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公开(公告)号：US5073529A
公开(公告)日：1991-12-17
申请号：US453666
申请日：1989-12-20
IPC分类号： B01J29/90 , C10G35/095
CPC分类号： B01J29/90 , C10G35/095
摘要： A deactivated catalyst comprising a nonacidic zeolite and a Group VIII metal is regenerated by a two-step carbon burn process. The first oxidation step contacts the nonacidic zeolite catalyst with a halogen-free gaseous stream comprising oxygen and an inert gas at a first temperature sufficient to combust carbonaceous material while maintaining a substantial portion of the active Group VIII metal surface area withn the micropores of the nonacidic zeolite for a first period of time sufficient to substantially complete combustion of at least a portion the carbonaceous material at the first temperature. The second step contacts this nonacidic zeolite catalyst with a gaseous stream comprising oxygen and an inert gas at a second temperature sufficient to combust any remaining carbonaceous material for a second period of time sufficient to maintain a substantial portion of the active Group VIII metal surface area in the micropores of the nonacidic zeolite catalyst.
摘要翻译： 包含非酸性沸石和VIII族金属的失活催化剂通过两步碳燃烧方法再生。 第一氧化步骤用不含卤素的气态物流接触非酸性沸石催化剂，所述无卤素气流在足以燃烧含碳材料的第一温度下包含氧气和惰性气体，同时保持活性VIII族金属表面积的大部分与非酸性微孔 沸石第一时间段足以在第一温度下基本上完成至少一部分碳质材料的燃烧。 第二步与含有氧和惰性气体的气态物流接触，该气流在足以将任何剩余的含碳材料燃烧足以将活性VIII族金属表面积的大部分维持在第二时间的第二温度 非酸性沸石催化剂的微孔。
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公开(公告)号：US5028312A
公开(公告)日：1991-07-02
申请号：US359138
申请日：1989-05-31
IPC分类号： C07C5/41 , C10G35/095
CPC分类号： C10G35/095 , C07C5/417
摘要： A method is disclosed for reforming hydrocarbons, particularly C.sub.6 -C.sub.10 hydrocarbons, to aromatics, by passing the hydrocarbons over a dehydrocyclization catalyst at dehydrocyclization conditions. The catalyst comprises a non-acidic large pore zeolite having a Group VIII metal and an alkaline earth metal, said alkaline earth metal having been impregnated onto the zeolite by contacting the zeolite with an alkaline earth metal solution of a concentration sufficient to result in the zeolite having an alkaline earth metal content of less than about 2% by weight of the zeolite.
摘要翻译： 公开了一种通过使烃在脱氢环化条件下通过脱氢环化催化剂将烃，特别是C 6 -C 10烃重整成芳族化合物的方法。 催化剂包括具有VIII族金属和碱土金属的非酸性大孔沸石，所述碱土金属已经通过使沸石与足以导致沸石的浓度的碱土金属溶液接触而浸渍到沸石上 其碱土金属含量小于沸石重量的约2％。
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3.发明授权Catalyst and process for high selectivity reforming with Pt/Re on Ba-K-L zeolite 失效Pt / Re对Ba-K-L沸石进行高选择性重整的催化剂和方法
公开(公告)号：US4954245A
公开(公告)日：1990-09-04
申请号：US287397
申请日：1988-12-20
申请人： Jeffrey T. Miller , Victor K. Shum
发明人： Jeffrey T. Miller , Victor K. Shum
IPC分类号： B01J29/60 , C10G35/095
CPC分类号： B01J29/60 , C10G35/095 , B01J2229/26 , B01J2229/42
摘要： This invention comprises a reforming catalyst and process with an unsulfided catalyst comprising Zeolite L, in which the cationic sites have been exchanged to contain potassium or barium or both; a Group VIII noble metal and rhenium, where the ratio of noble metal to rhenium is from about 0.1:1 to about 10:0. This catalyst gives improved selectivity toward aromatics formation and has improved sulfur tolerance compared to other L zeolite reforming catalysts.
摘要翻译： 本发明包括重整催化剂和具有包含沸石L的未硫化催化剂的方法，其中阳离子位点已经被交换以含有钾或钡或两者; 第VIII族贵金属和铼，其中贵金属与铼的比例为约0.1:1至约10:0。 该催化剂提高了芳烃形成的选择性，并且与其它L沸石重整催化剂相比具有改善的耐硫化性。
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4.发明授权Catalyst and process for high selectivity reforming with PT/RE on BA-K-L zeolite 失效在BA-K-L沸石上用PT / RE进行高选择性重整的催化剂和方法
公开(公告)号：US5066628A
公开(公告)日：1991-11-19
申请号：US528038
申请日：1990-05-23
申请人： Jeffrey T. Miller , Victor K. Shum
发明人： Jeffrey T. Miller , Victor K. Shum
IPC分类号： B01J29/60 , C10G35/095
CPC分类号： C10G35/095 , B01J29/60 , B01J2229/26 , B01J2229/42
摘要： This invention comprises a reforming catalyst and process with an unsulfided catalyst comprising Zeolite L, in which the cationic sites have been exchanged to contain potassium or barium or both; a Group VIII noble metal and rhenium, where the ratio of noble metal to rhenium is from about 0.1:1 to about 10:0. This catalyst gives improved selectivity toward aromatics formation and has improved sulfur tolerance compared to other L zeolite reforming catalysts.
摘要翻译： 本发明包括重整催化剂和具有包含沸石L的未硫化催化剂的方法，其中阳离子位点已经被交换以含有钾或钡或两者; 第VIII族贵金属和铼，其中贵金属与铼的比例为约0.1:1至约10:0。 该催化剂提高了芳烃形成的选择性，并且与其它L沸石重整催化剂相比具有改善的耐硫化性。
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公开(公告)号：US5196634A
公开(公告)日：1993-03-23
申请号：US775209
申请日：1991-10-11
申请人： Don M. Washecheck , Mark K. Barr , George A. Huff, Jr. , Mark P. Kaminsky , Mark S. Kleefisch , Victor K. Shum
发明人： Don M. Washecheck , Mark K. Barr , George A. Huff, Jr. , Mark P. Kaminsky , Mark S. Kleefisch , Victor K. Shum
IPC分类号： C07C2/84
CPC分类号： C07C2/84 , C07C2521/02 , Y10S585/943
摘要： A contact material composition containing an intimately mixed, mixed oxide of at least one cationic species of a naturally occurring Group IIIB element, at least one cationic species of a Group IIA metal of magnesium, calcium, strontium, and barium and a cationic species of aluminum, as well as methods for hydrocarbon conversion using such contact material compositions are provided.
摘要翻译： 包含天然存在的IIIB族元素的至少一种阳离子物质，镁，钙，锶和钡的IIA族金属的至少一种阳离子物质和阳离子物质的铝的接触材料组合物 ，以及使用这种接触材料组合物的烃转化方法。
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公开(公告)号：US4808763A
公开(公告)日：1989-02-28
申请号：US82031
申请日：1987-08-05
申请人： Victor K. Shum
发明人： Victor K. Shum
CPC分类号： B01J29/87 , C07C2/00 , B01J2229/20 , B01J2229/42 , C07C2521/04 , C07C2521/08 , C07C2521/12 , C07C2523/42 , C07C2529/87
摘要： The present invention relates to a process for producing aromatic compounds from a hydrocarbon gas containing paraffinic hydrocarbons under conversion conditions in the presence of a catalyst comprising a gallosilicate molecular sieve and a platinum metal component.
摘要翻译： 本发明涉及在含有硅酸镓分子筛和铂金属组分的催化剂存在下，在转化条件下由含有链烷烃的烃气制备芳族化合物的方法。
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公开(公告)号：US4971680A
公开(公告)日：1990-11-20
申请号：US287399
申请日：1988-12-20
IPC分类号： B01J23/888 , B01J29/16 , C10G47/16
CPC分类号： B01J23/888 , B01J29/166 , C10G47/16
摘要： A hydrocarbon conversion process is disclosed involving the hydrocracking of a catalytic cycle oil in the presence of a catalyst having a nickel component, a tungsten component, and a support component containing a crystalline molecular sieve material present in an amount ranging from about 25 to about 60 wt. % based on the weight of the support component wherein at least about 1 to about 80 wt. % of the sieve material is a gallosilicate, based on the total weight of the sieve component.
摘要翻译： 公开了一种烃转化方法，其涉及在具有镍组分，钨组分和含有结晶分子筛材料的载体组分的催化剂存在下催化循环油的加氢裂化，所述结晶分子筛材料的存在量为约25至约60 重量 基于支持组分的重量，其中至少约1至约80重量％ 基于筛组分的总重量，筛材料的百分比是硅酸盐。
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公开(公告)号：US4962266A
公开(公告)日：1990-10-09
申请号：US401978
申请日：1989-08-31
申请人： Victor K. Shum
发明人： Victor K. Shum
CPC分类号： C07C5/373 , C07C5/3337 , C07C2523/42 , C07C2529/04
摘要： The invention relates to a process for the conversion of linear alkanes such as n-butane to dehydrogenated and isomerized products in the presence of a catalyst comprising a platinum component and a zincosilicate component.
摘要翻译： 本发明涉及在包含铂组分和硅酸锌组分的催化剂存在下将直链烷烃如正丁烷转化为脱氢和异构化产物的方法。
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公开(公告)号：US4950828A
公开(公告)日：1990-08-21
申请号：US375139
申请日：1989-06-30
申请人： Victor K. Shum
发明人： Victor K. Shum
CPC分类号： B01J29/86 , C07C2/00 , B01J2229/20 , B01J2229/42 , C07C2523/08 , C07C2523/42 , C07C2529/86
摘要： The present invention relates to a process for producing aromatic compounds from a hydrocarbon gas containing C.sub.3 through C.sub.5 paraffinic hydrocarbons under conversion conditions in the presence of a catalyst comprising a borosilicate molecular sieve, a platinum metal component and a gallium metal component.
摘要翻译： 本发明涉及在包含硼硅酸盐分子筛，铂金属组分和镓金属组分的催化剂存在下，在转化条件下由含有C 3至C 5链烷烃的烃气制备芳族化合物的方法。
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公开(公告)号：US4946813A
公开(公告)日：1990-08-07
申请号：US233453
申请日：1988-08-18
申请人： Victor K. Shum
发明人： Victor K. Shum
CPC分类号： B01J29/87 , C07C2/00 , B01J2229/20 , B01J2229/42 , C07C2523/42 , C07C2523/52 , C07C2523/72 , C07C2529/87
摘要： The present invention relates to a process for producing aromatic compounds from hydrocarbon gas containing paraffinic hydrocarbons under conversion conditions in the presence of a catalyst comprising a gallosilicate molecular sieve, a Group VIII metal component, and a Group IB metal component.
摘要翻译： 本发明涉及在含有聚硅酸盐分子筛，第Ⅷ族金属组分和IB族金属组分的催化剂存在下，在转化条件下含有链烷烃的烃气体中制备芳族化合物的方法。
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