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1.发明授权Process for converting oxygenates to olefins using molecular sieve catalysts comprising desirable carbonaceous deposits 失效使用包含所需碳质沉积物的分子筛催化剂将含氧物转化为烯烃的方法
公开(公告)号：US6023005A
公开(公告)日：2000-02-08
申请号：US887766
申请日：1997-07-03
申请人： James Richardson Lattner , Hsiang-ning Sun , Stephen Neil Vaughn , Keith H. Kuechler , David C. Skouby
发明人： James Richardson Lattner , Hsiang-ning Sun , Stephen Neil Vaughn , Keith H. Kuechler , David C. Skouby
CPC分类号： B01J38/30 , B01J29/90 , C07C1/20 , B01J29/85 , C07C2529/85 , Y02P20/584 , Y02P30/42
摘要： The present invention relates to methods for selectively converting oxygenates to light olefins, preferably ethylene and propylene, in which desirable carbonaceous deposits are maintained on a total reaction volume of catalyst by totally regenerating only a portion of the total reaction volume of catalyst and mixing the regenerated portion with the unregenerated total reaction volume of catalyst.
摘要翻译： 本发明涉及选择性地将含氧化合物转化为轻质烯烃，优选乙烯和丙烯的方法，其中所需的碳质沉积物通过仅催化催化剂的总反应体积的一部分再生而混合在催化剂的总反应体积上，并将再生的 部分与催化剂未反应的总反应体积。
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公开(公告)号：US06552240B1
公开(公告)日：2003-04-22
申请号：US09708753
申请日：2000-11-08
IPC分类号： C07C170
CPC分类号： C10G3/60 , B01J29/85 , B01J29/90 , B01J38/30 , C07C1/20 , C07C2529/85 , C10G3/49 , C10G3/62 , C10G2300/4018 , C10G2300/4081 , C10G2300/802 , C10G2400/20 , Y02P20/584 , Y02P30/42 , C07C11/02
摘要： The present invention provides a method for converting a feed containing oxygenates to olefins and comprises the following steps: providing a feed including an oxygenate; contacting the feed in a reactor apparatus with a catalyst including a molecular sieve, the contacting taking place under conditions effective to convert the oxygenate to a product including a light olefin, the conditions including a gas superficial velocity of at least two meters per second at least one point in the reaction zone; and recirculating a first portion of the catalyst to recontact the feed.
摘要翻译： 本发明提供一种将含有含氧物的进料转化为烯烃的方法，包括以下步骤：提供包含含氧化合物的进料; 使反应器装置中的进料与包含分子筛的催化剂接触，在有效地将含氧化合物转化为包含轻质烯烃的产物的条件下进行接触，所述条件至少包括至少两米/秒的气体表观速度至少 反应区一点; 并再循环催化剂的第一部分以重新进料。
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公开(公告)号：US06455747B1
公开(公告)日：2002-09-24
申请号：US09414256
申请日：1999-10-07
IPC分类号： C07C170
CPC分类号： C07C1/20 , C07C2529/85 , C10G3/49 , C10G3/60 , C10G3/62 , C10G2300/4006 , C10G2300/4018 , C10G2300/4081 , C10G2300/802 , C10G2400/20 , Y02P30/42 , C07C11/02
摘要： The present invention provides a method for converting a feed containing oxygenates to olefins and comprises the following steps: providing a feed including an oxygenate; contacting the feed in a reactor apparatus with a catalyst including a molecular sieve, the contacting taking place under conditions effective to convert the oxygenate to a product including a light olefin, the conditions including a gas superficial velocity of at least two meters per second; and recirculating a first portion of the catalyst to recontact the feed.
摘要翻译： 本发明提供一种将含有含氧物的进料转化为烯烃的方法，包括以下步骤：提供包含含氧化合物的进料; 使反应器装置中的进料与包含分子筛的催化剂接触，在有效地将含氧化合物转化为包含轻质烯烃的产物的条件下进行接触，所述条件包括至少两米/秒的气体空塔速度; 并再循环催化剂的第一部分以重新进料。
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公开(公告)号：US06717023B2
公开(公告)日：2004-04-06
申请号：US10350502
申请日：2003-01-24
IPC分类号： C07C1207
CPC分类号： C10G3/60 , B01J29/85 , B01J29/90 , B01J38/30 , C07C1/20 , C07C2529/85 , C10G3/49 , C10G3/62 , C10G2300/4018 , C10G2300/4081 , C10G2300/802 , C10G2400/20 , Y02P20/584 , Y02P30/42 , C07C11/02
摘要： The present invention provides a method for converting a feed containing oxygenates to olefins and comprises the following steps: providing a feed including an oxygenate; contacting the feed in a reactor apparatus with a catalyst including a molecular sieve, the contacting taking place under conditions effective to convert the oxygenate to a product including a light olefin, the conditions including a gas superficial velocity of at least two meters per second at at least one point in the reaction zone; and recirculating a first portion of the catalyst to recontact the feed.
摘要翻译： 本发明提供一种将含有含氧物的进料转化为烯烃的方法，包括以下步骤：提供包含含氧化合物的进料; 将反应器装置中的进料与包含分子筛的催化剂接触，在有效地将含氧化合物转化为包含轻质烯烃的产物的条件下进行接触，所述条件包括在至少两米/秒的气体空塔速度 反应区至少有一点; 并再循环催化剂的第一部分以重新进料。
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公开(公告)号：US07223896B2
公开(公告)日：2007-05-29
申请号：US10835494
申请日：2004-04-29
申请人： Luc R. M. Martens , James R. Lattner , Rutton D. Patel , David C. Skouby , Stephen Neil Vaughn , Yun-feng Chang , Jesse F. Goellner , Mareel J. Janssen , Richard C. Senior
发明人： Luc R. M. Martens , James R. Lattner , Rutton D. Patel , David C. Skouby , Stephen Neil Vaughn , Yun-feng Chang , Jesse F. Goellner , Mareel J. Janssen , Richard C. Senior
CPC分类号： B01J8/1809 , B01J8/0025 , B01J2208/00672 , B01J2208/00752 , B01J2208/00769 , C07C1/20 , C10G3/42 , C10G3/45 , C10G3/47 , C10G3/49 , C10G2300/703 , C10G2400/20 , Y02P30/20 , C07C11/02
摘要： This invention provides processes for maintaining a desired particle size distribution in an oxygenate to olefin reaction system. In one embodiment, the invention comprises replacing lost catalyst fines with less active co-catalyst particles. By adding less active co-catalyst particles to the reaction system, desirable fluidization characteristics and hydrodynamics can be maintained without affecting the overall (or primary catalyst) performance and product selectivities. The invention is also directed to a population of catalyst particles having a desirable particle size distribution well-suited for realizing ideal fluidization and hydrodynamic characteristics.
摘要翻译： 本发明提供了在含氧化合物至烯烃反应体系中维持所需粒度分布的方法。 在一个实施方案中，本发明包括用较少活性的助催化剂颗粒代替失去的催化剂细粉。 通过将更少的活性助催化剂颗粒加入到反应体系中，可以保持所需的流化特性和流体动力学，而不影响总体（或初级催化剂）性能和产物选择性。 本发明还涉及具有适合于实现理想的流化和流体动力特性的理想粒度分布的催化剂颗粒群。
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公开(公告)号：US06613950B1
公开(公告)日：2003-09-02
申请号：US09587766
申请日：2000-06-06
IPC分类号： C07C100
CPC分类号： C07C1/20 , B01J29/85 , B01J29/90 , Y02P20/584 , C07C11/02
摘要： A process for method for the production of olefin product from an oxygenate-containing feedstock includes exposing a silicoaluminophosphate catalyst to an oxygenate-containing feedstock in a reaction zone under conditions effective to convert the oxygenate-containing feedstock to an olefin product, by stripping at least a portion of the exposed catalyst with a stripping gas; and returning at least a portion of the stripped catalyst directly to the reaction zone.
摘要翻译： 用于从含氧化合物原料生产烯烃产物的方法的方法包括在有效将含氧化合物的原料转化为烯烃产物的条件下，在反应区中将硅铝磷酸盐催化剂暴露于含氧化合物的原料，至少通过汽提 一部分暴露的催化剂与汽提气体; 并将至少一部分汽提的催化剂直接返回到反应区。
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公开(公告)号：US07396971B2
公开(公告)日：2008-07-08
申请号：US10210217
申请日：2002-08-01
申请人： Jeffrey S. Smith , Keith Holroyd Kuechler , Nicolas P. Coute , Rathna P. Davuluri , David C. Skouby
发明人： Jeffrey S. Smith , Keith Holroyd Kuechler , Nicolas P. Coute , Rathna P. Davuluri , David C. Skouby
IPC分类号： C07C1/20
CPC分类号： C10G3/62 , C10G3/49 , C10G2300/4018 , C10G2300/4093 , C10G2400/20 , Y02P30/20 , Y02P30/42
摘要： This invention is to a method and system for operating a hydrocarbon conversion process. A two stage reactor system is used in which the gas superficial velocity of the second reaction stage is greater than that in the first reaction stage. The first reaction stage operates at more continuous stirred tank reactor (CSTR) like characteristics, and the second reaction stage operates at more plug flow reactor (PFR) like characteristics.
摘要翻译： 本发明是用于操作烃转化方法的方法和系统。 使用两级反应器系统，其中第二反应级的气体表观速度大于第一反应级中的气体表观速度。 第一反应阶段在更连续的搅拌釜反应器（CSTR）的特性下操作，第二反应阶段在更多的活塞流反应器（PFR）的特性下操作。
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