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公开(公告)号：US06319960B1
公开(公告)日：2001-11-20
申请号：US07118619
申请日：1987-11-06
IPC分类号： C07C2706
CPC分类号： B01J37/0232 , B01J23/75 , B01J23/83 , B01J23/8896 , B01J23/8913 , C07C1/0435 , C07C1/0445 , C07C2521/06 , C07C2523/10 , C07C2523/12 , C07C2523/36 , C07C2523/46 , C07C2523/75 , C07C2523/83 , C07C2523/889
摘要： A method for hydrocarbon synthesis reactions from carbon monoxide and hydrogen using a catalyst pellet which includes a solid core and a coated layer of porous support impregnated with a catalyst which optimizes the CO conversion.
摘要翻译： 一种使用催化剂颗粒从一氧化碳和氢气中进行碳氢化合物反应的方法，所述催化剂颗粒包括固体芯和浸渍有优化CO转化率的催化剂的多孔载体的涂层。
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2.发明授权Cobalt-titania catalysts, process utilizing these catalysts for the preparation of hydrocarbons from synthesis gas, and process for the preparation of said catalysts 失效钴 - 二氧化钛催化剂，利用这些催化剂从合成气中制备烃的方法，以及制备所述催化剂的方法
公开(公告)号：US4962078A
公开(公告)日：1990-10-09
申请号：US252215
申请日：1988-10-03
CPC分类号： B01J37/0232 , B01J23/75 , B01J23/83 , B01J23/8896 , B01J23/8913 , C07C1/0435 , C07C1/0445 , C07C2521/06 , C07C2523/10 , C07C2523/12 , C07C2523/36 , C07C2523/46 , C07C2523/75 , C07C2523/83 , C07C2523/889
摘要： A supported particulate cobalt catalyst is formed by dispersing cobalt, alone or with a metal promoter, particularly rhenium, as a thin catalytically active film upon a particulate titania or titania-containing support, especially one wherein the rutile:anatase ratio of the support is at least about 3:2. This catalyst can be used to convert an admixture of carbon monoxide and hydrogen to a distillate fuel constituted principally of an admixture of linear paraffins and olefins, particularly a C.sub.10+ distillate, at high productivity, with low methane selectivity. A process is also disclosed for the preparation of these catalysts.
摘要翻译： 通过将单独或与金属促进剂，特别是铼作为薄催化活性膜分散在颗粒二氧化钛或二氧化钛载体上，特别是其中载体的金红石：锐钛矿比在 至少约3：2。 该催化剂可用于将一氧化碳和氢气的混合物转化为主要由线性链烷烃和烯烃，特别是C10 +馏出物的混合物组成的馏出物燃料，其生产率高，甲烷选择性低。 还公开了制备这些催化剂的方法。
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3.发明授权
公开(公告)号：US5545674A
公开(公告)日：1996-08-13
申请号：US377293
申请日：1995-01-24
CPC分类号： B01J37/0221 , B01J23/75 , B01J23/83 , B01J23/8896 , B01J23/8913 , B01J37/0232 , C07C1/0435 , C07C1/0445 , B01J35/008 , C07C2521/06 , C07C2523/10 , C07C2523/12 , C07C2523/36 , C07C2523/46 , C07C2523/75 , C07C2523/83 , C07C2523/889
摘要： A supported particulate cobalt catalyst is formed by dispersing cobalt, alone or with a metal promoter, particularly rhenium, as a thin catalytically active film upon a particulate support, especially a silica or titania support. This catalyst can be used to convert an admixture of carbon monoxide and hydrogen to a distillate fuel constituted principally of an admixture of linear paraffins and olefins, particularly a C.sub.10+ distillate, at high productivity, with low methane selectivity. A process is also disclosed for the preparation of these catalysts.
摘要翻译： 通过将单独或与金属促进剂，特别是铼作为薄催化活性的膜分散在颗粒载体上，特别是二氧化硅或二氧化钛载体上来形成负载的颗粒状钴催化剂。 该催化剂可用于将一氧化碳和氢气的混合物转化为主要由线性链烷烃和烯烃，特别是C10 +馏出物的混合物组成的馏出物燃料，其生产率高，甲烷选择性低。 还公开了制备这些催化剂的方法。
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4.再颁专利公开(公告)号：USRE37406E1
公开(公告)日：2001-10-09
申请号：US09133422
申请日：1998-08-13
IPC分类号： C07C2706
CPC分类号： B01J37/0221 , B01J23/75 , B01J23/83 , B01J23/8896 , B01J23/8913 , B01J35/008 , B01J37/0232 , C07C1/0435 , C07C1/0445 , C07C2521/06 , C07C2523/10 , C07C2523/12 , C07C2523/36 , C07C2523/46 , C07C2523/75 , C07C2523/83 , C07C2523/889
摘要： A supported particulate cobalt catalyst is formed by dispersing cobalt, alone or with a metal promoter, particularly rhenium, as a thin catalytically active film upon a particulate support, especially a silica or titania support. This catalyst can be used to convert an admixture of carbon monoxide and hydrogen to a distillate fuel constituted principally of an admixture of linear paraffins and olefins, particularly a C10+ distillate, at high productivity, with low methane selectivity. A process is also disclosed for the preparation of these catalysts.
摘要翻译： 通过将单独或与金属促进剂，特别是铼作为薄催化活性的膜分散在颗粒载体上，特别是二氧化硅或二氧化钛载体上来形成负载的颗粒状钴催化剂。 该催化剂可用于将一氧化碳和氢气的混合物转化为主要由线性链烷烃和烯烃，特别是C10 +馏出物的混合物组成的馏出物燃料，其生产率高，甲烷选择性低。 还公开了制备这些催化剂的方法。
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5.发明授权Cobalt-titania catalysts, process utilizing these catalysts for the preparation of hydrocarbons from synthesis gas, and process for the preparation of said catalysts (C-2448) 失效钴 - 二氧化钛催化剂，利用这些催化剂从合成气制备烃的方法，以及制备所述催化剂的方法（C-2448）
公开(公告)号：US5128377A
公开(公告)日：1992-07-07
申请号：US513372
申请日：1990-04-23
CPC分类号： B01J23/8913 , B01J23/75 , B01J23/83 , B01J23/8896 , B01J37/0232 , C07C1/0435 , C07C1/0445 , C07C2521/06 , C07C2523/10 , C07C2523/12 , C07C2523/36 , C07C2523/46 , C07C2523/75 , C07C2523/83 , C07C2523/889
摘要： A supported particulate cobalt catalyst is formed by dispersing cobalt, alone or with a metal promoter, particularly rhenium, as a thin catalytically active film upon a particulate titania or titania-containing support, especially one wherein the rutile:anatase ratio of the support is at least about 3:2. This catalyst can be used to convert an admixture of carbon monoxide and hydrogen to a distillate fuel constituted principally of an admixture of linear paraffins and olefins, particularly a C.sub.10 + distillate, at high productivity, with low methane selectivity. A process is also disclosed for the preparation of these catalysts.
摘要翻译： 通过将单独或与金属促进剂，特别是铼作为薄催化活性膜分散在颗粒二氧化钛或二氧化钛载体上，特别是其中载体的金红石：锐钛矿比在 至少约3：2。 该催化剂可用于将一氧化碳和氢气的混合物转化为主要由线性链烷烃和烯烃，特别是C10 +馏出物的混合物组成的馏出物燃料，其生产率高，甲烷选择性低。 还公开了制备这些催化剂的方法。
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6.发明授权Cobalt catalysts for the conversion of methanol and for Fischer-Tropsch synthesis to produce hydrocarbons 失效用于甲醇转化和费 - 托合成以生产碳氢化合物的钴催化剂
公开(公告)号：US4663305A
公开(公告)日：1987-05-05
申请号：US813918
申请日：1985-12-27
IPC分类号： B01J23/75 , B01J23/83 , B01J23/889 , C07C1/04 , C07C1/20 , C10G3/00 , B01J21/06 , B01J23/10 , B01J23/12 , B01J23/76
CPC分类号： C07C1/0435 , B01J23/75 , B01J23/83 , B01J23/8896 , C07C1/20 , C10G3/45 , C10G3/48 , C07C2521/06 , C07C2523/10 , C07C2523/12 , C07C2523/36 , C07C2523/75 , C07C2523/83 , C07C2523/889 , C10G2300/1022 , Y02P20/52 , Y02P30/20
摘要： A zirconium, hafnium, cerium or uranium promoted cobalt catalyst and process for the conversion of methanol or synthesis gas to hydrocarbons. Methanol is contacted, preferably with added hydrogen, over said catalyst, or synthesis gas is contacted over said catalyst to produce, at reaction conditions, an admixture of C.sub.10 + linear paraffins and olefins. These hydrocarbons can be further refined to high quality middle distillate fuels, and other valuable products such as mogas, diesel fuel, and jet fuel, particularly premium middle distillate fuels of carbon number ranging to about C.sub.20.
摘要翻译： 锆，铪，铈或铀促进了钴催化剂和将甲醇或合成气转化为烃的方法。 甲醇在所述催化剂上接触，优选与加入的氢气接触，或者合成气在所述催化剂上接触，以在反应条件下产生C10 +直链烷烃和烯烃的混合物。 这些碳氢化合物可以进一步精制成高质量的中间馏分燃料，以及其他有价值的产品，如摩尔瓦，柴油和喷气燃料，特别是碳数高于约C20的优质中间馏分燃料。
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公开(公告)号：US4762959A
公开(公告)日：1988-08-09
申请号：US57302
申请日：1987-06-04
CPC分类号： C07C1/20 , B01J23/75 , B01J23/83 , C07C1/0435 , C07C2521/06 , C07C2523/10 , C07C2523/12 , C07C2523/75 , C07C2523/83 , Y02P20/52
摘要： A zirconium, hafnium, cerium or uranium promoted cobalt catalyst and process for the conversion of methanol or synthesis gas to hydrocarbons. Methanol is contacted, preferably with added hydrogen, over said catalyst, or synthesis gas is contacted over said catalyst to produce, at reaction conditions, an admixture of C.sub.10 + linear paraffins and olefins. These hydrocarbons can be further refined to high quality middle distillate fuels, and other valuable products such as mogas, diesel fuel, and jet fuel, particularly premium middle distillate fuels of carbon number ranging to about C.sub.20.
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8.发明授权Ruthenium-rhenium catalyst on titania support for Fischer-Tropsch synthesis 失效二氧化钛上的钌 - 铼催化剂用于费 - 托合成
公开(公告)号：US4558030A
公开(公告)日：1985-12-10
申请号：US626024
申请日：1984-06-29
申请人： Kym B. Arcuri , Charles H. Mauldin , Dave H. Shaw
发明人： Kym B. Arcuri , Charles H. Mauldin , Dave H. Shaw
IPC分类号： B01J21/06 , B01J23/64 , B01J23/656 , C07C1/04
CPC分类号： B01J23/6567 , C07C1/0435 , B01J21/063 , C07C2521/06 , C07C2523/36 , C07C2523/46 , C07C2523/656
摘要： A novel ruthenium catalyst, notably a ruthenium-titania catalyst, is disclosed to which is added sufficient rhenium to obtain, at corresponding process conditions, improved activity maintenance in the production of hydrocarbons via carbon monoxide-hydrogen synthesis reactions vis-a-vis a catalyst composition otherwise similar except that it does not contain rhenium. High quality middle distillate fuels, characterized generally as admixtures of linear paraffins and olefins, are formed in a process wherein a feed mixture of carbon monoxide and hydrogen are contacted at reaction conditions over such catalyst.
摘要翻译： 公开了一种新型的钌催化剂，特别是钌 - 二氧化钛催化剂，其中加入足够的铼，以在相应的工艺条件下获得通过一氧化碳 - 氢合成反应相对于催化剂生产烃的改进的活性维持 组合物除了不含铼以外，其他方面相似。 在其中一氧化碳和氢气的进料混合物在这种催化剂上的反应条件下接触的过程中形成了高质量的中间馏分燃料，其特征通常以直链烷烃和烯烃的混合物形式。
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9.发明授权Cobalt catalysts, and use thereof for the conversion of methanol and for Fischer-Tropsch synthesis, to produce hydrocarbons 失效钴催化剂及其用于甲醇转化和费 - 托合成的用途，以生产烃
公开(公告)号：US4755536A
公开(公告)日：1988-07-05
申请号：US922885
申请日：1986-10-24
CPC分类号： C07C1/20 , B01J23/75 , B01J23/83 , C07C1/0435 , C07C2521/06 , C07C2523/10 , C07C2523/12 , C07C2523/75 , C07C2523/83 , Y02P20/52
摘要： A zirconium, hafnium, cerium or uranium promoted cobalt catalyst and process for the conversion of methanol or synthesis gas to hydrocarbons. Methanol is contacted, preferably with added hydrogen, over said catalyst, or synthesis gas is contacted over said catalyst to produce, at reaction conditions, an admixture of C.sub.10 + linear paraffins and olefins. These hydrocarbons can be further refined to high quality middle distillate fuels, and other valuable products such as mogas, diesel fuel, and jet fuel, particularly premium middle distillate fuels of carbon number ranging to about C.sub.20.
摘要翻译： 锆，铪，铈或铀促进了钴催化剂和将甲醇或合成气转化为烃的方法。 甲醇在所述催化剂上接触，优选与加入的氢气接触，或者合成气在所述催化剂上接触，以在反应条件下产生C10 +直链烷烃和烯烃的混合物。 这些碳氢化合物可以进一步精制成高质量的中间馏分燃料，以及其他有价值的产品，如摩尔瓦，柴油和喷气燃料，特别是碳数高于约C20的优质中间馏分燃料。
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公开(公告)号：US4567205A
公开(公告)日：1986-01-28
申请号：US735783
申请日：1985-05-20
申请人： Kym B. Arcuri , Charles H. Mauldin , Dave H. Shaw
发明人： Kym B. Arcuri , Charles H. Mauldin , Dave H. Shaw
IPC分类号： B01J21/06 , B01J23/656 , C07C1/04
CPC分类号： B01J23/6567 , C07C1/0435 , B01J21/063 , C07C2521/06 , C07C2523/36 , C07C2523/46 , C07C2523/656
摘要： A novel ruthenium catalyst, notably a ruthenium-titania catalyst, is disclosed to which is added sufficient rhenium to obtain, at corresponding process conditions, improved activity maintenance in the production of hydrocarbons via carbon monoxide-hydrogen synthesis reactions vis-a-vis a catalyst composition otherwise similar except that it does not contain rhenium. High quality middle distillate fuels, characterized generally as admixtures of linear paraffins and olefins, are formed in a process wherein a feed mixture of carbon monoxide and hydrogen are contacted at reaction conditions over such catalyst.
摘要翻译： 公开了一种新型的钌催化剂，特别是钌 - 二氧化钛催化剂，其中加入足够的铼，以在相应的工艺条件下获得通过一氧化碳 - 氢合成反应相对于催化剂生产烃的改进的活性维持 组合物除了不含铼以外，其他方面相似。 在其中一氧化碳和氢气的进料混合物在这种催化剂上的反应条件下接触的过程中形成了高质量的中间馏分燃料，其特征通常以直链烷烃和烯烃的混合物形式。
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