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1.发明申请公开(公告)号：US20140134096A1
公开(公告)日：2014-05-15
申请号：US14115831
申请日：2012-05-07
发明人： Fabio Angelini , Lucia Barbato
CPC分类号： C01B17/0495 , B01D53/8612 , B01D2251/102 , B01D2256/16 , B01J8/00 , C01B3/02 , C01B3/04 , C01B17/0404 , C01B17/0408 , C01B17/0426 , Y02E60/364 , Y02P20/129
摘要： Disclosed is a process for the concurrent production of hydrogen and sulphur from a H2S-containing gas stream, with reduced, and preferably zero, emissions. The method comprises the catalytic oxidative cracking of H2S so as to form H2 and S2. Preferably, the oxidation is conducted using oxygen-enriched air, preferably pure oxygen. The process is conducted in a reaction chamber comprising a bifunctional catalyst material, so as to favor both the partial oxidation of H2S and the dissociation thereof.
摘要翻译： 公开了一种从含H 2 S的气流同时生产氢和硫的方法，具有减少的，优选为零的排放。 该方法包括H2S的催化氧化裂化，形成H2和S2。 优选地，使用富氧空气，优选纯氧进行氧化。 该方法在包含双官能催化剂材料的反应室中进行，以有利于H2S的部分氧化和其解离。
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公开(公告)号：US10654719B2
公开(公告)日：2020-05-19
申请号：US14757761
申请日：2015-12-23
发明人： Lucio Molinari , Fabio Angelini , Lucia Barbato
摘要： Disclosed is a process for the concurrent production of hydrogen and sulphur from a H2S-containing gas stream, with zero emissions. The method comprises the thermal oxidative cracking of H2S so as to form H2 and S2. Preferably, the oxidation is conducted using oxygen-enriched air, preferably pure oxygen. The ratio H2S/O2 in the feedstock is higher than 2:1, preferably in the range of 3:1-5:1.
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3.发明授权公开(公告)号：US10046967B2
公开(公告)日：2018-08-14
申请号：US14441162
申请日：2013-11-08
发明人： Michele Colozzi , Lucia Barbato , Fabio Angelini , Emma Palo , Vincenzo Palma , Vincenzo Vaiano
IPC分类号： C01B3/04 , B01J27/051 , B01J21/04
摘要： Disclosed is a method for the production of hydrogen from a H2S-containing gas stream also containing ammonia, comprising subjecting both gas stream to catalytic oxidative cracking of both the H2S and the NH3, so as to form H2, S2 and N2. In this method, preferably, an additional amount of oxygen is added as compared to the amount used for H2S catalytic oxidative cracking. Also, preferably, the contact time of the gas stream with the catalyst is increased. The catalyst preferably is provided as a single bed, and then preferably comprises iron and molybdenum supported by a carrier comprising aluminum. The preferred carrier is alumina. The iron and molybdenum preferably are in the form of sulfides.
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4.发明授权Catalyst for a sulphur recovery process with concurrent hydrogen production, method of making thereof and the sulphur recovery process with concurrent hydrogen production using the catalyst 有权用于同时进行氢气生产的硫回收方法的催化剂，其制备方法和使用催化剂的氢气同时进行的硫回收方法公开(公告)号：US09573118B2
公开(公告)日：2017-02-21
申请号：US14441155
申请日：2013-11-08
发明人： Michele Colozzi , Lucia Barbato , Fabio Angelini , Emma Palo , Vincenzo Palma , Vincenzo Vaiano
IPC分类号： B01J27/051 , B01J35/08 , B01J37/08 , C01B3/04 , B01J37/20 , B01J37/02 , B01J23/881 , C01B17/04
CPC分类号： B01J27/0515 , B01J23/881 , B01J35/08 , B01J37/0201 , B01J37/0207 , B01J37/0215 , B01J37/08 , B01J37/20 , C01B3/04 , C01B17/046 , C01B17/0465 , C01B17/0495 , Y02E60/364
摘要： Disclosed is a catalyst suitable for the catalytic oxidative cracking of a H2S-containing gas stream, particularly in the event that the stream also contains methane and/or ammonia. The catalyst comprises iron and molybdenum supported by a carrier comprising aluminum. The carrier preferably is alumina. The iron and molybdenum preferably are in the form of sulphides. Also disclosed is a method for the production of hydrogen from a H2S-containing gas stream, comprising subjecting the gas stream to catalytic oxidative cracking so as to form H2 and S2, using a catalyst in accordance with any one of the preceding claims.
摘要翻译： 公开了一种适用于含H2S的气流的催化氧化裂解的催化剂，特别是在流还含有甲烷和/或氨的情况下。 催化剂包括由包含铝的载体负载的铁和钼。 载体优选为氧化铝。 铁和钼优选为硫化物的形式。 还公开了一种用于从含H 2 S的气流生产氢的方法，包括使用根据前述权利要求中任一项的催化剂使气流进行催化氧化裂化以形成H 2和S 2。
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5.发明申请公开(公告)号：US20150283537A1
公开(公告)日：2015-10-08
申请号：US14441155
申请日：2013-11-08
发明人： Michele Colozzi , Lucia Barbato , Fabio Angelini , Emma Palo , Vincenzo Palma , Vincenzo Vaiano
CPC分类号： B01J27/0515 , B01J23/881 , B01J35/08 , B01J37/0201 , B01J37/0207 , B01J37/0215 , B01J37/08 , B01J37/20 , C01B3/04 , C01B17/046 , C01B17/0465 , C01B17/0495 , Y02E60/364
摘要： Disclosed is a catalyst suitable for the catalytic oxidative cracking of a H2S-containing gas stream, particularly in the event that the stream also contains methane and/or ammonia. The catalyst comprises iron and molybdenum supported by a carrier comprising aluminium. The carrier preferably is alumina. The iron and molybdenum preferably are in the form of sulphides. Also disclosed is a method for the production of hydrogen from a H2S-containing gas stream, comprising subjecting the gas stream to catalytic oxidative cracking so as to form H2 and S2, using a catalyst in accordance with any one of the preceding claims.
摘要翻译： 公开了一种适用于含H2S的气流的催化氧化裂解的催化剂，特别是在流还含有甲烷和/或氨的情况下。 催化剂包括由包含铝的载体负载的铁和钼。 载体优选为氧化铝。 铁和钼优选为硫化物的形式。 还公开了一种用于从含H 2 S的气流生产氢的方法，包括使用根据前述权利要求中任一项的催化剂使气流进行催化氧化裂化以形成H 2和S 2。
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公开(公告)号：US09981253B2
公开(公告)日：2018-05-29
申请号：US15395093
申请日：2016-12-30
发明人： Michele Colozzi , Lucia Barbato , Fabio Angelini , Emma Palo , Vincenzo Palma , Vincenzo Vaiano
CPC分类号： B01J27/0515 , B01J23/881 , B01J35/08 , B01J37/0201 , B01J37/0207 , B01J37/0215 , B01J37/08 , B01J37/20 , C01B3/04 , C01B17/046 , C01B17/0465 , C01B17/0495 , Y02E60/364
摘要： Disclosed is a catalyst suitable for the catalytic oxidative cracking of a H2S-containing gas stream, particularly in the event that the stream also contains methane and/or ammonia. The catalyst comprises iron and molybdenum supported by a carrier comprising aluminum. The carrier preferably is alumina. The iron and molybdenum preferably are in the form of sulphides. Also disclosed is a method for the production of hydrogen from a H2S-containing gas stream, comprising subjecting the gas stream to catalytic oxidative cracking so as to form H2 and S2, using a catalyst in accordance with any one of the preceding claims.
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7.发明申请公开(公告)号：US20160122184A1
公开(公告)日：2016-05-05
申请号：US14757761
申请日：2015-12-23
发明人： Lucio Molinari , Fabio Angelini , Lucia Barbato
CPC分类号： C01B3/065 , B01D53/8612 , B01D2251/102 , B01D2256/16 , B01J19/24 , B01J19/245 , B01J2219/0015 , B01J2219/00157 , B01J2219/24 , C01B3/02 , C01B3/04 , C01B17/0413 , C01B17/0495 , C01B2203/0255 , C01B2203/06 , Y02E60/364 , Y02P20/129
摘要： Disclosed is a process for the concurrent production of hydrogen and sulphur from a H2S-containing gas stream, with zero emissions. The method comprises the thermal oxidative cracking of H2S so as to form H2 and S2. Preferably, the oxidation is conducted using oxygen-enriched air, preferably pure oxygen. The ratio H2S/O2 in the feedstock is higher than 2:1, preferably in the range of 3:1-5:1.
摘要翻译： 公开了一种从含H2S的气流同时生产氢和硫的方法，零排放。 该方法包括H2S的热氧化裂化，形成H2和S2。 优选地，使用富氧空气，优选纯氧进行氧化。 原料中H 2 S / O 2的比例高于2:1，优选在3：1-5：1的范围内。
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