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公开(公告)号：US08129575B2
公开(公告)日：2012-03-06
申请号：US12377388
申请日：2007-08-15
IPC分类号： C07C1/00
摘要： A process is disclosed for fluid catalytic cracking of oxygenated hydrocarbon compounds such as glycerol and bio-oil.In the process the oxygenated hydrocarbon compounds are contacted with a fluid cracking catalyst material for a period of less than 3 seconds.In a preferred process a crude-oil derived material, such as VGO, is also contacted with the catalyst.
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52.发明申请公开(公告)号：US20120037486A1
公开(公告)日：2012-02-16
申请号：US13130092
申请日：2009-11-25
申请人： Paul O'Connor , Steve Yanlk , Sjoerd Daamen
发明人： Paul O'Connor , Steve Yanlk , Sjoerd Daamen
IPC分类号： C10B57/12
CPC分类号： C10L1/02 , C10B53/02 , C10B57/06 , C10G2/30 , C10G2300/1014 , C10G2300/4006 , Y02E50/14 , Y02E50/32 , Y02P30/20
摘要： A process is disclosed for the conversion of cellulosic biomass, in particular ligno-cellulosic biomass. The process comprises heating the biomass to a conversion temperature in the range of from 200 to 500° C. in the presence of a catalyst system. The catalyst system comprises a basic functionality comprising an alkali metal component and a multivalent metal component. The catalyst system optionally further comprises an acidic component.
摘要翻译： 公开了用于转化纤维素生物质，特别是木质纤维素生物质的方法。 该方法包括在催化剂体系的存在下将生物质加热至200-500℃的转化温度。 催化剂体系包含碱金属组分和多价金属组分的基本官能团。 催化剂体系任选地还包含酸性组分。
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53.发明申请公开(公告)号：US20120022307A1
公开(公告)日：2012-01-26
申请号：US12867214
申请日：2009-06-29
申请人： Steve Yanik , Paul O'Connor , Robert Bartek
发明人： Steve Yanik , Paul O'Connor , Robert Bartek
CPC分类号： C09K3/00 , C10G1/002 , C10G1/08 , C10G11/00 , C10G11/18 , C10G2300/1014 , C10G2300/1037 , C10G2300/4056 , C10G2400/02 , C10G2400/04 , C10G2400/08 , C10G2400/20 , C10G2400/28 , Y02P30/20
摘要： Preparing solid biomass particles for catalytic conversion includes agitating solid biomass particles and providing a biomass-catalyst mixture to a conventional petroleum refinery process unit. The biomass-catalyst mixture includes the solid biomass particles and a catalyst. Agitating solid biomass particles includes flowing a gas to provide a velocity to at least a portion of the solid biomass particles sufficient to reduce their sizes. Co-processing a biomass feedstock and a conventional petroleum feedstock includes liquefying at least a portion of a biomass-catalyst mixture and co-processing at least a portion of the liquefied biomass feedstock and a conventional petroleum feedstock in a conventional petroleum refinery process unit. The biomass feedstock includes a plurality of solid biomass particles and a catalyst, which is liquefied to produce a liquefied biomass feedstock.
摘要翻译： 制备用于催化转化的固体生物质颗粒包括搅拌固体生物质颗粒并向传统的炼油工艺单元提供生物质 - 催化剂混合物。 生物质 - 催化剂混合物包括固体生物质颗粒和催化剂。 搅拌固体生物质颗粒包括使气体流动以提供足以减小其尺寸的至少一部分固体生物质颗粒的速度。 共同处理生物质原料和常规石油原料包括液化生物质 - 催化剂混合物的至少一部分，并在常规的炼油工艺单元中共同处理至少一部分液化生物质原料和常规石油原料。 生物质原料包括多个固体生物质颗粒和催化剂，其被液化以产生液化生物质原料。
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公开(公告)号：US20120017492A1
公开(公告)日：2012-01-26
申请号：US12915872
申请日：2010-10-29
IPC分类号： C10L1/02
CPC分类号： C10L1/02 , C10G1/02 , C10G1/08 , C10G3/42 , C10G2300/1011 , C10G2300/1014 , C10G2300/1037 , C10G2300/301 , C10G2300/80 , C10L1/04 , C11B13/00 , C11C3/00 , Y02E50/10 , Y02E50/13 , Y02E50/30 , Y02P30/20 , Y02W30/74
摘要： A process and system for separating a light fraction, a bio-distillate fraction, and a heavy fraction from a bio-oil, and for producing a renewable distillate including at least in part the bio-distillate fraction and a stabilizing additive, is provided. The process comprises separating bio-oil into light, bio-distillate, and heavy fractions based on their boiling points. At least a portion of the bio-distillate fraction and a stabilizing additive are blended with a petroleum-derived-diesel-range stream, without any prior hydrotreatment, to thereby provide a renewable distillate composition.
摘要翻译： 提供了用于从生物油分离轻馏分，生物馏出物馏分和重馏分，以及用于生产至少部分包括生物馏分和稳定添加剂的可再生馏出物的方法和系统。 该方法包括基于其沸点将生物油分离成轻质，生物馏分和重馏分。 至少一部分生物馏出物馏分和稳定添加剂与石油衍生的柴油范围物流混合，而无需任何先前的加氢处理，从而提供可再生的馏出物组合物。
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公开(公告)号：US08057641B2
公开(公告)日：2011-11-15
申请号：US12838629
申请日：2010-07-19
申请人： Robert Bartek , Ronald Lee Cordle
发明人： Robert Bartek , Ronald Lee Cordle
IPC分类号： C10B49/20
摘要： A method and apparatus for effective pyrolysis of a biomass utilizing rapid heat transfer from a solid heat carrier or catalyst. Particularly, various embodiments of the present invention provide methods and apparatuses which incorporate progressive temperature quenching and rapid disengagement of the heat carrier material and reaction product.
摘要翻译： 一种利用从固体热载体或催化剂的快速热传递来有效地热解生物质的方法和装置。 特别地，本发明的各种实施方案提供了包含渐进式温度淬火和热载体材料和反应产物的快速脱离的方法和装置。
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公开(公告)号：US20110256615A1
公开(公告)日：2011-10-20
申请号：US13057968
申请日：2009-12-22
申请人： Michael Brady , Dennis Stamires , Paul O'Connor
发明人： Michael Brady , Dennis Stamires , Paul O'Connor
CPC分类号： D21C1/02 , C12P2201/00 , D21C3/00 , D21C11/0007 , Y02E50/16
摘要： A process is disclosed for preparing biomass particles for thermolytic or enzymatic conversion whereby the biomass particles baying a moisture content of at least 20% are subjected to flash heating. The flash heating may be preceded by one or more adsorption/desorption cycles with water or steam. A swelling aid may be added during the adsorption part of an adsorption/desorption cycle.
摘要翻译： 公开了一种用于制备用于热分解或酶促转化的生物质颗粒的方法，其中使水分含量至少为20％的生物质颗粒经受闪蒸加热。 闪蒸加热之前可以用水或蒸汽进行一次或多次吸附/解吸循环。 在吸附/解吸循环的吸附部分可以加入溶胀助剂。
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公开(公告)号：US20110114765A1
公开(公告)日：2011-05-19
申请号：US12934006
申请日：2009-11-30
申请人： Michael Brady , Robert Bartek , Dennis Stamires , Paul O'Connor
发明人： Michael Brady , Robert Bartek , Dennis Stamires , Paul O'Connor
摘要： A method is disclosed for reducing the mechanical strength of solid biomass material, in particular ligno-cellulosic biomass. The method comprises heating the solid biomass material to a temperature in the range of 105° C. to 200° C. The heat treatment, which is referred to as “toasting”, significantly reduces the mechanical energy required for reducing the particle size of the solid biomass material.The method is particularly suitable as a pretreatment step to a conversion reaction of the solid biomass material.
摘要翻译： 公开了一种降低固体生物质材料，特别是木质纤维素生物质的机械强度的方法。 该方法包括将固体生物质材料加热至105℃至200℃的温度。被称为“烘烤”的热处理显着降低了降低颗粒尺寸所需的机械能 固体生物质材料。 该方法特别适用于固体生物质材料的转化反应的预处理步骤。
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公开(公告)号：US20100293839A1
公开(公告)日：2010-11-25
申请号：US12746140
申请日：2008-12-02
申请人： Paul O'Connor
发明人： Paul O'Connor
IPC分类号： C10L1/00
摘要： A reactive distillation process is disclosed for converting aquatic biomass to a bio-oil. In the process a slurry of aquatic biomass is contacted with a particulate inorganic material. The mixture is heated to or above its boiling point. During the heating step biomass is converted to bio-oil. In a preferred embodiment water vapors emanating from the slurry are collected and condensed. The fresh water obtained may be used for irrigation, in human domestic uses, and for human consumption.
摘要翻译： 公开了将水生生物质转化为生物油的反应蒸馏方法。 在该过程中，水生生物质的浆液与颗粒状无机材料接触。 将混合物加热至或高于其沸点。 在加热阶段，生物质被转化为生物油。 在优选的实施方案中，从浆液中发出的水蒸汽被收集并冷凝。 所获得的淡水可用于灌溉，在家庭用途和人类消费。
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公开(公告)号：US20100113849A1
公开(公告)日：2010-05-06
申请号：US12612378
申请日：2009-11-04
申请人： Robert Bartek , Steve Yanik , Paul O'Connor
发明人： Robert Bartek , Steve Yanik , Paul O'Connor
CPC分类号： C10L1/04 , C10G1/08 , C10G1/083 , C10G2300/1011 , C10G2300/4006 , C10G2300/708 , Y02E50/14 , Y02P30/20
摘要： A process is disclosed including: contacting solid biomass with a first catalyst stream in a first reaction zone operated at a temperature T1 (from about 250 to about 400° C.), for conversion of a portion of the solid biomass and forming a first gaseous product stream; downwardly passing unconverted biomass to a second reaction zone for contact with a second catalyst stream charged to the second reaction zone operated at a temperature T2, for conversion to form a second gaseous product stream and a spent catalyst; burning coke off the spent catalyst in a regenerator to form a regenerated catalyst; charging a portion of the regenerated catalyst to each of the first and second reaction zones, as the first and second catalyst streams, respectively; upwardly passing the second gaseous product stream to the first reaction zone; and removing both first and second gaseous product streams from the first reaction zone.
摘要翻译： 公开了一种方法，包括：使第一催化剂流与第一反应区在温度T1（约250至约400℃）下操作，以使一部分固体生物质转化并形成第一气态 产品流; 向下通过未转化的生物质到第二反应区，以与加入在温度T2下操作的第二反应区的第二催化剂流接触，以转化以形成第二气态产物流和废催化剂; 在再生器中燃烧焦炭废催化剂以形成再生催化剂; 将一部分再生催化剂分别装入第一和第二反应区中的第一和第二反应区，作为第一和第二催化剂流; 向上通过第二气态产物流到第一反应区; 以及从所述第一反应区域除去第一和第二气态产物流。
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公开(公告)号：US09044741B2
公开(公告)日：2015-06-02
申请号：US13446926
申请日：2012-04-13
申请人： Bruce Adkins , Dennis Stamires , Robert Bartek , Michael Brady , John Hackskaylo
发明人： Bruce Adkins , Dennis Stamires , Robert Bartek , Michael Brady , John Hackskaylo
CPC分类号： B01J29/40 , B01J37/0009 , B01J37/28 , B01J2229/18 , B01J2229/42 , C10G3/49 , C10G3/57 , C10G2300/1014 , C10G2400/02 , C10G2400/04 , C10G2400/08 , C10L1/04 , C10L2200/0469 , C10L2290/02 , Y02P30/20
摘要： Catalyst compositions comprising a phosphorous-promoted ZSM-5 component and a silica-containing binder, and methods for making and using same, are disclosed. More specifically, processes for making a catalyst for biomass conversion are provided. The process includes: treating a ZSM-5 zeolite with a phosphorous-containing compound to form a phosphorous-promoted ZSM-5 component; preparing a slurry comprising the phosphorous-promoted ZSM-5 component and a silica-containing binder; and shaping the slurry into shaped bodies. Such catalysts can be used for the thermocatalytic conversion of particulate biomass to liquid products such as bio-oil, resulting in higher bio-oil yields and lower coke than conventional catalysts.
摘要翻译： 公开了包含磷促进的ZSM-5组分和含二氧化硅的粘合剂的催化剂组合物及其制备和使用方法。 更具体地，提供了用于制备用于生物质转化的催化剂的方法。 该方法包括：用含磷化合物处理ZSM-5沸石以形成磷促进的ZSM-5组分; 制备包含磷促进的ZSM-5组分和含二氧化硅的粘合剂的浆料; 并将浆料成型为成型体。 这种催化剂可用于将微生物量热生物转化为液体产物如生物油，导致比常规催化剂更高的生物油产率和较低的焦炭。
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