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    METHOD FOR PRODUCING PROPENE FROM PROPANE
    1.
    发明申请
    METHOD FOR PRODUCING PROPENE FROM PROPANE 审中-公开
    从丙烷生产丙烯的方法

    公开(公告)号：US20090312591A1

    公开(公告)日：2009-12-17

    申请号：US12294748

    申请日：2007-03-13

    申请人： Markus Schubert ,  Ulrich Müller ,  Christoph Kiener ,  Friedhalm Teich ,  Sven Crone ,  Falk Simon ,  Jörg Pastre

    发明人： Markus Schubert ,  Ulrich Müller ,  Christoph Kiener ,  Friedhalm Teich ,  Sven Crone ,  Falk Simon ,  Jörg Pastre

    IPC分类号： C07C5/327

    CPC分类号： C07C5/333 ,  C07C7/12 ,  C07C7/13 ,  C07C11/06

    摘要： The present invention relates to processes for preparing propene from propane, comprising the steps: A) a feed gas stream a comprising propane is provided; B) the feed gas stream a comprising propane, if appropriate steam and if appropriate and an oxygenous gas stream are fed into a dehydrogenation zone and propane is subjected to a dehydrogenation to propene to obtain a product gas stream b comprising propane, propene, methane, ethane, ethene, hydrogen, if appropriate carbon monoxide, carbon dioxide, steam and oxygen; C) the product gas stream b is cooled, if appropriate compressed and steam is removed by condensation to obtain a steam-depleted product gas stream c; D) the product gas stream c is contacted with a selective adsorbent which adsorbs propene selectively under the selected adsorption conditions to obtain a propene-laden adsorbent and a propene-depleted gas stream d2 comprising propane, methane, ethane, ethene and hydrogen, carbon monoxide and carbon dioxide; E) a propene-comprising gas stream e1 is released from the propane-laden adsorbent by pressure reduction and/or heating of the adsorbent.

    摘要翻译： 本发明涉及从丙烷制备丙烯的方法，包括以下步骤：A）提供包含丙烷的原料气流a; B）包含丙烷的进料气流a（如果合适的话，蒸汽和适当的话）和含氧气流被送入脱氢区，丙烷经脱氢至丙烯以获得包含丙烷，丙烯，甲烷， 乙烷，乙烯，氢气，如果适用，一氧化碳，二氧化碳，蒸气和氧气; C）产物气流b被冷却，如果合适的话压缩并通过冷凝除去蒸汽，得到蒸汽消耗产物气流c; D）产物气流c与在选择的吸附条件下选择性吸附丙烯的选择性吸附剂接触以获得含有丙烯的吸附剂和包含丙烷，甲烷，乙烷，乙烯和氢气的一种贫含丙烯的气流d2，一氧化碳 和二氧化碳; E）通过吸附剂的减压和/或加热将含丙烯气流e1从载有丙烷的吸附剂中释放。

    Method for the separation of carbon dioxide using a porous metal-organic framework material
    4.
    发明授权
    Method for the separation of carbon dioxide using a porous metal-organic framework material 失效
    使用多孔金属 - 有机骨架材料分离二氧化碳的方法

    公开(公告)号：US07556673B2

    公开(公告)日：2009-07-07

    申请号：US11563101

    申请日：2006-11-24

    申请人： Markus Schubert ,  Ulrich Müller ,  Christoph Kiener

    发明人： Markus Schubert ,  Ulrich Müller ,  Christoph Kiener

    IPC分类号： B01D53/04

    CPC分类号： B01D53/02 ,  B01D2253/204 ,  B01D2257/504 ,  B01J20/226 ,  C01B32/50 ,  Y02C10/08 ,  Y02P20/152

    摘要： The present invention relates to a method for the separation of carbon dioxide from a gas mixture containing carbon dioxide comprising the steps of (a) contacting the gas mixture with at least one sorbent comprising a porous metal-organic framework material, the framework material taking up the carbon dioxide from the gas mixture and comprising at least one at least bidentate organic compound coordinately bound to at least one metal ion, wherein the at least bidentate organic compound comprises at least one substituted or unsubstituted amino group and wherein the at last one metal ion is an ion selected from the group of metals consisting of magnesium, calcium, strontium, barium, aluminium, gallium, indium, scandium, yttrium, titanium, zirconium, iron, copper and lanthanoids; and (b) desorbing the carbon dioxide.

    摘要翻译： 本发明涉及一种从含有二氧化碳的气体混合物中分离二氧化碳的方法，包括以下步骤：（a）使气体混合物与至少一种包含多孔金属 - 有机骨架材料的吸附剂接触，骨架材料占据 来自气体混合物的二氧化碳并且包含与至少一种金属离子配位结合的至少一种至少二齿有机化合物，其中至少二齿有机化合物包含至少一个取代或未取代的氨基，并且其中最后一个金属离子 是选自由镁，钙，锶，钡，铝，镓，铟，钪，钇，钛，锆，铁，铜和镧系元素组成的金属组的离子; 和（b）解吸二氧化碳。

    Process for preparing porous metal organic frameworks
    6.
    发明授权
    Process for preparing porous metal organic frameworks 有权
    制备多孔金属有机骨架的方法

    公开(公告)号：US07879221B2

    公开(公告)日：2011-02-01

    申请号：US12300902

    申请日：2007-05-11

    申请人： Hermann Pütter ,  Markus Schubert ,  Ingo Richter ,  Ulrich Müller ,  Natalia Trukhan

    发明人： Hermann Pütter ,  Markus Schubert ,  Ingo Richter ,  Ulrich Müller ,  Natalia Trukhan

    IPC分类号： C25B3/12 ,  C07F15/00 ,  C07F3/00

    CPC分类号： C25B3/12

    摘要： The present invention relates to a process for preparing a porous metal organic framework comprising at least two organic compounds coordinated to at least one metal ion, which comprises the steps (a) oxidation of at least one anode comprising the metal corresponding to at least one metal ion in a reaction medium in the presence of at least one first organic compound which is an optionally substituted monocyclic, bicyclic or polycyclic saturated or unsaturated hydrocarbon in which at least two ring carbons have been replaced by heteroatoms selected from the group consisting of N, O and S to form a reaction intermediate comprising the at least one metal ion and the first organic compound; and (b) reaction of the reaction intermediate at a prescribed temperature with at least one second organic compound which coordinates to the at least one metal ion, with the second organic compound being derived from a dicarboxylic, tricarboxylic or tetracarboxylic acid.

    摘要翻译： 本发明涉及一种制备多孔金属有机骨架的方法，所述多孔金属有机骨架包括与至少一种金属离子配位的至少两种有机化合物，其包括以下步骤：（a）至少一个阳极的氧化，所述至少一个阳极包含对应于至少一种金属 在至少一种第一有机化合物存在下的反应介质中，所述第一有机化合物是任选取代的单环，双环或多环饱和或不饱和烃，其中至少两个环碳已经被选自N，O 和S形成包含所述至少一种金属离子和所述第一有机化合物的反应中间体; 和（b）将反应中间体在规定温度下与至少一种与至少一种金属离子配位的第二有机化合物反应，第二有机化合物衍生自二羧酸，三羧酸或四羧酸。

    METAL-ORGANIC ZIRCONIUM-BASED FRAMEWORK MATERIALS
    7.
    发明申请
    METAL-ORGANIC ZIRCONIUM-BASED FRAMEWORK MATERIALS 审中-公开
    金属有机基于ZIRCONIUM的框架材料

    公开(公告)号：US20090281341A1

    公开(公告)日：2009-11-12

    申请号：US12297294

    申请日：2007-04-17

    申请人： Markus Schubert ,  Ulrich Müller ,  Stefan Marx

    发明人： Markus Schubert ,  Ulrich Müller ,  Stefan Marx

    IPC分类号： C07F7/00

    CPC分类号： C07C51/412 ,  C07C29/70 ,  C07F7/003 ,  C07C63/28 ,  C07C63/14

    摘要： The present invention relates to a porous metal-organic framework material comprising at least one at least bidentate organic compound which is bound to at least one metal ion by coordination, the at least one metal ion being zirconium, and the at least one at least bidentate organic compound being derived from a dicarboxylic, tricarboxylic or tetracarboxylic acid. In addition, the invention relates to methods for production thereof and also use thereof.

    摘要翻译： 多孔金属 - 有机骨架材料本发明涉及多孔金属 - 有机骨架材料，其包含至少一种至少二齿有机化合物，其通过配位与至少一种金属离子结合，所述至少一种金属离子是锆，以及所述至少一种至少二齿 有机化合物衍生自二羧酸，三羧酸或四羧酸。 此外，本发明涉及其生产方法及其用途。

    POROUS METAL ORGANIC FRAMEWORK BASED ON PYRROLES AND PYRIDINONES
    8.
    发明申请
    POROUS METAL ORGANIC FRAMEWORK BASED ON PYRROLES AND PYRIDINONES 审中-公开
    基于PYRROLES和PYRIDINONES的多孔金属有机框架

    公开(公告)号：US20090183996A1

    公开(公告)日：2009-07-23

    申请号：US12300942

    申请日：2007-05-11

    申请人： Ingo Richter ,  Markus Schubert ,  Ulrich Müller

    发明人： Ingo Richter ,  Markus Schubert ,  Ulrich Müller

    IPC分类号： C25B3/02

    CPC分类号： C07D233/54 ,  B01J20/226 ,  C07D235/22 ,  C25B3/12

    摘要： Processes comprising: (i) providing an anode comprising zinc; and (ii) oxidizing the anode in a reaction medium in the presence of at least one organic compound to form a porous metal organic framework comprising the least one organic compound coordinated to at least one zinc ion; wherein the at least one organic compound comprises a ring system selected from the group consisting of compounds corresponding to the following structures wherein the ring system optionally bears one or more substituents selected independently from the group consisting of halogens, C1-6-alkyls, phenyl, NH2, NH(C1-6-alkyls), N(C1-6-alkyls)2, OH, O-phenyl and O—C1-6-alkyls, and wherein each C1-6-alkyl and phenyl substituent may independently and optionally bear one or more substituents selected independently from the group consisting of halogens, NH2, NH(C1-6-alkyls), N(C1-6-alkyls)2, OH, O-phenyl and O—C1-6-alkyls.

    摘要翻译： 方法包括：（i）提供包含锌的阳极; 和（ii）在至少一种有机化合物的存在下在反应介质中氧化阳极以形成包含与至少一种锌离子配位的至少一种有机化合物的多孔金属有机骨架; 其中所述至少一种有机化合物包括选自对应于以下结构的化合物的环系统，其中所述环系统任选地带有一个或多个独立地选自卤素，C 1-6 - 烷基，苯基， NH 2，NH（C 1-6 - 烷基），N（C 1-6 - 烷基）2，OH，O-苯基和O-C 1-6 - 烷基，其中每个C 1-6 - 烷基和苯基取代基可以独立地和任选地 含有一个或多个独立地选自卤素，NH 2，NH（C 1-6 - 烷基），N（C 1-6 - 烷基）2，OH，O-苯基和O-C 1-6 - 烷基的取代基。

    PROCESS FOR PREPARING POROUS METAL ORGANIC FRAMEWORKS
    10.
    发明申请
    PROCESS FOR PREPARING POROUS METAL ORGANIC FRAMEWORKS 有权
    制备多孔金属有机框架的方法

    公开(公告)号：US20090171107A1

    公开(公告)日：2009-07-02

    申请号：US12300902

    申请日：2007-05-11

    申请人： Hermann Pütter ,  Markus Schubert ,  Ingo Richter ,  Ulrich Müller ,  Natalia Trukhan

    发明人： Hermann Pütter ,  Markus Schubert ,  Ingo Richter ,  Ulrich Müller ,  Natalia Trukhan

    IPC分类号： C07F1/08

    CPC分类号： C25B3/12

    摘要： The present invention relates to a process for preparing a porous metal organic framework comprising at least two organic compounds coordinated to at least one metal ion, which comprises the steps (a) oxidation of at least one anode comprising the metal corresponding to at least one metal ion in a reaction medium in the presence of at least one first organic compound which is an optionally substituted monocyclic, bicyclic or polycyclic saturated or unsaturated hydrocarbon in which at least two ring carbons have been replaced by heteroatoms selected from the group consisting of N, O and S to form a reaction intermediate comprising the at least one metal ion and the first organic compound; and (b) reaction of the reaction intermediate at a prescribed temperature with at least one second organic compound which coordinates to the at least one metal ion, with the second organic compound being derived from a dicarboxylic, tricarboxylic or tetracarboxylic acid.

    摘要翻译： 本发明涉及一种制备多孔金属有机骨架的方法，所述多孔金属有机骨架包括与至少一种金属离子配位的至少两种有机化合物，其包括以下步骤：（a）至少一个阳极的氧化，所述至少一个阳极包含对应于至少一种金属 在至少一种第一有机化合物存在下的反应介质中，所述第一有机化合物是任选取代的单环，双环或多环饱和或不饱和烃，其中至少两个环碳已经被选自N，O 和S形成包含所述至少一种金属离子和所述第一有机化合物的反应中间体; 和（b）将反应中间体在规定温度下与至少一种与至少一种金属离子配位的第二有机化合物反应，第二有机化合物衍生自二羧酸，三羧酸或四羧酸。