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    1-cycloalkenyltetrazolinones
    1.
    发明授权
    1-cycloalkenyltetrazolinones 失效
    1-环烯基四唑啉酮

    公开(公告)号：US5654257A

    公开(公告)日：1997-08-05

    申请号：US601748

    申请日：1996-02-15

    申请人： Toshio Goto ,  Yoshinori Kitagawa ,  Seishi Ito ,  Katsuhiko Shibuya ,  Tatsuya Yamaoka ,  Chieko Ueno ,  Yoshiko Kyo

    发明人： Toshio Goto ,  Yoshinori Kitagawa ,  Seishi Ito ,  Katsuhiko Shibuya ,  Tatsuya Yamaoka ,  Chieko Ueno ,  Yoshiko Kyo

    IPC分类号： C07D401/06 ,  A01N47/38 ,  C07D257/04 ,  C07D403/06 ,  A01N43/713

    CPC分类号： C07D257/04 ,  A01N47/38

    摘要： 1-cycloalkenyltetrazolinone derivatives of the following herbicidal formula ##STR1## R.sup.1 is cycloalkenyl which may optionally be substituted by halogen C.sub.1-4 alkyl, or bicycloalkenyl which may optionally be substituted by halogen or C.sub.1-4 alkyl, andR.sup.2 and R.sup.3 each independently is alkyl, cycloalkyl, phenyl (optionally substituted by a member selected from the group consisting of nitro, cyano, halogen, alkyl, haloalkyl, alkoxy, haloalkoxy and alkylthio), alkenyl and alkynyl,orR.sup.2 and R.sup.3 together with the N-atom to which they are bonded form, a 5- or 6-membered heterocyclic ring which may optionally contain a further hetero atom, said heterocyclic ring optionally being benzo-condensed, or a C-.sub.1-4 alkyl,and intermediates therefore of the formula ##STR2##

    摘要翻译： 以下除草式R 1的1-环烯基四唑啉酮衍生物是可任选被卤素C 1-4烷基取代的环烯基，或可任意被卤素或C 1-4烷基取代的双环烯基，R 2和R 3各自独立地为烷基 ，环烷基，苯基（任选被选自硝基，氰基，卤素，烷基，卤代烷基，烷氧基，卤代烷氧基和烷硫基的成员取代），烯基和炔基，或者R 2和R 3与它们的N-原子一起 键合形式，可任选地含有另外的杂原子的所述5或6元杂环，所述杂环任选地被苯并稠合，或C 1-4烷基，因此具有下式的中间体：

    Tetrazolinones
    2.
    发明授权
    Tetrazolinones 失效
    四唑啉酮

    公开(公告)号：US5605920A

    公开(公告)日：1997-02-25

    申请号：US618954

    申请日：1996-03-20

    申请人： Toshio Goto ,  Yoshinori Kitagawa ,  Seishi Ito ,  Katsuhiko Shibuya ,  Tatsuya Yamaoka ,  Chieko Ueno ,  Yoshiko Kyo

    发明人： Toshio Goto ,  Yoshinori Kitagawa ,  Seishi Ito ,  Katsuhiko Shibuya ,  Tatsuya Yamaoka ,  Chieko Ueno ,  Yoshiko Kyo

    IPC分类号： C07D401/06 ,  A01N47/38 ,  C07D257/04 ,  C07D401/12 ,  C07D403/06 ,  C07D403/12 ,  A01N43/713 ,  A61K31/41

    CPC分类号： C07D257/04 ,  A01N47/38 ,  C07D401/12 ,  C07D403/12

    摘要： Disclosed are herbicidal tetrazolinone derivatives, selective in paddy fields of the formula ##STR1## wherein X represents C.sub.1-4 alkyl,n represents 1, 2, 3 or 4,R.sup.1 and R.sup.2 each independently represents C.sub.1-6 alkyl, C.sub.2-4 alkenyl, C.sub.2-6 alkynyl, C.sub.3-8 cycloalkyl, aryl which may optionally be substituted (wherein the substituent is at least one radical selected from the group consisting of halogen, C.sub.1-4 alkyl, C.sub.1-2 haloalkyl, C.sub.1-2 haloalkoxy, C.sub.1-2 haloalkylthio, acyl, nitro and cyano) or aralkyl optionally substituted by halogen orR.sup.1 and R.sup.2 form, together with the N-atom to which they are bonded, a cyclic ring which may be substituted. Also, disclosed are novel intermediates useful in the preparation of the compounds of formula (I).

    摘要翻译： 公开了除草性四唑啉酮衍生物，其在式（I）的水田中是选择性的，其中X表示C1-4烷基，n表示1,2,3或4，R1和R2各自独立地表示C1-6烷基，C2- 4链烯基，C 2-6炔基，C 3-8环烷基，可任选取代的芳基（其中取代基是至少一个选自卤素，C 1-4烷基，C 1-2卤代烷基，C 1-2卤代烷氧基 ，C 1-2卤代烷硫基，酰基，硝基和氰基）或任选被卤素或R 1和R 2形式取代的芳烷基与它们所键合的N-原子一起可以被取代的环状基团。 还公开了可用于制备式（I）化合物的新型中间体。

    Herbicidal 1-substituted methyl-tetrazolinones
    3.
    发明授权
    Herbicidal 1-substituted methyl-tetrazolinones 失效
    除草剂1-取代的甲基 - 四唑啉酮

    公开(公告)号：US06262275B1

    公开(公告)日：2001-07-17

    申请号：US09368475

    申请日：1999-08-04

    申请人： Toshio Goto ,  Yoshinori Kitagawa ,  Seishi Ito ,  Katsuhiko Shibuya ,  Chieko Ueno ,  Yoshiko Kyo

    发明人： Toshio Goto ,  Yoshinori Kitagawa ,  Seishi Ito ,  Katsuhiko Shibuya ,  Chieko Ueno ,  Yoshiko Kyo

    IPC分类号： C07D41306

    CPC分类号： C07D257/04 ,  A01N47/38

    摘要： Novel 1-substituted methyltetrazolinones of the formula (I) wherein R1 represents a 5-membered heterocyclic radical which has 1 to 3 heteroatoms selected arbitrarily from the group consisting of N, O and S and which is optionally substituted by halogen and/or C1-4 alkyl, or represents oxiran-2-yl, optionally chloro-substituted pyridyl or C1-4 alkyl-S(O)m— wherein m represents 0, 1 or 2, or represents a C3-6 alicyclic hydrocarbon radical; R2 and R3 represent, independently of one another, C1-6 alkyl, C3-7 cycloalkyl or optionally substituted phenyl, or R2 and R3 may form, together with the N-atom to which they are bonded, an optionally substituted ring; R4 represents a hydrogen atom or methyl; and n represents 0 or 1; as well as for their preparation processes and novel intermediates in their production. The inventive compounds of formula (I) are used as herbicides.

    摘要翻译： 式（I）的新的1-取代的甲基四唑啉酮，其中R 1表示具有1至3个杂原子的5元杂环基，其任选地由N，O和S组成，并且任选被卤素和/或C 1-4取代 烷基，或表示环氧乙烷-2-基，任选氯取代的吡啶基或C 1-4烷基-S（O）m - ，其中m表示0,1或2，或表示C 3-6脂族烃基; R 2和R 3彼此独立地表示C 1-6烷基，C 3-7环烷基或任选取代的苯基，或者R 2和R 3可以与它们所键合的N-原子一起形成任选取代的环; R4表示氢原子或甲基; n表示0或1; 以及它们的制备过程和新型中间体的生产。 本发明式（I）化合物用作除草剂。

    Herbicidal 1-substituted methyl-tetrazolinones
    4.
    发明授权
    Herbicidal 1-substituted methyl-tetrazolinones 失效
    除草剂1-取代的甲基 - 四唑啉酮

    公开(公告)号：US6017853A

    公开(公告)日：2000-01-25

    申请号：US890432

    申请日：1997-07-09

    申请人： Toshio Goto ,  Yoshinori Kitagawa ,  Seishi Ito ,  Katsuhiko Shibuya ,  Chieko Ueno ,  Yoshiko Kyo

    发明人： Toshio Goto ,  Yoshinori Kitagawa ,  Seishi Ito ,  Katsuhiko Shibuya ,  Chieko Ueno ,  Yoshiko Kyo

    IPC分类号： A01N47/38 ,  C07D257/04 ,  A01N43/72 ,  C07D413/12

    CPC分类号： C07D257/04 ,  A01N47/38

    摘要： Novel 1-substituted methyltetrazolinones of the formula (I) ##STR1## wherein R.sup.1 represents a 5-membered heterocyclic radical which has 1 to 3 heteroatoms selected arbitrarily from the group consisting of N, O and S and which is optionally substituted by halogen and/or C.sub.1-4 alkyl, or represents oxiran-2-yl, optionally chloro-substituted pyridyl or C.sub.1-4 alkyl-S(O).sub.m --wherein m represents 0, 1 or 2, or represents a C.sub.3-6 alicyclic hydrocarbon radical; R.sup.2 and R.sup.3 represent, independently of one another, C.sub.1-4 alkyl, C.sub.3-7 cycloalkyl or optionally substituted phenyl, or R.sup.2 and R.sup.3 may form, together with the N-atom to which they are bonded, an optionally substituted ring; R.sup.4 represents a hydrogen atom or methyl; and n represents 0 or 1; as well as for their preparation processes and novel intermediates in their production. The inventive compounds of formula (I) are used as herbicides.

    摘要翻译： 式（I）的新型1-取代的甲基四唑啉酮，其中R 1表示具有1至3个杂原子的5元杂环基，其任选地由N，O和S组成的组中选择，并且其任选被卤素和/或C1- 或烷基，或表示环氧乙烷-2-基，任选氯取代的吡啶基或C 1-4烷基-S（O）m - ，其中m表示0,1或2，或表示C 3-6脂环族烃基; R 2和R 3彼此独立地表示C 1-4烷基，C 3-7环烷基或任选取代的苯基，或者R 2和R 3可以与它们所键合的N-原子一起形成任选取代的环; R4表示氢原子或甲基; n表示0或1; 以及它们的制备过程和新型中间体的生产。 本发明式（I）化合物用作除草剂。

    Herbicidal 1-cyclopropyl tetrazolinones
    5.
    发明授权
    Herbicidal 1-cyclopropyl tetrazolinones 失效
    除草1-环丙基四唑啉酮

    公开(公告)号：US5650374A

    公开(公告)日：1997-07-22

    申请号：US553160

    申请日：1995-11-07

    申请人： Toshio Goto ,  Yoshinori Kitagawa ,  Seishi Ito ,  Katsuhiko Shibuya ,  Kazuhiro Ukawa ,  Yoshiko Kyo

    发明人： Toshio Goto ,  Yoshinori Kitagawa ,  Seishi Ito ,  Katsuhiko Shibuya ,  Kazuhiro Ukawa ,  Yoshiko Kyo

    IPC分类号： C07D401/06 ,  A01N47/38 ,  C07D257/04 ,  C07D403/06 ,  C07D405/12 ,  A01N43/713 ,  A01N43/72

    CPC分类号： C07D257/04 ,  A01N47/38

    摘要： Herbicidal 1-cyclopropyl tetrazolinones of the formula ##STR1## wherein X represents C.sub.1-3 alkyl, C.sub.2-4 alkenyl or halogen,n represents 0 to 5,R.sup.1 and R.sup.2 each independently represents C.sub.1-6 alkyl, C.sub.2-6 alkenyl, C.sub.2-6 alkynyl, C.sub.3-7 cycloalkyl which may optionally be substituted by C.sub.1-3 alkyl, epoxy-C.sub.3-5 alkan-1-yl, phenyl which may optionally be substituted, or aralkyl which may optionally be substituted, orR.sup.1 and R.sup.2 together with the N-atom to which they are attached, represent a cyclic ring which may be substituted, and some novel intermediates therefor.

    摘要翻译： 式（I）的除草1-环丙基四唑啉酮其中X代表C1-3烷基，C2-4烯基或卤素，n代表0-5，R1和R2各自独立地表示C1-6烷基，C2-6烯基 C 2-6炔基，可任选被C 1-3烷基取代的C 3-7环烷基，环烷基-C 3-5烷基-1-基，可任意被取代的苯基或可任意被取代的芳烷基，或R 1和 R2与它们所连接的N-原子一起表示可以被取代的环状环，以及一些新的中间体。

    Phenylacetylene derivatives
    7.
    发明授权
    Phenylacetylene derivatives 失效
    苯乙炔衍生物

    公开(公告)号：US06174839B1

    公开(公告)日：2001-01-16

    申请号：US09255959

    申请日：1999-02-23

    申请人： Akihiko Yanagi ,  Shin-ichi Narabu ,  Toshio Goto ,  Seishi Ito ,  Natsuko Minegishi ,  Tatsuya Yamaoka ,  Chieko Ueno

    发明人： Akihiko Yanagi ,  Shin-ichi Narabu ,  Toshio Goto ,  Seishi Ito ,  Natsuko Minegishi ,  Tatsuya Yamaoka ,  Chieko Ueno

    IPC分类号： A01N43647

    CPC分类号： C07D231/38 ,  A01N43/54 ,  A01N43/56 ,  A01N43/713 ,  A01N43/82 ,  A01N47/20 ,  A01N55/00 ,  C07D239/22 ,  C07D239/54 ,  C07D257/04 ,  C07D271/113 ,  C07D405/04 ,  C07F7/0812

    摘要： The invention is related to a novel phenylacetylene derivates of formula: wherein X represents hydrogen, halogen, optionally substituted C1-6 alkyl; Y represents hydrogen, halogen, cyano, nitro, optionally substituted C1-6 alkyl, C1-6 alkoxy, C3-8 cycloalkoxy, optionally substituted C1-6 alkylthio, C3-8 cycloalkylthio, C1-6 alkylsulfinyl, optionally substituted C1-6 alkylsulfonyl, C3-8 cycloalkylsulfonyl, C1-6 alkylsulfonyloxy, optionally substituted sulfonamide, optionally substituted carboxamide, etc., or Y may form together with Z which is bonded to the vicinal carbon atom a 5- or 6-membered ring; n is 0 or 1; Z represents hydrogen or halogen; m is 1 or 2; R represents hydrogen, halogen, C1-6 alkyl, tri(C1-6 alkyl)silyl, COORc or CONRdRe; Q represents a heterocyclic group, and their use as herbicid.

    摘要翻译： 本发明涉及下式的新型苯乙炔衍生物：其中X表示氢，卤素，任选取代的C 1-6烷基; Y代表氢，卤素，氰基，硝基，任选取代的C 1-6烷基，C 1-6烷氧基，C 3-8环烷氧基，任选取代的C 1-6烷硫基，C 3-8环硫基，C 1-6烷基亚磺酰基，任选取代的C 1-6烷基磺酰基 ，C 3-8环烷基磺酰基，C 1-6烷基磺酰氧基，任选取代的磺酰胺，任选取代的羧酰胺等，或Y可以与连接在邻位碳原子上的5或6元环一起形成; n为0或1; Z表示氢或卤素; m为1或2; R表示氢，卤素，C 1-6烷基，三（C 1-6烷基）甲硅烷基，COOR c或CONR d Re; Q表示杂环基，它们用作除草剂。

    1-azinyl-tetrazolinones
    9.
    发明授权
    1-azinyl-tetrazolinones 失效
    1-吖嗪基 - 四唑啉酮

    公开(公告)号：US5776858A

    公开(公告)日：1998-07-07

    申请号：US736867

    申请日：1996-10-25

    申请人： Toshio Goto ,  Seishi Ito ,  Natsuko Minegishi ,  Tatsuya Yamaoka ,  Chieko Ueno ,  Koichi Moriya ,  Fritz Maurer ,  Ryo Watanabe

    发明人： Toshio Goto ,  Seishi Ito ,  Natsuko Minegishi ,  Tatsuya Yamaoka ,  Chieko Ueno ,  Koichi Moriya ,  Fritz Maurer ,  Ryo Watanabe

    IPC分类号： C07D401/06 ,  A01N43/713 ,  A01N47/38 ,  C07D257/04 ,  C07D401/14 ,  C07D403/04 ,  C07D403/06 ,  C07D403/14 ,  A01N43/58 ,  A01N43/60 ,  A01N43/66 ,  C07D403/02

    CPC分类号： C07D403/04 ,  A01N47/38

    摘要： 1-Azinyl-tetraozolinones of the following formulae (I) and (II): ##STR1## wherein R.sup.1 and R.sup.2 are independently represent alkyl, haloalkyl, cycloalkyl, alkenyl, haloalkenyl, alkynyl or optionally substituted phenyl, or R.sup.1 and R.sup.2, together with the nitrogen atom to which they are bonded, may form a 5- or 6-membered heterocyclic ring which may optionally contain a further heteroatom, and said heterocyclic ring may optionally be benzo-condensed and/or be substituted by one or more of C.sub.1-4 alkyl(s), and R.sup.3 is a 6-membered heterocyclic aromatic group consisting of carbon atoms and 2 or 3 nitrogen atoms, which may optionally be substituted by halogen, C.sub.1-4 alkyl, C.sub.1-4 alkoxy, C.sub.1-4 alkylthio, di(C.sub.1-4 alkyl)amino or phenyl. The compounds of the formula (I) exhibit an excellent herbicidal activity and the compounds of the formula (II) are useful as starting materials in the production of the compounds of the formula (I).

    摘要翻译： 下式（I）和（II）的1-氮杂环丁烷基 - 四唑啉酮：其中R 1和R 2独立地表示烷基，卤代烷基，环烷基，烯基，卤代烯基，炔基或任意取代的 苯基或R 1和R 2与它们所键合的氮原子一起可以形成可以任选地含有另外的杂原子的5-或6-元杂环，并且所述杂环可任选地被苯并稠合和/或 被一个或多个C 1-4烷基取代，并且R 3是由碳原子和2或3个氮原子组成的6元杂环芳基，其可任选被卤素，C 1-4烷基，C 1 -4-烷氧基，C 1-4烷硫基，二（C 1-4烷基）氨基或苯基。 式（I）的化合物显示出优异的除草活性，并且式（II）的化合物可用作制备式（I）化合物的原料。