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1.发明申请HYDROTHERMAL HYDROCATALYTIC TREATMENT OF BIOMASS USING WATER TOLERANT CATALYSTS 审中-公开使用耐水催化剂的生物质的氢热水解处理
公开(公告)号：WO2014100307A2
公开(公告)日：2014-06-26
申请号：PCT/US2013076330
申请日：2013-12-19
Applicant: SHELL OIL CO , SHELL INT RESEARCH
CPC classification number: C07C29/60 , B01J21/063 , B01J21/066 , B01J23/86 , B01J23/88 , B01J23/882 , B01J27/188 , B01J27/19 , B01J35/002 , B01J35/008 , B01J35/1009 , B01J35/1014 , B01J35/1019 , B01J35/1038 , B01J35/1061 , B01J37/0201 , B01J37/20 , B01J2523/00 , C10G1/065 , C10G3/46 , C10G3/48 , C10G3/50 , C10G2300/1014 , Y02E50/343 , Y02P30/20 , B01J2523/48 , B01J2523/51 , B01J2523/68 , B01J2523/845
Abstract: A method of hydrothermal hydrocatalytic treating biomass is provided. Lignocellulosic biomass solids is provided to a hydrothermal digestion unit in the presence of a digestive solvent, and a supported hydrogenolysis catalyst containing (a) sulfur, (b) Mo or W, and (c) Co, Ni or mixture thereof, incorporated into a group 4 metal oxide support; (ii) heating the lignocellulosic biomass solids and digestive solvent in the presence of hydrogen, and the supported hydrogenolysis catalyst thereby forming a product solution containing plurality of oxygenated hydrocarbons, said catalyst retaining a crush strength of at least 50% after being subjected to an aqueous phase stability test compared with before the aqueous phase stability test or a crush strength of at least 0.25 kg after being subjected to an aqueous phase stability test.
Abstract translation: 提供了一种水热催化处理生物质的方法。 在消化溶剂存在下将木质纤维素生物质固体提供给水热消解装置，以及负载的氢解催化剂，其包含（a）硫，（b）Mo或W，和（c）Co，Ni或其混合物， 第4组金属氧化物载体; （ii）在氢气存在下加热木质纤维素生物质固体和消化溶剂，以及负载的氢解催化剂，由此形成含有多个含氧烃的产物溶液，所述催化剂在经受水溶液后保持至少50％的压碎强度 进行水相稳定性试验后的相稳定性试验或进行水相稳定性试验后的至少0.25kg的压碎强度。
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2.发明申请
公开(公告)号：WO2014100303A3
公开(公告)日：2014-08-14
申请号：PCT/US2013076325
申请日：2013-12-19
Applicant: SHELL OIL CO , SHELL INT RESEARCH
Inventor： POWELL JOSEPH BROUN , KOMPLIN GLENN CHARLES , SMEGAL JOHN ANTHONY , JOHNSON KIM ANN
CPC classification number: D21C3/006 , C07G1/00 , C10G1/065 , C10G3/46 , C10G3/50 , C10G3/56 , C10G2300/1014 , Y02P20/582 , Y02P30/20
Abstract: A method of hydrothermal hydrocatalytic treating biomass is provided. Lignocellulosic biomass solids is provided to a hydrothermal digestion unit in the presence of a digestive solvent, at least one of ammonia or a source of ammonia, and a supported hydrogenolysis catalyst containing (a) sulfur, (b) Mo or W, and (c) Co, Ni or mixture thereof, incorporated into a suitable support. The lignocellulosic biomass solids and digestive solvent are heated in the presence of hydrogen, supported hydrogenolysis catalyst and the at least one of ammonia or a source of ammonia forming a product solution containing plurality of oxygenated hydrocarbons and ammonia. At least a portion of ammonia is separated and recycled to the hydrothermal digestion unit.
Abstract translation: 提供了一种水热催化处理生物质的方法。 在消解溶剂，氨或氨源中的至少一种和含有（a）硫，（b）Mo或W和（c）的负载氢解催化剂的存在下，向水热消解单元提供木质纤维素生物质固体。 ）Co，Ni或其混合物，并入合适的载体中。 木质纤维素生物质固体和消化溶剂在氢气，负载氢解催化剂和氨或氨源中的至少一种的存在下加热，形成含有多个含氧烃和氨的产物溶液。 将氨的至少一部分分离并再循环至水热消解装置。
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公开(公告)号：WO2007121219A3
公开(公告)日：2008-01-17
申请号：PCT/US2007066395
申请日：2007-04-11
Applicant: SHELL OIL CO , SHELL INT RESEARCH , KOMPLIN GLENN CHARLES , SMEGAL JOHN ANTHONY
Inventor： KOMPLIN GLENN CHARLES , SMEGAL JOHN ANTHONY
IPC: B01J21/04 , B01J23/883 , B01J37/02 , C07C29/141
CPC classification number: B01J23/883 , B01J21/04 , B01J35/10 , B01J35/1014 , B01J37/0201 , C07C29/141 , C07C31/205
Abstract: The present invention relates to a process for hydrogenating an aldehyde. An aldehyde is contacted with a catalyst comprising a support containing at least 95% a-alumina and non-support metals dispersed on the surface of the support. The non-support metals comprise nickel and/or one or more compounds thereof and molybdenum and/or one or more compounds thereof. The nickel and/or one or more compounds thereof comprise from 3 wt.% to 9 wt.% of the catalyst, by metallic weight, and the molybdenum and/or one or more compounds thereof comprise from 1 wt.% to 4 wt.% of the catalyst, by metallic weight.
Abstract translation: 本发明涉及一种氢化醛的方法。 将醛与包含分散在载体表面上的至少95％的α-氧化铝和非支撑金属的载体的催化剂接触。 非支撑金属包含镍和/或其一种或多种化合物，钼和/或其一种或多种化合物。 镍和/或其一种或多种化合物包含3重量％至9重量％的催化剂，以金属重量计，并且钼和/或其一种或多种化合物包含1重量％至4重量％ ％的催化剂，以金属重量计。
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Patent Agency Ranking4.发明申请HYDROTHERMAL HYDROCATALYTIC TREATMENT OF BIOMASS USING WATER TOLERANT CATALYSTS 审中-公开用耐水催化剂水热法加氢处理生物质
公开(公告)号：WO2014100304A3
公开(公告)日：2014-08-14
申请号：PCT/US2013076327
申请日：2013-12-19
Applicant: SHELL OIL CO , SHELL INT RESEARCH
CPC classification number: C10L1/1802 , B01J21/04 , B01J23/86 , B01J23/88 , B01J23/882 , B01J35/0046 , B01J35/026 , B01J35/1009 , B01J35/1014 , B01J35/1066 , B01J37/0201 , B01J37/20 , C10G1/065 , C10G3/46 , C10G3/48 , C10G3/50 , C10G2300/1014 , Y02E50/13 , Y02P30/20
Abstract: A method of hydrothermal hydrocatalytic treating biomass is provided. Lignocellulosic biomass solids is provided to a hydrothermal digestion unit in the presence of a digestive solvent, and a supported hydrogenolysis catalyst containing (a) sulfur, (b) Mo or W, and (c) Co, Ni or mixture thereof, incorporated into an alumina support, which support is predominantly alpha alumina; (ii) heating the lignocellulosic biomass solids and digestive solvent in the presence of hydrogen, and supported hydrogenolysis catalyst thereby forming a product solution containing plurality of oxygenated hydrocarbons, said alumina support having a specific surface area of up to 30 m2/g and said catalyst retaining a crush strength of at least 50% after being subjected to an aqueous phase stability test compared with before the aqueous phase stability test or a crush strength of at least 0.25 kg after being subjected to an aqueous phase stability test.
Abstract translation: 提供了一种水热加氢催化处理生物质的方法。 将木质纤维素生物质固体在消化溶剂和含有（a）硫，（b）Mo或W，和（c）Co，Ni或其混合物的载体氢解催化剂的情况下提供给水热消化装置， 氧化铝载体，该载体主要是α-氧化铝; （ii）在氢气存在下加热木质纤维素生物质固体和消化溶剂，并负载氢解催化剂，由此形成含有多种氧化烃的产物溶液，所述氧化铝载体具有至多30m 2 / g的比表面积，并且所述催化剂 与进行水相稳定性试验前相比，在进行水相稳定性试验后保持至少50％的抗碎强度或在进行水相稳定性试验后至少0.25kg的抗碎强度。
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5.发明申请AN AMORPHOUS SILICA-ALUMINA COMPOSITION AND A METHOD OF MAKING AND USING SUCH COMPOSITION 审中-公开一种无定形二氧化硅 - 氧化铝组合物及其制备和使用方法
公开(公告)号：WO2009029580A2
公开(公告)日：2009-03-05
申请号：PCT/US2008074221
申请日：2008-08-25
Applicant: SHELL OIL CO , SHELL INT RESEARCH , ACKERMAN RUSSELL CRAIG , MICHEL CHRISTIAN GABRIEL , SMEGAL JOHN ANTHONY , VAN VEEN JOHANNES ANTHONIUS RO
Inventor： ACKERMAN RUSSELL CRAIG , MICHEL CHRISTIAN GABRIEL , SMEGAL JOHN ANTHONY , VAN VEEN JOHANNES ANTHONIUS ROBERT
CPC classification number: B01J21/12 , B01J23/42 , B01J23/44 , B01J35/023 , B01J35/1019 , B01J35/1042 , B01J35/1047 , B01J35/1061 , B01J35/1066 , B01J37/0009 , C07C5/10 , C07C2523/44 , C10G45/46 , C10G45/52 , C10G2300/1096
Abstract: Described is a novel amorphous silica-alumina composition having a high ratio of pore volume contained in large pores to pore volume contained in medium to small pores. The amorphous silica-alumina composition also may have the characteristic of a strong aluminum-NMR penta-coordinated peak representing greater than 30% of the total aluminum and a method of making such novel amorphous silica-alumina composition using a pH swing preparation method.
Abstract translation: 描述了一种新型无定形二氧化硅 - 氧化铝组合物，其具有大孔隙中包含的孔隙体积与中孔隙至小孔隙中包含的孔隙体积的高比率。 无定形二氧化硅 - 氧化铝组合物还可以具有代表大于总铝量30％的强铝-NMR五配位峰的特征，以及使用pH摆动制备方法制备这种新型无定形二氧化硅 - 氧化铝组合物的方法。
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6.发明申请A COMPOSITION USEFUL IN THE CATALYTIC HYDROPROCESSING OF HYDROCARBON FEEDSTOCKS, A METHOD OF MAKING SUCH CATALYST, AND A PROCESS OF USING SUCH CATALYST 审中-公开烃类催化剂催化氢化有用的组合物，制备这种催化剂的方法和使用这种催化剂的方法
公开(公告)号：WO2009020913A3
公开(公告)日：2009-09-11
申请号：PCT/US2008072092
申请日：2008-08-04
Applicant: SHELL OIL CO , SHELL INT RESEARCH , GABRIELOV ALEXEI GRIGORIEVICH , SMEGAL JOHN ANTHONY , TORRISI SALVATORE PHILIP
IPC: B01J21/04 , B01J23/75 , B01J23/755 , B01J27/185 , B01J37/02 , B01J37/18 , B01J37/20 , C10G45/06
CPC classification number: B01J23/883 , B01J21/04 , B01J23/24 , B01J23/74 , B01J23/85 , B01J27/185 , B01J37/0009 , B01J37/0201 , B01J37/0203 , B01J37/18 , B01J37/20 , C10G45/06 , C10G45/08 , C10G2400/04
Abstract: A hydrocarbon oil-impregnated composition that comprises a support material having incorporated therein a metal component and impregnated with a hydrocarbon oil. The hydrocarbon oil-impregnated composition is useful in the hydrotreating of hydrocarbon feedstocks, and it is especially useful in applications involving delayed feed introduction whereby the hydrocarbon oil-impregnated composition is first treated with hot hydrogen, and, optionally, a sulfur compound, prior to contacting it with a hydrocarbon feedstock under hydrodesulfurization process conditions.
Abstract translation: 一种烃油浸渍的组合物，其包括其中掺入金属组分并浸渍有烃油的载体材料。 烃油浸渍的组合物可用于烃原料的加氢处理，特别适用于涉及延迟进料引入的应用，其中烃油浸渍的组合物首先用热氢和任选的硫化合物在 在加氢脱硫工艺条件下将其与烃原料接触。
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7.发明申请METHOD FOR DECOMPOSING DI(PHENYLALKYL)PEROXIDES TO PRODUCE HYDROXYBENZENES AND PHENYLALKENES USING SOLID CATALYSTS 审中-公开使用固体催化剂分解DI（苯甲醇）过氧化物生产羟基苯甲酸和苯乙烯的方法
公开(公告)号：WO2007137020A3
公开(公告)日：2008-07-31
申请号：PCT/US2007068855
申请日：2007-05-14
Applicant: SHELL OIL CO , SHELL INT RESEARCH , SAUKAITIS JOHN CHARLES , SMEGAL JOHN ANTHONY
Inventor： SAUKAITIS JOHN CHARLES , SMEGAL JOHN ANTHONY
CPC classification number: C07C37/08 , B01J21/08 , B01J23/30 , B01J37/0205 , C07C1/20 , C07C2521/06 , C07C2523/06 , C07C2523/10 , C07C2523/14 , C07C2523/30 , Y02P20/52 , C07C15/44 , C07C39/04
Abstract: A method for decomposing di(phenylalkyl)peroxides to hydroxybenzenes and phenylalkene(s) using solid catalyst.
Abstract translation: 使用固体催化剂将二（苯基烷基）过氧化物分解成羟基苯和苯基烯烃的方法。
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8.发明申请CATALYSTS COMPRISING A COMBINATION OF OXIDIZED METALS AND A METHOD FOR CLEAVING PHENYLALKYL HYDROPEROXIDES USING THE CATALYSTS 审中-公开包含氧化金属组合的催化剂和使用催化剂清洗苯乙烯氢过氧化物的方法
公开(公告)号：WO2007137021A3
公开(公告)日：2008-04-10
申请号：PCT/US2007068860
申请日：2007-05-14
Applicant: SHELL OIL CO , SHELL INT RESEARCH , MYSORE NARAYANA , SAUKAITIS JOHN CHARLES , SMEGAL JOHN ANTHONY
Inventor： MYSORE NARAYANA , SAUKAITIS JOHN CHARLES , SMEGAL JOHN ANTHONY
CPC classification number: B01J37/0207 , B01J23/002 , B01J23/14 , B01J23/18 , B01J23/30 , B01J23/31 , B01J23/888 , B01J37/0205 , B01J2523/00 , C07C37/08 , C07C45/53 , Y02P20/52 , C07C49/08 , B01J2523/3712 , B01J2523/69 , B01J2523/54 , B01J2523/43 , B01J2523/48 , B01J2523/842 , B01J2523/53 , B01J2523/27 , C07C39/04
Abstract: Catalyst comprising a combination of oxidized metals and processes for cleaving phenylalkyl hydroperoxides in the presence of the catalyst.
Abstract translation: 催化剂包含氧化金属的组合和在催化剂存在下裂解苯基烷基氢过氧化物的方法。
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