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    Method of producing polyhydroxyalkanoate from alkane having residue containing aromatic ring in its molecule
    43.
    发明授权
    Method of producing polyhydroxyalkanoate from alkane having residue containing aromatic ring in its molecule 失效
    从其分子中含有芳环的残基的烷烃生产聚羟基链烷酸酯的方法

    公开(公告)号：US07056708B2

    公开(公告)日：2006-06-06

    申请号：US10410349

    申请日：2003-04-10

    申请人： Takashi Kenmoku ,  Etsuko Sugawa ,  Tetsuya Yano ,  Takeshi Imamura ,  Tsutomu Honma

    发明人： Takashi Kenmoku ,  Etsuko Sugawa ,  Tetsuya Yano ,  Takeshi Imamura ,  Tsutomu Honma

    IPC分类号： C12P11/00 ,  C12P7/62

    CPC分类号： C08G63/6882 ,  C12P7/625 ,  C12P11/00

    摘要： The present invention provides a method of effectively producing polyhydroxyalkanoate having an aromatic substituted residue in its monomer unit. In the method of producing polyhydroxyalkanoate by using microorganisms, microorganisms capable of producing polyhydroxyalkanoate are cultured in a culture medium containing at least one starting compound selected from the group consisting of substituted alkanes represented by formula (1) to produce polyhydroxyalkanoate having, in its molecule, at least one unit selected from the group consisting of 3-hydroxy-substituted alkanoate units represented by formula (2): R—(CH2)n—CH2—CH2—CH3  (1) wherein R represents a residue containing a substituted aromatic ring, and n represents any integer of 1 to 8; wherein R represents a residue containing a substituted aromatic ring, and n represents any integer of 1 to 8. In formulas (1) and (2), a residue R is as described in the specification.

    摘要翻译： 本发明提供了在其单体单元中有效制备具有芳族取代残基的聚羟基链烷酸酯的方法。 在通过使用微生物制备聚羟基链烷酸酯的方法中，能够在含有选自由式（1）表示的取代烷烃中的至少一种起始化合物的培养基中培养能够产生聚羟基链烷酸酯的微生物，从而产生在其分子中具有的聚羟基链烷酸酯， 选自由式（2）表示的3-羟基取代的链烷酸酯单元中的至少一个单元：<？in-line-formula description =“In-line Formulas”end =“lead”？> R-（CH （2）-CH 2 CH 2 CH 2 CH 2（1） 其中，R表示含有取代芳环的残基，n表示1〜8的整数，n表示1〜8的整数。 其中R表示含有取代芳环的残基，n表示1至8的任何整数。在式（1）和（2）中，残基R如说明书所述。

    Polyhydroxyalkanoate, method for production thereof and microorganisms for use in the same
    45.
    发明授权
    Polyhydroxyalkanoate, method for production thereof and microorganisms for use in the same 失效
    聚羟基链烷酸酯，其制备方法和用于其的微生物

    公开(公告)号：US06586562B2

    公开(公告)日：2003-07-01

    申请号：US09748205

    申请日：2000-12-27

    申请人： Tsutomu Honma ,  Toyoko Kobayashi ,  Tetsuya Yano ,  Shin Kobayashi ,  Takeshi Imamura ,  Sakae Suda ,  Takashi Kenmoku

    发明人： Tsutomu Honma ,  Toyoko Kobayashi ,  Tetsuya Yano ,  Shin Kobayashi ,  Takeshi Imamura ,  Sakae Suda ,  Takashi Kenmoku

    IPC分类号： C08G6306

    CPC分类号： C12P7/62 ,  C08G63/06 ,  C08G63/6822 ,  C08G63/6852 ,  Y10S435/874

    摘要： A polyhydroxyalkanoate having a monomer unit composition represented by General Formula (1): AmB(1−m)  (1) wherein A is represented by General Formula (2), B is at least one selected from the group consisting of monomer units represented by General Formula (3) or (4), and m has a value of 0.01 or larger and smaller than 1:  wherein n has a value of 0 to 10, k has a value of 3 or 5, and R is at least one group selected from the group consisting of groups represented by General Formulae (5) to (7):  in Formula (5) R1 is a group selected from the group consisting of a hydrogen atom (H), halogen atoms, —CN, —NO2, —CF3, —C2F5 and —C3F7; and q is an integer selected from 1 to 8;  in Formula (6) R2 is a group selected from the group consisting of a hydrogen atom (H), halogen atoms, —CN, —NO2, —CF3, —C2F5 and —C3F7; and r is an integer selected from 1 to 8;  in Formula (7) R3 is a group selected from the group consisting of a hydrogen atom (H), halogen atoms, —CN, —NO2, —CF3, —C2F5 and —C3F7; and s is an integer selected from 1 to 8. The efficient production methods are also provided.

    摘要翻译： 具有由通式（1）表示的单体单元组成的聚羟基链烷酸酯：其中A由通式（2）表示，B为选自由通式（3）或（4）表示的单体单元中的至少一种， ，m的值为0.01以上且小于1，其中n为0〜10，k为3或5，R为选自由通式 （5）〜（7）中，式（5）中，R 1为选自氢原子（H），卤素原子，-CN，-NO 2，-CF 3，-C 2 F 5和-C 3 F 7的基团。 q为选自1至8的整数; 在式（6）中，R 2是选自氢原子（H），卤素原子，-CN，-NO 2，-CF 3，-C 2 F 5和-C 3 F 7的基团; 并且r是选自1至8的整数; 在式（7）中，R 3是选自氢原子（H），卤素原子，-CN，-NO 2，-CF 3，-C 2 F 5和-C 3 F 7的基团; s是选自1至8的整数。还提供了有效的制备方法。

    Novel polyhydroxyalkanoate having amide, sulfonic acid or sulfonate ester group, charge control agent and toner
    48.
    发明申请
    Novel polyhydroxyalkanoate having amide, sulfonic acid or sulfonate ester group, charge control agent and toner 失效
    具有酰胺，磺酸或磺酸酯基的新型聚羟基链烷酸酯，电荷控制剂和调色剂

    公开(公告)号：US20060287473A1

    公开(公告)日：2006-12-21

    申请号：US11172662

    申请日：2005-06-24

    申请人： Tatsuki Fukui ,  Tetsuya Yano ,  Chieko Mihara ,  Shinya Kozaki ,  Tsutomu Honma ,  Takashi Kenmoku ,  Ako Kusakari

    发明人： Tatsuki Fukui ,  Tetsuya Yano ,  Chieko Mihara ,  Shinya Kozaki ,  Tsutomu Honma ,  Takashi Kenmoku ,  Ako Kusakari

    IPC分类号： C08G63/02

    CPC分类号： C08G63/912 ,  C08G63/6852 ,  C08G63/6882 ,  G03G9/08755 ,  G03G9/08791

    摘要： The invention provides a novel polyester adapted for use in a charge control agent for a toner for an electrophotographic process, having a charge stability, a high charge amount, an improved dispersibility and a biodegradability, and a producing method and an application technology therefor. According to the invention, there is provided polyhydroxyalkanoate comprising at least one unit represented by the following chemical formula in a molecule: —(O—CH(—(CH2)m—CH2-p-C6H4—CONH-A1SO2R1)CH2CO)— (wherein R1 represents OH, a halogen atom, ONa, OK or OR1a; A1 and R1a each represents a substituted or unsubstituted aliphatic hydrocarbon structure, a substituted or unsubstituted aromatic cyclic structure or a substituted or unsubstituted heterocyclic structure; m represents an integer selected from a range of 0 to 7; and R1, A1, R1a and m have the aforementioned meanings independently for each unit when plural units are present), a charge control agent containing such polyhydroxyalkanoate, a toner utilizing such charge control agent, and an image forming method and an image forming apparatus utilizing such toner.

    摘要翻译： 本发明提供一种适用于电荷控制剂用电荷控制剂的新型聚酯，其具有电荷稳定性，高电荷量，改进的分散性和生物降解性，以及其制备方法和应用技术。 根据本发明，提供了在分子中包含由以下化学式表示的至少一个单元的聚羟基链烷酸酯：<？in-line-formula description =“In-line Formulas”end =“lead”→> - （O- CH（ - （CH 2 CH 2）m CH 2 CH 2 CH 2 CH 2 CH 2 - -CONH-A 1 2 1 CO 2） （其中R 1表示OH，卤素原子，ONa，OK或OR 1a; A < 取代或未取代的脂族烃结构，取代或未取代的芳族环状结构或取代或未取代的杂环结构; m表示选自以下的整数; R 1，R 2， 0至7;当存在多个单元时，R 1，A 1，R 1a和m对于每个单元具有上述含义 ），含有这种聚羟基链烷酸酯的电荷控制剂 e，使用这种电荷控制剂的调色剂，以及使用这种调色剂的图像形成方法和图像形成装置。

    Novel polyhydroxy alkanoate copolymer including within molecule unit having vinyl group or carboxyl group in side chain, and producing method therefor
    49.
    发明申请
    Novel polyhydroxy alkanoate copolymer including within molecule unit having vinyl group or carboxyl group in side chain, and producing method therefor 有权
    在侧链中具有乙烯基或羧基的分子单元内的新型多羟基链烷酸酯共聚物及其制造方法

    公开(公告)号：US20060211100A1

    公开(公告)日：2006-09-21

    申请号：US10531689

    申请日：2003-10-23

    申请人： Takashi Kenmoku ,  Tetsuya Yano ,  Chieko Mihara ,  Shinya Kozaki ,  Tsutomu Honma ,  Tatsuki Fukui ,  Takeshi Imamura ,  Etsuko Sugawa

    发明人： Takashi Kenmoku ,  Tetsuya Yano ,  Chieko Mihara ,  Shinya Kozaki ,  Tsutomu Honma ,  Tatsuki Fukui ,  Takeshi Imamura ,  Etsuko Sugawa

    IPC分类号： C12P7/62 ,  C08G63/87

    CPC分类号： C08G63/06 ,  C08G63/6882 ,  C12P7/625

    摘要： The invention provides a PHA copolymer including at least a 3-hydroxy-ω-carboxyalkanoic acid represented by a formula (19) or (32) and simultaneously at least a unit represented by a formula (2) or a formula (3) in a molecule, a precursor PHA copolymer having a corresponding vinyl group or a corresponding alkoxycarbonyl group, a biosynthesis method thereof by microorganisms, and a method of producing a desired PHA copolymer from the precursor PHA copolymer: (wherein k, m, n are integers; R18 represents H, Na, K, R27? represents (A); R1 represents a substituent on a cyclohexyl group and represents H, CN, NO2, a halogen atom, CH3, C2H5, C3H7, CF3, C2F5, or C3F7; R includes a residue including a phenyl structure or a thienyl structure; these being independent for each unit).

    摘要翻译： 本发明提供一种PHA共聚物，其包含至少一种由式（19）或（32）表示的3-羟基-ω-羧基烷酸，同时至少由式（2）或式（3）表示的单元在 分子，具有相应的乙烯基或相应的烷氧基羰基的前体PHA共聚物，微生物的生物合成方法以及由前体PHA共聚物制备所需PHA共聚物的方法（其中k，m，n为整数; R 表示H，Na，K，R “custom 27？表示（A）; R 1表示环己基上的取代基，代表H，CN ，NO 2 2，卤素原子，CH 3，C 2 H 5，C 3， H 3，CF 3，C 2 H 5，或C 3 H 3， R> R包括残基 e包括苯基结构或噻吩基结构; 这些对于每个单元是独立的）。

    Production method of polyester containing epoxy group in side chain and production method of crosslinked polymer
    50.
    发明授权
    Production method of polyester containing epoxy group in side chain and production method of crosslinked polymer 失效
    侧链中含有环氧基的聚酯的生产方法和交联聚合物的制备方法

    公开(公告)号：US06872788B2

    公开(公告)日：2005-03-29

    申请号：US10427919

    申请日：2003-05-02

    申请人： Takeshi Imamura ,  Etsuko Sugawa ,  Tetsuya Yano ,  Shin Kobayashi ,  Tsutomu Honma ,  Takashi Kenmoku

    发明人： Takeshi Imamura ,  Etsuko Sugawa ,  Tetsuya Yano ,  Shin Kobayashi ,  Tsutomu Honma ,  Takashi Kenmoku

    IPC分类号： C12N1/28 ,  C12P7/62 ,  C08F20/00

    CPC分类号： C12P7/625 ,  C12N1/28 ,  Y10S435/874

    摘要： A method is provided which biosynthesizes a PHA having an epoxy group on a side chain with improved physicochemical properties. Specifically, a method of producing a polyester containing an epoxy group in a side chain thereof using alkene as a raw material is provided which comprises the steps of bringing alkene into contact with a microorganism having an ability to uptake alkene and convert it to a polyester and allowing the microorganism to convert the alkene into a polyester containing an epoxy group in a side chain thereof. Further, a method of producing a crosslinked polymer is provided which comprises reacting the polyester obtained by the above mentioned method with a diamine compound.

    摘要翻译： 提供一种方法，其生物合成具有改善的物理化学性质的侧链上具有环氧基的PHA。 具体地说，提供了使用烯烃作为原料在其侧链中制备含有环氧基的聚酯的方法，其包括使烯与具有吸收烯烃的能力并将其转化为聚酯的微生物接触的步骤，以及 允许微生物将烯烃转化成其侧链中含有环氧基的聚酯。 此外，提供了一种制备交联聚合物的方法，其包括使通过上述方法获得的聚酯与二胺化合物反应。