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    METHOD FOR PRODUCING PROPYLENE OXIDE
    1.
    发明申请
    METHOD FOR PRODUCING PROPYLENE OXIDE 失效
    生产丙烯氧化物的方法

    公开(公告)号：US20100197945A1

    公开(公告)日：2010-08-05

    申请号：US12665172

    申请日：2008-06-19

    申请人： Hiroaki Abekawa ,  Tomonori Kawabata ,  Makoto Yako

    发明人： Hiroaki Abekawa ,  Tomonori Kawabata ,  Makoto Yako

    IPC分类号： C07D301/03

    CPC分类号： C07D301/06 ,  Y02P20/52

    摘要： There is disclosed a method for producing propylene oxide, which includes: reacting propylene, oxygen, and hydrogen in the presence of a noble metal catalyst and a titanosilicate catalyst in a liquid phase containing a polycyclic compound, which is unsubstituted or substituted with at least one substituent selected from Group B below, wherein the polycyclic compound is composed of two or more identical or different ring compounds selected from Group A below and the ring compounds are fused, directly bonded, or bonded by a linkage group selected from the group consisting of an oxygen atom, carbon chain, and a group composed of oxygen atom(s) and a carbon chain, provided that said polycyclic compound is not a polycyclic compound having hydroxy groups or oxo groups at para or. ortho positions. Group A consisting of benzene, cyclopentadiene, cycloheptatriene, furane, pyrane, cyclopentene, cyclopentane, cyclohexane, cyclohexene, cyclohexadiene, cycloheptane, cycloheptene, and cycloheptadiene. Group B consisting of halogen atom, alkyl group, alkenyl group, alkoxy group, hydroxyalkyl group, acyl group, oxo group, hydroxy group, and cyano group.

    摘要翻译： 公开了一种生产环氧丙烷的方法，其包括：在贵金属催化剂和钛硅酸盐催化剂存在下，在含有多环化合物的液相中使丙烯，氧和氢反应，该多环化合物是未取代的或被至少一个 取代基，其中所述多环化合物由两种或更多种相同或不同的选自下述A组的环化合物组成，并且所述环化合物通过选自以下的连接基团进行稠合，直接键合或键合： 氧原子，碳链和由氧原子和碳链组成的基团，条件是所述多环化合物不是在对位或具有羟基或氧代基的多环化合物。 邻位。 A组由苯，环戊二烯，环庚三烯，呋喃，吡喃，环戊烯，环戊烷，环己烷，环己烯，环己二烯，环庚烷，环庚烯和环庚二烯组成。 B族由卤素原子，烷基，烯基，烷氧基，羟基烷基，酰基，氧代基，羟基和氰基组成。

    Method for producing propylene oxide
    2.
    发明授权
    Method for producing propylene oxide 失效
    生产环氧丙烷的方法

    公开(公告)号：US07999125B2

    公开(公告)日：2011-08-16

    申请号：US12665172

    申请日：2008-06-19

    申请人： Hiroaki Abekawa ,  Tomonori Kawabata ,  Makoto Yako

    发明人： Hiroaki Abekawa ,  Tomonori Kawabata ,  Makoto Yako

    IPC分类号： C07D301/12 ,  C07D301/06

    CPC分类号： C07D301/06 ,  Y02P20/52

    摘要： There is disclosed a method for producing propylene oxide, which includes: reacting propylene, oxygen, and hydrogen in the presence of a noble metal catalyst and a titanosilicate catalyst in a liquid phase containing a polycyclic compound, which is unsubstituted or substituted with at least one substituent selected from Group B below, wherein the polycyclic compound is composed of two or more identical or different ring compounds selected from Group A below and the ring compounds are fused, directly bonded, or bonded by a linkage group selected from the group consisting of an oxygen atom, carbon chain, and a group composed of oxygen atom(s) and a carbon chain, provided that said polycyclic compound is not a polycyclic compound having hydroxy groups or oxo groups at para or. ortho positions. Group A consisting of benzene, cyclopentadiene, cycloheptatriene, furane, pyrane, cyclopentene, cyclopentane, cyclohexane, cyclohexene, cyclohexadiene, cycloheptane, cycloheptene, and cycloheptadiene. Group B consisting of halogen atom, alkyl group, alkenyl group, alkoxy group, hydroxyalkyl group, acyl group, oxo group, hydroxy group, and cyano group.

    摘要翻译： 公开了一种生产环氧丙烷的方法，其包括：在贵金属催化剂和钛硅酸盐催化剂存在下，在含有多环化合物的液相中使丙烯，氧和氢反应，该多环化合物是未取代的或被至少一个 取代基，其中所述多环化合物由两种或更多种相同或不同的选自下述A组的环化合物组成，并且所述环化合物通过选自以下的连接基团进行稠合，直接键合或键合： 氧原子，碳链和由氧原子和碳链组成的基团，条件是所述多环化合物不是在对位或具有羟基或氧代基的多环化合物。 邻位。 A组由苯，环戊二烯，环庚三烯，呋喃，吡喃，环戊烯，环戊烷，环己烷，环己烯，环己二烯，环庚烷，环庚烯和环庚二烯组成。 B族由卤素原子，烷基，烯基，烷氧基，羟基烷基，酰基，氧代基，羟基和氰基组成。

    METHOD FOR PRODUCING PROPYLENE OXIDE
    4.
    发明申请
    METHOD FOR PRODUCING PROPYLENE OXIDE 审中-公开
    生产丙烯氧化物的方法

    公开(公告)号：US20120296102A1

    公开(公告)日：2012-11-22

    申请号：US13576319

    申请日：2011-01-27

    申请人： Tomonori Kawabata ,  Hiroaki Abekawa

    发明人： Tomonori Kawabata ,  Hiroaki Abekawa

    IPC分类号： C07D301/06

    CPC分类号： C07D301/06 ,  B01J21/063 ,  B01J21/18 ,  B01J23/42 ,  B01J23/44 ,  B01J29/00 ,  Y02P20/52

    摘要： It is intended to provide a production method for producing propylene oxide from propylene, hydrogen and oxygen, with improved reaction rate. The present invention provides a method for producing propylene oxide, comprising a step of reacting propylene, hydrogen and oxygen, in the presence of a Pd-supported catalyst, a titanosilicate catalyst and a Pd-free carbon material, in a liquid phase.

    摘要翻译： 旨在提供从丙烯，氢气和氧气生产环氧丙烷的制备方法，其反应速率提高。 本发明提供了一种生产环氧丙烷的方法，包括在Pd相负载的催化剂，钛硅酸盐催化剂和无Pd的碳材料存在下，在液相中使丙烯，氢气和氧气反应的步骤。

    Process for Producing of Epoxy Compound
    5.
    发明申请
    Process for Producing of Epoxy Compound 失效
    环氧化合物生产工艺

    公开(公告)号：US20090054670A1

    公开(公告)日：2009-02-26

    申请号：US12087461

    申请日：2007-01-09

    申请人： Tomonori Kawabata ,  Hiroaki Abekawa

    发明人： Tomonori Kawabata ,  Hiroaki Abekawa

    IPC分类号： C07D301/06

    CPC分类号： C07D301/06

    摘要： An object of the present invention is to provide an efficient process for producing an epoxy compound from olefin, oxygen and hydrogen. The process of the present invention is characterized in that an olefin, oxygen and hydrogen are reacted in a liquid phase in the presence of a titanosilicate selected from the group consisting of a crystalline titanosilicate having MEL structure, MTW structure, BEA structure, MWW structure or DON structure, a mesoporous titanosilicate and a lamellar titanosilicate, a noble metal catalyst, and a quinoid compound or a dihydro-form of quinoid compound.

    摘要翻译： 本发明的目的是提供从烯烃，氧和氢生产环氧化合物的有效方法。 本发明的方法的特征在于，在钛酸硅酸盐存在下，在液相中使烯烃，氧和氢反应，所述钛硅酸盐选自具有MEL结构的结晶钛硅酸盐，MTW结构，BEA结构，MWW结构或 DON结构，介孔钛硅酸盐和层状钛硅酸盐，贵金属催化剂和醌类化合物或二氢型喹啉化合物。

    Method for producing epoxy compound
    6.
    发明授权
    Method for producing epoxy compound 失效
    环氧化合物的制备方法

    公开(公告)号：US08207359B2

    公开(公告)日：2012-06-26

    申请号：US12226729

    申请日：2007-04-26

    申请人： Tomonori Kawabata ,  Hiroaki Abekawa

    发明人： Tomonori Kawabata ,  Hiroaki Abekawa

    IPC分类号： C07D301/12 ,  C07D301/06

    CPC分类号： C07D301/04 ,  C07D303/04

    摘要： A method for producing an epoxy compound characterized by comprising contacting an olefin, oxygen and hydrogen with a noble metal and a crystalline titanosilicate having an MFI structure in a liquid phase in the presence of a quinoid compound selected from the group consisting of a phenanthraquinone compound and a compound represented by formula (1) wherein R1, R2, R3 and R4 represent a hydrogen atom, or R1 and R2 or R3 and R4 adjacent to each other are each independently bound at the ends and represent, together with a carbon atom of a quinone to which they are respectively attached, a benzene ring which may be substituted with an alkyl group or a hydroxyl group, or a naphthalene ring which may be substituted with an alkyl group or a hydroxyl group; and X and Y, which is the same or different, represent an oxygen atom or an NH group, or a dihydro compound thereof.

    摘要翻译： 一种制备环氧化合物的方法，其特征在于包括在烯烃化合物存在下，将烯烃，氧和氢与贵金属和具有MFI结构的结晶钛硅酸盐接触，所述醌类化合物选自菲醌化合物和 由式（1）表示的化合物，其中R 1，R 2，R 3和R 4表示氢原子，或者R 1和R 2或彼此相邻的R 3和R 4各自独立地结合，并且与 分别连接的醌，可被烷基或羟基取代的苯环，或可被烷基或羟基取代的萘环; X和Y相同或不同，表示氧原子或NH基，或其二氢化合物。

    Process for producing propylene oxide
    8.
    发明授权
    Process for producing propylene oxide 失效
    生产环氧丙烷的方法

    公开(公告)号：US08273907B2

    公开(公告)日：2012-09-25

    申请号：US12097975

    申请日：2006-12-25

    申请人： Tomonori Kawabata ,  Hiroaki Abekawa

    发明人： Tomonori Kawabata ,  Hiroaki Abekawa

    IPC分类号： C07D301/06

    CPC分类号： B01J29/89 ,  B01J23/44 ,  B01J2229/186 ,  C07D301/10 ,  C07D301/12 ,  C07D303/04 ,  Y02P20/52

    摘要： A process for more efficiently producing propylene oxide from propylene, oxygen, and hydrogen with catalysts which comprise a noble metal and a titanosilicate having pores not smaller than a 12-membered oxygen ring. The process for propylene oxide production is characterized by reacting propylene, oxygen, and hydrogen in a solution comprising water, a nitrite compound, and an ammonium salt in the presence of a noble metal catalyst and a titanosilicate catalyst having pores not smaller than a 12-membered oxygen ring.

    摘要翻译： 一种用丙烯，氧气和氢气更有效地生产环氧丙烷的方法，该催化剂包含贵金属和具有不小于12元氧环的孔的钛硅酸盐。 环氧丙烷生产方法的特征在于在贵金属催化剂和具有不小于12重量％的孔的钛硅酸盐催化剂存在下，在包含水，亚硝酸盐化合物和铵盐的溶液中使丙烯，氧气和氢气反应， 元氧环。

    PROCESS FOR PRODUCING PROPYLENE OXIDE
    9.
    发明申请
    PROCESS FOR PRODUCING PROPYLENE OXIDE 失效
    生产丙烯氧化物的方法

    公开(公告)号：US20090264665A1

    公开(公告)日：2009-10-22

    申请号：US12097975

    申请日：2006-12-25

    申请人： Tomonori Kawabata ,  Hiroaki Abekawa

    发明人： Tomonori Kawabata ,  Hiroaki Abekawa

    IPC分类号： C07D301/06

    CPC分类号： B01J29/89 ,  B01J23/44 ,  B01J2229/186 ,  C07D301/10 ,  C07D301/12 ,  C07D303/04 ,  Y02P20/52

    摘要： A process for more efficiently producing propylene oxide from propylene, oxygen, and hydrogen with catalysts which comprise a noble metal and a titanosilicate having pores not smaller than a 12-membered oxygen ring. The process for propylene oxide production is characterized by reacting propylene, oxygen, and hydrogen in a solution comprising water, a nitrite compound, and an ammonium salt in the presence of a noble metal catalyst and a titanosilicate catalyst having pores not smaller than a 12-membered oxygen ring.

    摘要翻译： 一种用丙烯，氧气和氢气更有效地生产环氧丙烷的方法，该催化剂包含贵金属和具有不小于12元氧环的孔的钛硅酸盐。 环氧丙烷生产方法的特征在于在贵金属催化剂和具有不小于12重量％的孔的钛硅酸盐催化剂存在下，在包含水，亚硝酸盐化合物和铵盐的溶液中使丙烯，氧气和氢气反应， 元氧环。

    Process for producing of epoxy compound
    10.
    发明授权
    Process for producing of epoxy compound 失效
    环氧化合物的制备方法

    公开(公告)号：US07994349B2

    公开(公告)日：2011-08-09

    申请号：US12087461

    申请日：2007-01-09

    申请人： Tomonori Kawabata ,  Hiroaki Abekawa

    发明人： Tomonori Kawabata ,  Hiroaki Abekawa

    IPC分类号： C07D301/12 ,  C07D301/06

    CPC分类号： C07D301/06

    摘要： An object of the present invention is to provide an efficient process for producing an epoxy compound from olefin, oxygen and hydrogen. The process of the present invention is characterized in that an olefin, oxygen and hydrogen are reacted in a liquid phase in the presence of a titanosilicate selected from the group consisting of a crystalline titanosilicate having MEL structure, MTW structure, BEA structure, MWW structure or DON structure, a mesoporous titanosilicate and a lamellar titanosilicate, a noble metal catalyst, and a quinoid compound or a dihydro-form of quinoid compound.

    摘要翻译： 本发明的目的是提供从烯烃，氧和氢生产环氧化合物的有效方法。 本发明的方法的特征在于，在钛酸硅酸盐存在下，在液相中使烯烃，氧和氢反应，所述钛硅酸盐选自具有MEL结构的结晶钛硅酸盐，MTW结构，BEA结构，MWW结构或 DON结构，介孔钛硅酸盐和层状钛硅酸盐，贵金属催化剂和醌类化合物或二氢型喹啉化合物。