatic hydroxy compound with oxygen and carbon monoxide in the presence of a carbonylation catalyst system that includes a catalytic amount of an inorganic co-catalyst containing copper. In various alternative embodiments, the carbonylation catalyst system can include an effective amount of a palladium source and an effective amount of a halide composition. Further alternative embodiments can include catalytic amounts of various inorganic co-catalyst combinations.
摘要翻译： 用于从芳族羟基化合物经济地生产芳族碳酸酯的方法和催化剂体系。 在一个实施方案中，本发明提供了一种通过在包含催化量的含铜无机助催化剂的羰基化催化剂体系的存在下使至少一种芳族羟基化合物与氧和一氧化碳接触而使芳族羟基化合物羰基化的方法。 在各种替代实施方案中，羰基化催化剂体系可以包括有效量的钯源和有效量的卤化物组合物。 另外的替代实施方案可以包括催化量的各种无机助催化剂组合。
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公开(公告)号：US06380417B1
公开(公告)日：2002-04-30
申请号：US09662356
申请日：2000-09-15
申请人： James Lawrence Spivack , Donald Wayne Whisenhunt, Jr. , James Norman Cawse , Bruce Fletcher Johnson , Grigorii Lev Soloveichik , John Yaw Ofori , Eric James Pressman
发明人： James Lawrence Spivack , Donald Wayne Whisenhunt, Jr. , James Norman Cawse , Bruce Fletcher Johnson , Grigorii Lev Soloveichik , John Yaw Ofori , Eric James Pressman
IPC分类号： C07C6800
CPC分类号： B01J31/0231 , B01J23/6562 , B01J31/0239 , B01J31/0251 , B01J31/0271 , B01J31/2234 , B01J2231/34 , B01J2531/38 , B01J2531/39 , B01J2531/72 , B01J2531/824 , B01J2531/842 , B01J2531/847 , C07C68/005 , C07C69/96
摘要： A method and catalyst system for economically producing aromatic carbonates from aromatic hydroxy compounds. In one embodiment, the present invention provides a method of carbonylating aromatic hydroxy compounds by contacting at least one aromatic hydroxy compound with oxygen and carbon monoxide in the presence of a carbonylation catalyst system that includes a catalytic amount of a combination of inorganic co-catalysts containing manganese and nickel; manganese and iron; manganese and chromium; manganese and cerium; manganese and europium; manganese, cerium, and europium; manganese, iron, and europium; or manganese and thorium. In various alternative embodiments, the carbonylation catalyst system can include an effective amount of a palladium source and an effective amount of a halide composition. Further alternative embodiments can include catalytic amounts of various other inorganic co-catalyst combinations.
摘要翻译： 用于从芳族羟基化合物经济地生产芳族碳酸酯的方法和催化剂体系。 在一个实施方案中，本发明提供了一种通过在羰基化催化剂体系存在下使至少一种芳族羟基化合物与氧和一氧化碳接触来羰基化芳族羟基化合物的方法，所述羰基化催化剂体系包括催化量的无机助催化剂的组合， 锰和镍; 锰和铁; 锰和铬; 锰和铈; 锰和铕; 锰，铈和铕; 锰，铁和铕; 或锰和钍。 在各种替代实施方案中，羰基化催化剂体系可以包括有效量的钯源和有效量的卤化物组合物。 另外的替代实施方案可以包括催化量的各种其它无机助催化剂组合。
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公开(公告)号：US6143914A
公开(公告)日：2000-11-07
申请号：US301700
申请日：1999-04-29
申请人： James Lawrence Spivack , Donald Wayne Whisenhunt, Jr. , James Norman Cawse , Bruce Fletcher Johnson , Grigorii Lev Soloveichik , John Yaw Ofori , Eric James Pressman
发明人： James Lawrence Spivack , Donald Wayne Whisenhunt, Jr. , James Norman Cawse , Bruce Fletcher Johnson , Grigorii Lev Soloveichik , John Yaw Ofori , Eric James Pressman
CPC分类号： B01J31/0231 , B01J23/6562 , B01J31/0239 , B01J31/0251 , B01J31/0271 , B01J31/2234 , C07C68/005 , B01J2231/34 , B01J2531/38 , B01J2531/39 , B01J2531/72 , B01J2531/824 , B01J2531/842 , B01J2531/847
摘要： A method and catalyst system for economically producing aromatic carbonates from aromatic hydroxy compounds. In one embodiment, the present invention provides a method of carbonylating aromatic hydroxy compounds by contacting at least one aromatic hydroxy compound with oxygen and carbon monoxide in the presence of a carbonylation catalyst system that includes a catalytic amount of a combination of inorganic co-catalysts containing manganese and nickel; manganese and iron; manganese and chromium; manganese and cerium; manganese and europium; manganese, cerium, and europium; manganese, iron, and europium; or manganese and thorium. In various alternative embodiments, the carbonylation catalyst system can include an effective amount of a palladium source and an effective amount of a halide composition. Further alternative embodiments can include catalytic amounts of various other inorganic co-catalyst combinations.
摘要翻译： 用于从芳族羟基化合物经济地生产芳族碳酸酯的方法和催化剂体系。 在一个实施方案中，本发明提供了一种通过在羰基化催化剂体系存在下使至少一种芳族羟基化合物与氧和一氧化碳接触来羰基化芳族羟基化合物的方法，所述羰基化催化剂体系包括催化量的无机助催化剂的组合， 锰和镍; 锰和铁; 锰和铬; 锰和铈; 锰和铕 锰，铈和铕; 锰，铁和铕; 或锰和钍。 在各种替代实施方案中，羰基化催化剂体系可以包括有效量的钯源和有效量的卤化物组合物。 另外的替代实施方案可以包括催化量的各种其它无机助催化剂组合。
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公开(公告)号：US06514900B2
公开(公告)日：2003-02-04
申请号：US09780702
申请日：2001-02-12
申请人： James Lawrence Spivack , James Norman Cawse , Donald Wayne Whisenhunt, Jr. , Bruce Fletcher Johnson , Grigorii Lev Soloveichik
发明人： James Lawrence Spivack , James Norman Cawse , Donald Wayne Whisenhunt, Jr. , Bruce Fletcher Johnson , Grigorii Lev Soloveichik
IPC分类号： B01J2706
CPC分类号： B01J31/2234 , B01J23/56 , B01J31/0231 , B01J31/0239 , B01J31/0251 , B01J31/0271 , B01J2231/34 , B01J2531/16 , B01J2531/26 , B01J2531/38 , B01J2531/46 , B01J2531/54 , B01J2531/72 , B01J2531/824 , B01J2531/847 , C07C68/005 , C07C69/96
摘要： A method and catalyst system for economically producing aromatic carbonates from aromatic hydroxy compounds. In one embodiment, the present invention provides a method of carbonylating aromatic hydroxy compounds by contacting at least one aromatic hydroxy compound with oxygen and carbon monoxide in the presence of a carbonylation catalyst system that includes a catalytic amount of an inorganic co-catalyst containing titanium. In various alternative embodiments, the carbonylation catalyst system can include an effective amount of a palladium source and an effective amount of a halide composition. Further alternative embodiments can include catalytic amounts of various inorganic co-catalyst combinations.
摘要翻译： 用于从芳族羟基化合物经济地生产芳族碳酸酯的方法和催化剂体系。 在一个实施方案中，本发明提供了一种通过使羰基化芳族羟基化合物在包含催化量的含有钛的无机助催化剂的羰基化催化剂体系的存在下使至少一种芳族羟基化合物与氧和一氧化碳接触的方法。 在各种替代实施方案中，羰基化催化剂体系可以包括有效量的钯源和有效量的卤化物组合物。 另外的替代实施方案可以包括催化量的各种无机助催化剂组合。
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公开(公告)号：US06201146B1
公开(公告)日：2001-03-13
申请号：US09301697
申请日：1999-04-29
申请人： James Lawrence Spivack , James Norman Cawse , Donald Wayne Whisenhunt, Jr. , Bruce Fletcher Johnson , Grigorii Lev Soloveichik
发明人： James Lawrence Spivack , James Norman Cawse , Donald Wayne Whisenhunt, Jr. , Bruce Fletcher Johnson , Grigorii Lev Soloveichik
IPC分类号： C07C6800
CPC分类号： B01J31/2234 , B01J23/56 , B01J31/0231 , B01J31/0239 , B01J31/0251 , B01J31/0271 , B01J2231/34 , B01J2531/16 , B01J2531/26 , B01J2531/38 , B01J2531/46 , B01J2531/54 , B01J2531/72 , B01J2531/824 , B01J2531/847 , C07C68/005 , C07C69/96
摘要： A method and catalyst system for economically producing aromatic carbonates from aromatic hydroxy compounds. In one embodiment, the present invention provides a method of carbonylating aromatic hydroxy compounds by contacting at least one aromatic hydroxy compound with oxygen and carbon monoxide in the presence of a carbonylation catalyst system that includes a catalytic amount of an inorganic co-catalyst containing titanium. In various alternative embodiments, the carbonylation catalyst system can include an effective amount of a palladium source and an effective amount of a halide composition. Further alternative embodiments can include catalytic amounts of various inorganic co-catalyst combinations.
摘要翻译： 用于从芳族羟基化合物经济地生产芳族碳酸酯的方法和催化剂体系。 在一个实施方案中，本发明提供了一种通过使羰基化芳族羟基化合物在包含催化量的含有钛的无机助催化剂的羰基化催化剂体系的存在下使至少一种芳族羟基化合物与氧和一氧化碳接触的方法。 在各种替代实施方案中，羰基化催化剂体系可以包括有效量的钯源和有效量的卤化物组合物。 另外的替代实施方案可以包括催化量的各种无机助催化剂组合。
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公开(公告)号：US06566299B1
公开(公告)日：2003-05-20
申请号：US09604703
申请日：2000-06-23
申请人： James Lawrence Spivack , Donald Wayne Whisenhunt, Jr. , James Norman Cawse , Grigorii Lev Soloveichik
发明人： James Lawrence Spivack , Donald Wayne Whisenhunt, Jr. , James Norman Cawse , Grigorii Lev Soloveichik
IPC分类号： B01J2300
CPC分类号： B01J31/0231 , B01J31/0239 , B01J31/0251 , B01J31/0271 , B01J31/2234 , B01J2231/34 , B01J2531/16 , B01J2531/38 , B01J2531/46 , B01J2531/54 , B01J2531/62 , B01J2531/72 , B01J2531/824 , B01J2531/842 , B01J2531/847 , C07C68/005 , C07C69/96
摘要： A catalyst system for economically producing aromatic carbonates from aromatic hydroxy compounds. In one embodiment, the present invention provides a carbonylation catalyst system that includes a catalytic amount of an inorganic co-catalyst containing ytterbium. In various alternative embodiments, the carbonylation catalyst system can include an effective amount of a palladium source and an effective amount of a halide composition. Further alternative embodiments can include catalytic amounts of various inorganic co-catalyst combinations.
摘要翻译： 用于从芳族羟基化合物经济地生产芳族碳酸酯的催化剂体系。 在一个实施方案中，本发明提供了包含催化量的含有镱的无机助催化剂的羰基化催化剂体系。 在各种替代实施方案中，羰基化催化剂体系可以包括有效量的钯源和有效量的卤化物组合物。 另外的替代实施方案可以包括催化量的各种无机助催化剂组合。
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公开(公告)号：US6160155A
公开(公告)日：2000-12-12
申请号：US301699
申请日：1999-04-29
申请人： James Lawrence Spivack , Donald Wayne Whisenhunt, Jr. , James Norman Cawse , Grigorii Lev Soloveichik
发明人： James Lawrence Spivack , Donald Wayne Whisenhunt, Jr. , James Norman Cawse , Grigorii Lev Soloveichik
CPC分类号： B01J31/0231 , B01J31/0239 , B01J31/0251 , B01J31/0271 , B01J31/2234 , B01J2231/34 , B01J2531/16 , B01J2531/38 , B01J2531/46 , B01J2531/54 , B01J2531/62 , B01J2531/72 , B01J2531/824 , B01J2531/842 , B01J2531/847 , C07C68/005 , C07C69/96
摘要： A method and catalyst system for economically producing aromatic carbonates from aromatic hydroxy compounds. In one embodiment, the present invention provides a method of carbonylating aromatic hydroxy compounds by contacting at least one aromatic hydroxy compound with oxygen and carbon monoxide in the presence of a carbonylation catalyst system that includes a catalytic amount of an inorganic co-catalyst containing ytterbium. In various alternative embodiments, the carbonylation catalyst system can include an effective amount of a palladium source and an effective amount of a halide composition. Further alternative embodiments can include catalytic amounts of various inorganic co-catalyst combinations.
摘要翻译： 用于从芳族羟基化合物经济地生产芳族碳酸酯的方法和催化剂体系。 在一个实施方案中，本发明提供了一种通过在包含催化量的含有镱的无机助催化剂的羰基化催化剂体系的存在下使至少一种芳族羟基化合物与氧和一氧化碳接触而使芳族羟基化合物羰基化的方法。 在各种替代实施方案中，羰基化催化剂体系可以包括有效量的钯源和有效量的卤化物组合物。 另外的替代实施方案可以包括催化量的各种无机助催化剂组合。
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公开(公告)号：US06420587B2
公开(公告)日：2002-07-16
申请号：US09777818
申请日：2001-02-05
申请人： James Lawrence Spivack , Donald Wayne Whisenhunt , James Norman Cawse , Bruce Fletcher Johnson , Grigorii Lev Soloveichik , John Yaw Ofori , Eric James Pressman
发明人： James Lawrence Spivack , Donald Wayne Whisenhunt , James Norman Cawse , Bruce Fletcher Johnson , Grigorii Lev Soloveichik , John Yaw Ofori , Eric James Pressman
IPC分类号： B01J2344
CPC分类号： B01J31/2234 , B01J23/622 , B01J31/0231 , B01J31/0239 , B01J31/0251 , B01J31/0271 , B01J31/26 , B01J31/28 , B01J31/32 , B01J2231/34 , B01J2531/44 , B01J2531/46 , B01J2531/48 , B01J2531/72 , B01J2531/80 , B01J2531/821 , B01J2531/822 , B01J2531/824 , B01J2531/827 , B01J2531/842 , B01J2531/847 , C07C68/005 , C07C69/96
摘要： A method and catalyst system for economically producing aromatic carbonates from aromatic hydroxy compounds. In one embodiment, the present invention provides a method of carbonylating aromatic hydroxy compounds by contacting at least one aromatic hydroxy compound with oxygen and carbon monoxide in the presence of a carbonylation catalyst system that includes a catalytic amount of an inorganic co-catalyst containing lead and a catalytic amount of an inorganic co-catalyst containing titanium. In various alternative embodiments, the carbonylation catalyst system can include an effective amount of a palladium source and an effective amount of a halide composition. Further alternative embodiments can include catalytic amounts of various inorganic co-catalyst combinations.
摘要翻译： 用于从芳族羟基化合物经济地生产芳族碳酸酯的方法和催化剂体系。 在一个实施方案中，本发明提供了一种通过在羰基化催化剂体系存在下使至少一种芳族羟基化合物与氧和一氧化碳接触来羰基化芳族羟基化合物的方法，所述羰基化催化剂体系包括催化量的含铅的无机助催化剂和 催化量的含钛的无机助催化剂。 在各种替代实施方案中，羰基化催化剂体系可以包括有效量的钯源和有效量的卤化物组合物。 另外的替代实施方案可以包括催化量的各种无机助催化剂组合。
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公开(公告)号：US06197991B1
公开(公告)日：2001-03-06
申请号：US09301703
申请日：1999-04-29
申请人： James Lawrence Spivack , Donald Wayne Whisenhunt , James Norman Cawse , Bruce Fletcher Johnson , Grigorii Lev Soloveichik , John Yaw Ofori , Eric James Pressman
发明人： James Lawrence Spivack , Donald Wayne Whisenhunt , James Norman Cawse , Bruce Fletcher Johnson , Grigorii Lev Soloveichik , John Yaw Ofori , Eric James Pressman
IPC分类号： C07C6800
CPC分类号： B01J31/2234 , B01J23/622 , B01J31/0231 , B01J31/0239 , B01J31/0251 , B01J31/0271 , B01J31/26 , B01J31/28 , B01J31/32 , B01J2231/34 , B01J2531/44 , B01J2531/46 , B01J2531/48 , B01J2531/72 , B01J2531/80 , B01J2531/821 , B01J2531/822 , B01J2531/824 , B01J2531/827 , B01J2531/842 , B01J2531/847 , C07C68/005 , C07C69/96
摘要： A method and catalyst system for economically producing aromatic carbonates from aromatic hydroxy compounds. In one embodiment, the present invention provides a method of carbonylating aromatic hydroxy compounds by contacting at least one aromatic hydroxy compound with oxygen and carbon monoxide in the presence of a carbonylation catalyst system that includes a catalytic amount of an inorganic co-catalyst containing lead and a catalytic amount of an inorganic co-catalyst containing titanium. In various alternative embodiments, the carbonylation catalyst system can include an effective amount of a palladium source and an effective amount of a halide composition. Further alternative embodiments can include catalytic amounts of various inorganic co-catalyst combinations.
摘要翻译： 用于从芳族羟基化合物经济地生产芳族碳酸酯的方法和催化剂体系。 在一个实施方案中，本发明提供了一种通过在羰基化催化剂体系存在下使至少一种芳族羟基化合物与氧和一氧化碳接触来羰基化芳族羟基化合物的方法，所述羰基化催化剂体系包括催化量的含铅的无机助催化剂和 催化量的含钛的无机助催化剂。 在各种替代实施方案中，羰基化催化剂体系可以包括有效量的钯源和有效量的卤化物组合物。 另外的替代实施方案可以包括催化量的各种无机助催化剂组合。
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公开(公告)号：US06355597B1
公开(公告)日：2002-03-12
申请号：US09559855
申请日：2000-04-27
申请人： James Lawrence Spivack , Donald Wayne Whisenhunt, Jr. , James Norman Cawse , Bruce Fletcher Johnson , Kirill Shalyaev
发明人： James Lawrence Spivack , Donald Wayne Whisenhunt, Jr. , James Norman Cawse , Bruce Fletcher Johnson , Kirill Shalyaev
IPC分类号： B01J2316
CPC分类号： C07C68/005 , C07C69/96
摘要： A catalyst system for economically producing aromatic carbonates from aromatic hydroxy compounds. In one embodiment, the present invention provides a carbonylation catalyst system that includes a catalytic amount of an inorganic co-catalyst containing bismuth. In various alternative embodiments, the carbonylation catalyst system can include an effective amount of a palladium source and an effective amount of a halide composition. Further alternative embodiments can include catalytic amounts of various inorganic co-catalyst combinations.
摘要翻译： 用于从芳族羟基化合物经济地生产芳族碳酸酯的催化剂体系。 在一个实施方案中，本发明提供了包含催化量的含有铋的无机助催化剂的羰基化催化剂体系。 在各种替代实施方案中，羰基化催化剂体系可以包括有效量的钯源和有效量的卤化物组合物。 另外的替代实施方案可以包括催化量的各种无机助催化剂组合。
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